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PP-I-32Conversion and selectivity are discussed. The model developed well-predicts both partialoxidation and steam reforming of methane on Ni catalysts at the wide range of temperatureand steam/methane ratio.References[1] J.R. Rostrup-Nielsen & J.H.B. Hansen. J. Catal. 144 (1993) 38-49[2] H. Zhu, R. J. Kee, V.M. Janardhanan, O. Deutschmann, D.G. Goodwin. J. Electrochemical Soc.152 (2005) A2427-A2440[3] E. Hecht, G.K. Gupta, H. Zhu. A.M. Dean, R.J. Kee, L. Maier, O. Deutschmann. AppliedCatalysis A: General 295 (2005) 40–51;[4] S.Tischer, C. Correa, O. Deutschmann. Catalysis Today 69 (2001) 57-62; www.detchem.com66
PP-I-33HYDROGEN PEROXIDE OXIDATION OF SATURATED HYDROCARBONSCATALYZED BY IRON(<strong>III</strong>) CHLORIDE AND 2,2’-BIPYRIDINEMandelli D., Shul’pina L.S. 1 , Golfeto C.C., Shul’pin G.B. 2Pontifícia Universidade Católica de Campinas, Faculdade de Química, Rod. D. Pedro I,km 136, Pq. das Universidades, Campinas, SP, 13086-900, Brazil1Nesmeyanov Institute of Organoelement Compounds, Russian Academy of Sciences,Moscow, Russia2N.N. Semenov Institute of Chemical Physics, Russian Academy of Sciences, Moscow, RussiaE-mail: dalmo_mandelli@mail.ruThe H 2 O 2 –FeCl 3 –bipy system in acetonitrile efficiently oxidizes alkanes predominantlyto alkyl hydroperoxides. Turnover numbers attain 500 after 1 h at 60 ºC. It has been assumedthat bipy facilitates proton abstraction from a H 2 O 2 molecule coordinated to the iron ion(these reactions are stages in the catalytic cycle generating hydroxyl radicals from thehydrogen peroxide). Hydroxyl radicals then attack alkane molecules finally yielding the alkylhydroperoxide.In the course of our studies of iron-catalyzed hydrocarbon oxygenations with peroxides[1] we explored the possibility of enhancing the reaction efficiency by addition of certainamines. Here we report that 2,2’-bipyridine added to iron(<strong>III</strong>) chloride used as a catalystaccelerates oxidation of alkanes with hydrogen peroxide in acetonitrile. Main features of thereaction will be discussed.Acknowledgments. This work was supported by the Russian Basic Research Foundation(06-03-32344-a), the State of São Paulo Research Foundation (FAPESP, 2002/08495-4,06/03984-8), the Brazilian National Council on Scientific and Technological Development(CNPq, 300984/2004-9, 300601/01-8). G. B. Sh. expresses his gratitude to FAPESP, CNPq,Faculdade de Química, Pontifícia Universidade Católica de Campinas (PUC) for making itpossible for him to stay at PUC as invited Professor and to perform a part of the present work.References1. G. B. Shul’pin, J. Mol. Catal., A: Chem. 2002, 189, 39–66. G. B. Shul’pin, Comptes Rend. Chim.2003, 6, 163–178. G. V. Nizova; B. Krebs; G. Süss-Fink; S. Schindler; L. Westerheide;L. Gonzalez Cuervo; G. B. Shul’pin, Tetrahedron 2002, 58, 9231–9237. G. B. Shul’pin;H. Stoeckli-Evans; D. Mandelli; Y. N. Kozlov; A. Tesouro Vallina; C. B. Woitiski;R. S. Jimenez; W. A. Carvalho, J. Mol. Catal. A: Chem. 2004, 219, 255–264. G. B. Shul’pin;G. V. Nizova; Y. N. Kozlov; L. Gonzalez Cuervo; G. Süss-Fink, Adv. Synth. Catal. 2004, 346,317–332. G. B. Shul’pin, C. C. Golfeto, G. Süss-Fink, L. S. Shul’pina, D. Mandelli, TetrahedronLett., 2005, 46, 4563–4567.67
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"Catalysis is not a branch of chemi
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Siberian Branch of Russian Academy
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INTERNATIONAL ADVISORY COMMITTEE:A.
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POSTER PRESENTATIONSSECTION IMECHAN
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PP-I-1more time in the oxidised sta
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PP-I-2Study of chemical reactions p
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PP-I-3It is suggested that during p
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PP-I-4reaction conditions, 100% con
Page 18 and 19: PP-I-5Catalytic properties of synth
Page 20 and 21: PP-I-6iii) The magnitude of above m
Page 22 and 23: PP-I-8ONE-DIMENSIONAL AND THREE-DIM
Page 24 and 25: PP-I-8This work was carried out at
Page 26 and 27: PP-I-9formed on their place. The PI
Page 28 and 29: PP-I-10CatalystЕа 1 ,kJ/mol(77÷1
Page 30 and 31: PP-I-11to increase of selectivity t
Page 32 and 33: PP-I-12The nanostructure of CS (clu
Page 34 and 35: PP-I-13The exchange in high-tempera
Page 36 and 37: PP-I-15ROLE OF CARBON DIOXIDE IN TH
Page 38 and 39: PP-I-16DIRECT OXIDATION OF BENZENE
Page 40 and 41: PP-I-17DFT STUDY OF REDUCTION REACT
Page 42 and 43: PP-I-18ORIGINAL MONTE CARLO METHOD
Page 44 and 45: PP-I-19STUDY ON THE MECHANISM OF TH
Page 46 and 47: PP-I-20NANOSIZED METAL OXIDES AS ST
Page 48 and 49: PP-I-21THE STUDYING OF THE NATURE O
Page 50 and 51: PP-I-22SYNTHESIS OF ETHYLENE-BUTADI
Page 52 and 53: PP-I-24REACTION OF PHENYLACETYLENE
Page 54 and 55: PP-I-25EFFECT OF THE PRESSURE ON TH
Page 56 and 57: PP-I-26INTERPRETATION OF THE ETHYLE
Page 58 and 59: PP-I-27STUDY OF ONE-POT REDUCTIVE D
Page 60 and 61: PP-I-28TUNING SURFACE MORPHOLOGY OF
Page 62 and 63: PP-I-29HIGHLY POROUS BLOCK CELLULAR
Page 64 and 65: PP-I-30STRUCTURE OF PHOTOCATALYTIC
Page 66 and 67: PP-I-31According to the 13 C MAS NM
Page 70 and 71: PP-I-34STUDY OF THE MECHANISM OF CA
Page 72 and 73: PP-I-35COMPARISON CATALYTIC ACTIVIT
Page 74 and 75: PP-I-36CRITICAL PHENOMENA FOR LANGM
Page 76 and 77: PP-I-37ISOTHERMS FOR STEPPED SURFAC
Page 78 and 79: PP-I-38RESOLUTION OF CHIRAL SULFOXI
Page 80 and 81: PP-I-39INVESTIGATION OF AMINO-CONTA
Page 82 and 83: PP-I-40APPLICATION OF POSITRON ANNI
Page 84 and 85: PP-I-41large pores (15-100 μm) of
Page 86 and 87: PP-I-42 Pd(1x2) Pd(1x1) Pd(1x2)-c
Page 88 and 89: PP-I-43the Al/Zr molar ratio has an
Page 90 and 91: PP-I-44transferred on nickel throug
Page 92 and 93: PP-I-45S BET , XRD, TPR, SEM, TEM a
Page 94 and 95: PP-I-46normal and branched alkanes
Page 96 and 97: PP-I-47growth stages (2) and (3) -
Page 98 and 99: PP-I-48system operated at frequenci
Page 100 and 101: PP-I-49The reactivity of these mate
Page 102 and 103: PP-I-51RECONSTRUCTION OF THE Pd(pol
Page 104 and 105: PP-I-53INTERMEDIATE PRODUCTS IN PAR
Page 106 and 107: PP-I-55MOLECULAR MECHANISM OF LOW T
Page 108 and 109: PP-I-56size of metals encapsulated
Page 110 and 111: PP-I-57activity of synthetic cataly
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Page 114 and 115: PP-I-59characteristics are as follo
Page 116 and 117: PP-I-60surfaces changes at 50% cove
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PP-I-611) using the parameter conti
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PP-I-62atoms to PhePA molecule. In
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PP-I-63interaction of CO molecule b
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PP-I-64cases method of Coats-Redfer
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PP-I-65adsorbates and metal atoms.
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PP-I-66were extrapolated then to th
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PP-I-67account an influence of oxyg
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PP-I-68been considered. With this a
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PP-I-70MODIFICATION OF ELECTRONIC S
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PP-I-71most of described methods ch
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PP-I-72Table 1Polymeric active carb
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PP-I-73lower than 450 °C with prac
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PP-I-74Fig. 1. Optimized structure
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PP-I-75(Zn Z d ). The catalytic cyc
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PP-I-76Photocatalytic reaction was
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PP-I-78FRAGMENT COMPOSITION OF DIES
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PP-I-79QUANTUM-CHEMICAL STUDIES OF
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PP-I-80INFUENCE OF CHEMICAL TREATME
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PP-I-81ADSORPTION OF SMALL SILVER S
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PP-I-82EXPLOSION SAFETY IN GAS TRAN
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PP-I-83(ONNO) ad → N 2 O ad + O a
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CATALYTIC ACTIVATION OF UNFAVOURABL
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PP-II-1Therefore, the observed incr
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PP-II-2The samples of uranium oxide
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PP-II-3catalysts prepared by hydrot
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PP-II-4[(C 6 H 5 ) 2 (CH 2 =CHSi] 2
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PP-II-6THE NEW Ni, Zr, Ti-CONTAININ
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PP-II-7SPATIALLY RESOLVED UV-VIS MI
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PP-II-8POLYOL MEDIATED SYNTHESIS OF
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PP-II-8CuO phase were detected, sug
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PP-II-9SHS-INTERMETALLIDES ON THE B
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PP-II-10CO OXIDATION IN HYDROGEN ST
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PP-II-11CATALYTIC PERFORMANCE OF CO
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PP-II-12FORMATION OF RADICAL CATION
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CATALYSTS MOLECULAR DESIGN BY SURFA
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PP-II-14THE CATALYTIC ACTIVITY OF F
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OXIDATION TRIMETHYLHYDROHYNONE IN T
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PP-II-16TECHNOLOGY CONCEPTS ON DEVE
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ACTIVATION OF POST-TITANOCENE OLEFI
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STRUCTURE FEATURES OF NANOCRYSTALLI
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THE H 2 ROLE IN SELECTIVE NO X REDU
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PP-II-20THE IN SITU FTIR STUDY OF T
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PP-II-21LUMINESCENT DIAGNOSTICS OF
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PP-II-22MODIFICATION OF PROPERTIES
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PP-II-23FTIR STUDY OF THE REACTION
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PP-II-24pores (the average diameter
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PP-II-25and the amount of the disso
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PP-II-27ACTIVITY OF PALLADIUM CATAL
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MODIFIED POLYOXIDE CATALYSTS FOR SY
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PP-II-29PRODUCTION OF HYDROGENCONTA
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INFLUENCE OF COMPOSITION AND STRUCT
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PP-II-311NEW COMPOSITE OF A POLYACE
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SOME ASPECTS OF THE SELECTION OF ST
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PP-II-33HYDROTREATING CATALYSTS MOD
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PP-II-34NORBORNADIENE IN NEW SHAPE-
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PP-II-36CATALYTIC SYSTEMS BASED ON
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PP-II-37EFFECT OF PHYSIOCHEMICAL PR
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PP-II-38INVESTIGATION OF STRUCTURE
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PP-II-38As a result of the combined
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PP-II-39synthesized by deposition-p
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PP-II-40halogen in NiX 2 (PPh 3 ) 2
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PP-II-41fell cell - with the requir
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PP-II-42SYNTHESIS OF CATALYSTS ON T
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PP-II-43-crucial role play peroxide
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PP-II-44According to the obtained d
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PP-II-46CYCLOALUMINATION OF α,ω-D
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PP-II-47ETHYLENE OLIGOMERIZATION TO
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PP-II-48aluminas are in the range o
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PP-II-49synthesis methods such as s
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PP-II-50Here, we report the first s
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PP-II-51hydrogenation. This peculia
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PP-II-524% and higher. Apparently t
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PP-II-53The secondary methods are b
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PP-II-55NOVEL CHIRAL NITROGEN CONTA
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PP-II-56NON-OXIDATIVE METHANE CONVE
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PP-II-57THE CATALYTIC ACTIVITY OF P
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PP-II-58The analysis of the raw mat
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PP-II-59analysis. Specific surface
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PP-II-60Ni-U catalysts were shown t
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PP-II-61Deep oxidation of CB vapors
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PP-II-62precipitate at 100 o C favo
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PP-II-63Х X n-С н-C 6 , %1008060
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PP-II-64mixture by microwave radiat
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PP-II-65and 99.995 % mass.) were sa
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PP-II-66CATALYTIC SYSTEMS BASED ON
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PHASE ANALYSIS OF MULTIELEMENT CATA
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PP-II-68EFFECT OF THE LIGAND SUBSTI
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PP-II-69Results and discussion: The
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PP-II-70tests in POM reaction and T
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PP-II-71The acidity, measured by tw
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PP-II-72The effect of nature and ac
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PP-II-74STUDY OF METHANE DEHYDROARO
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PP-II-75CATALYTIC OXIDATION OF ORGA
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Knowledge of the surface VO x speci
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PP-II-77propylene polymerization on
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THE EFFECT OF THE SUPPORT ON THE PE
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THE ACIDIC CATALYSIS IN REACTION OF
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HYDROGEN-RICH GAS PURIFICATION FROM
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PP-II-82During the stage of combine
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PP-II-83higher H 2 /propane ratios
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NANOSTRUCTURED MATERIALS BASED ON Z
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ELECTROCATALYTIC REDUCTION OF NITRO
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PP-II-87with CuKα radiation (λ ~
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PP-II-88The properties of the catal
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PP-II-89The stereospecificity of po
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PP-II-91SYNTHESIS AND CHARACTERIZAT
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PP-II-92INFLUENCE OF NATURE OF HETE
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PP-II-93OPTICALLY ACTIVE AMMONIUM S
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PP-II-94THE INFLUENCE OF FORMING CO
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PP-II-95NEW CATALYST OF LOW-TEMPERA
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PP-II-96DRIFTS AND UV-VIS STUDY OF
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PP-II-97NANOSTRUCTURED COMPLEX OXID
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PLATINUM CATALYSTS AND THEIR ACTIVI
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PP-II-99DESIGN OF STRUCTURED CATALY
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PP-II-100THE INFLUENCE OF CARBON ON
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PP-II-100sp 2 -carbon samples (Sibu
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PP-II-101Undoped LaMnO 3 has a stru
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PP-II-102The redox mechanisms of ca
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PP-II-103weak surface complexes of
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PP-II-104Ellipsometric, LA-XRD, TEM
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357PP-II-105It follows that MAO (or
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PP-II-106For the description of met
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361PP-II-1070.75, 1) were prepared
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PP-II-108(K⋅10 6 l/mole⋅mg⋅eq
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PP-II-110EFFECTS OF THE PROPERTIES
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PP-II-111CATALYTIC ACTIVITY OF POLY
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SYNTHESIS OF OXIRANES FROM RENEWABL
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PP-II-113SELECTIVE OXIDATION OF FOR
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BIODIESEL PRODUCTION FROM OLEIC ACI
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PP-II-115THE MECHANISM OF PHENOL OX
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PP-II-116THERMOSTABILITY OF Pd-ZEOL
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PP-II-117CO OXIDATION ON CuO-CeO 2
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PP-II-118THE ROLE OF I-CONTAINING P
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PP-II-119THE BULK POROUS ELECTRODE
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PP-II-120Methanol was suggested to
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PP-II-121Synthesis of catalysts on
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Yield, %PP-II-122Dynamics of variat
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PP-II-123The analysis of the hydroc
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PP-II-125THE MECHANISM OF COPPER CO
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PP-II-126The problem of the low act
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PP-II-127size of hydrocatalytic pro
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PP-II-128enhanced stability against
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PP-II-130HYDROGEN PRODUCTION BY MET
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CATALYTIC HYDROALKOXYCARBONYLATION
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NANOSTRUCTURED METAL-POLYMERIC CATA
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PP-II-133THE EFFECT OF THE SUPPORT
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PP-II-134АLTERNATIVE APPROACH TO D
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PP-II-135THE LOW-TEMPERATURE CATALY
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CATALYTIC PROPERTIES OF LAYERED OF
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PP-II-138EFFECT OF Zr ON THE OXIDAT
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PP-II-139THE NATURE OF ACTION OF TH
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PP-II-140CYCLOHEXANE OXIDATION OVER
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PP-II-141Mo AND W HETEROPOLYACID-CO
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HYDROCARBON CONVERSION CATALYSTS BA
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PP-II-142selectivity of the hexene-
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PP-II-143XPS, XRD and UV-Vis DRS st
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PP-II-144from the surface of sample
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PP-II-146THE INFLUENCE OF THE ACIDI
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PP-II-147CHARACTERISATION OF NEW GO
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STUDY ON THE REGULARITIES OF THE FO
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PP-II-148Platinum catalysts support
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PP-II-149selectivity to LHC, moreov
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PP-II-150steamed until a gel format
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PP-II-151ELECTRONIC STATE OF Cr n+
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PP-II-152METAL SUPPORTED CATALYSTS
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PP-II-153FORECASTING CATALYTIC CHAR
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RE - CONTENTING HC OXIDATION CATALY
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PP-II-155reaction are shown on the
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PP-II-156The product of stereoselec
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PP-II-157Supporting Pd on ZnO coate
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PP-II-158relating to acetone. With
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PP-II-159At the same time, catalyst
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PP-II-160The aim of our work is to
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PP-II-161crystallization state of t
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PP-II-162several carbon materials a
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PP-II-1625. J. M. H. Dirkx, H. S. v
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PP-III-1INFLUENCE OF DISSOLVED OXYG
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PP-III-2and microstructure, oxidati
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PP-III-3Aerosol, vapour of toxiccom
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PP-III-4inserted in PAn either in t
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PP-III-5The mechanism of pyrolysis
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ELECTROCATALYSTS WITH LOW PLATINUM
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PP-III-8VERY PURE SILICA FIBROUS AS
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PP-III-9METAL CONTAINING ZEOLITES -
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THE INFLUENCE OF TREATMENT METHOD O
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PARA-HYDROGEN INDUCED POLARIZATION
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PP-III-12NOVEL CHITOSAN-BASED CATAL
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PP-III-13Fig. 1. Dark adsorption (1
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PP-III-14residual pressure of 0.67
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PP-III-15using the same feedstock.
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PP-III-16Fig. 2. SEM-images of surf
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EPOXIDATION OF RAPESEED OIL BY HYDR
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PP-III-19THE PECULIARITIES OF CATAL
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PP-III-20CATALYTIC MEMBRANE CONTACT
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PP-III-21CATALYTIC ACTIVE LAYERS ON
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PP-III-22MODIFICATION OF COMPOUNDED
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EFFECT OF LIQUID POLYKETONE ON THE
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CATALYSTS SEARCH FOR α-METYLBENZYL
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PP-III-25PARTIAL OXIDATION OF PROPA
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PP-III-27BIODIESEL SYNTHESIS BY CAT
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PP-III-28PRODUCTION OF BIO-SYNGAS V
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PP-III-28Fig. 1. Changes in Н 2 an
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PP-III-29Table 1: Texture and adsor
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PP-III-30dimensionless front veloci
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PP-III-31synthesized. Experiments h
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PP-III-32It is established, that cr
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PP-III-33adsorptive catalysts in ad
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PP-III-34turbocompressor and two ca
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PP-III-35The Cu, Ni/ γ -Al 2 O 3 c
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PP-III-36pressure at 800-900 o C. T
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PP-III-370,50Concentration / Vol.-%
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PP-III-38HETEROGENEOUS-CATALYTIC DE
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PP-III-39HYDROISOMERIZATION OF CATA
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METHOD OF CATALYTIC UTILIZATION OF
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PP-III-41Catalytic properties of Fe
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PP-III-42heat in a steam-power unit
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PP-III-43In this way, the content o
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PP-III-45THE ECOLOGIC AND ECONOMIC
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PP-III-46INFLUENCE OF SUPPORT NATUR
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PP-III-47MIGRATION OF SUPPORTED PLA
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Table 2.PP-III-47The [Pt]/[Al] atom
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PP-III-48Under nitrogen atmosphere
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PP-III-49With aim to achieve the ho
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PP-III-50clinoptilolite (Aydag depo
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PP-III-51References1. Balzhinimaev
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PP-III-52Black light UV lamps. The
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USE OF THE NITROGEN-CONTAINING CARB
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PP-III-54CATALYTIC BEHAVIOUR OF VAR
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PP-III-55and sulfur, was spent (fig
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PP-III-56Specific reaction rates of
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PP-III-57special catalyst system wi
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PP-III-59UTILIZATION OF WASTE BIOMA
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MECHANOCHEMISTRY AND MECHANO-CATALY
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PP-III-62CATALYTIC INTENSIFICATION
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PP-III-64ABOUT WHAT MANUFACTURE OF
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PP-III-65OXDATIVE CONVERSION OF HYD
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PP-III-66COMPLEX QUALITY CONTROL SY
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PP-III-67INFLUENCE OF DIFFUSION, SI
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PP-III-68ONE STEP PROCESS FOR HYDRO
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FEATURES OF DRAG FACTOR FOR COMPLEX
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FIXED BED REACTORS WITH GRADIENT CA
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PP-III-70respective variational pro
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PP-III-71Operation at high volumetr
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PP-III-72It was performed the optim
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PP-III-73production stages of refin
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pik⎛N= fi ⎜∑j ∑⎝ j=1Nik,
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PP-III-75three MCP’s. In the seco
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PP-III-76during the reaction. The i
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PP-III-77enthalpy calculated for va
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PP-III-78calculating kinetics of pa
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PP-III-79ventilators 7 and 10, flam
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PP-III-801) C 6 H 5 CH 3 + 2 [YO]
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PP-III-81Δm/m coating, %204060V=0.
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PP-III-82• diameter of its genera
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PP-III-83ΔP,1mm H 2 O/m40023003420
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Concentration, vol.%PP-III-84The ef
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PP-III-85autocatalyst of thermoconv
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PP-III-86The influence of such para
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PP-III-87hydrocarbons increases wit
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AUTOWAVE PROCESSES IN A STATIC CATA
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PP-III-90KINETIC AND THERMODYNAMIC
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PP-III-91which mathematical descrip
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PP-III-93UTILIZATION OF LARGE-SCALE
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CATALYTIC TECHNOLOGY OF UTILIZATION
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PP-III-95PROPERTIES AND ACTIVITY OF
Page 651 and 652:
PREPARATION AND CHARACTERIZATION OF
Page 653 and 654:
PP-III-98The comparison of TPR runs
Page 655:
ADVERTISEMENT
Page 658 and 659:
PerformancePassionSuccessAutomotive
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Обслуживаемые рынк
Page 662:
Polyurethanes are an integral part
Page 666 and 667:
− prehydrotreating of gasolines a
Page 668 and 669:
Kovalyov E. 123Kovtunov K. 489Kozlo
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List ofparticipantsABRAMOVA Anna Vs
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BOEVA Olga AnatolievnaD.I. Mendelee
Page 674 and 675:
DJEKIC TanjaEindhoven University of
Page 676 and 677:
GIMUNDINOV Shamil AbzalovichD.V. So
Page 678 and 679:
KACHEVSKY Stanislav AndreevichLomon
Page 680 and 681:
KONEV Vasily NikolayevichBoreskov I
Page 682 and 683:
LEDOUX Marc-JacquesCNRS DPI3 Rue Mi
Page 684 and 685:
MIERCZYŃSKI PawełInstitute of Gen
Page 686 and 687:
OBYSKALOVA Elina AnatolievnaBoresko
Page 688 and 689:
REBROV EvgenyEindhoven University o
Page 690 and 691:
SHALAGINA Anastasia EvgenievnaBores
Page 692 and 693:
SPIRIDONOV Alexey AlexeevichBoresko
Page 694 and 695:
VEDYAGIN Alexei Anatol'evichBoresko
Page 696 and 697:
ZAKHARENKO Valery SemenovitchBoresk
Page 698 and 699:
Volume IVolume IICONTENTPOSTER PRES
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PP-I-25 Hocine S., Cherifi O., Bett
Page 702 and 703:
PP-I-52 Timoshenkov S.P., Artemov E
Page 704 and 705:
PP-I-80 Shinkarev V.V., Kuvshinov G
Page 706 and 707:
PP-II-21 Chistoforova N.V., Yelkina
Page 708 and 709:
PP-II-45 Khachani M., Boucetta C.,
Page 710 and 711:
PP-II-68 Malinskaya M.Ju., Sviridov
Page 712 and 713:
PP-II-90 Nikitin V., Mikenas T., Za
Page 714 and 715:
PP-II-114 Sepúlveda J., Santarosa
Page 716 and 717:
PP-II-139 Tkach V.S., Suslov D.S.,
Page 718 and 719:
Section III. Environmental and indu
Page 720 and 721:
PP-III-28 Yakovlev V.A., Kirillov V
Page 722 and 723:
PP-III-52 Shelimov B., Tolkachev N.
Page 724 and 725:
PP-III-77 Mel’gunov M., Kovalev M
Page 726:
III International Conference“Cata
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