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90 CHAPTER 2. ATMOSPHERE AND REMOTE SENSING<br />
2.5.19 Comparison of GOME NO2 retrievals analysed by different scientific<br />
groups<br />
Participating scientists: Walburga Wilms-Grabe, Steffen Beirle, Randall Martin, Andreas Richter,<br />
Michel van Roozendael, and Thomas Wagner<br />
Abstract In order to improve nonuniform GOME NO2 products of differing analysis tools applied<br />
at several institutes, NO2 SCDs have been compared for selected GOME orbits. The results show<br />
principal agreement between retrievals of IASB in Brussels, IUP Bremen and IUP Heidelberg, but in<br />
some extent clear discrepancies to retrievals of Dalhousie University in Halifax.<br />
Figure 2.53: NO2 SCDs of one GOME orbit crossing north-east of the United States and the Pacific,<br />
analysed for 03 February 1996 (left) and 06 February 2000 (right) by Heidelberg (blue), Bremen<br />
(black), Brussels (green) and Halifax (red)<br />
Background Several scientific groups are occupied<br />
with the analysis of GOME trace gas measurements.<br />
In dependence of the used retrieval<br />
tools, the resulting trace gas distributions differ<br />
from each other, though they were analyzed for<br />
the same location and time. Therefore, a comparison<br />
study is performed in order to assess the<br />
discrepancies and to evaluate the reliability of<br />
GOME products. The study is concentrated on<br />
NO2, an important trace gas for both the troposphere<br />
and stratosphere. The assessment of NO2<br />
retrievals can help all GOME data users to choose<br />
the most appropriate data set and particularly<br />
helps the provider of evaluated GOME data to<br />
unify the different existing analyzing algorithms.<br />
Funding See satellite group overview.<br />
Methods and results For the whole GOME<br />
measurement period, two GOME orbits per year<br />
have been selected as case studies: one orbit in<br />
the winter time (February) and one in the summer<br />
time (July). The chosen orbits are all located<br />
above nearly the same region, including high polluted<br />
areas in north-east of the United States and<br />
clean areas above the Pacific. This choice allows<br />
to compare NO2 retrievals for the complete orbit,<br />
but also to consider separately polluted and<br />
non-polluted parts of the orbit. In order to obtain<br />
really basic information about reasons for the<br />
variability of GOME NO2 products, in a first step<br />
pure SCDs were compared.<br />
The figure shows two examples of several NO2 retrievals.<br />
The principal agreement of all participating<br />
groups is existing. However, all selected<br />
orbits indicate better agreement between the NO2<br />
distributions of Bremen, Brussels and Heidelberg<br />
and more obvious deviations in the NO2 results<br />
of Halifax. The deviations of Halifax are related<br />
as well to the absolute SCD values (positive offset)<br />
as to the scattering of the data. In the figure,<br />
the differing scatter patterns of Halifax can<br />
be seen clearly in the region between −50 ◦ and<br />
−10 ◦ latitude. Correlations between NO2 results<br />
of Bremen, Brussels and Heidelberg lie around<br />
0.97 and 0.99 in both polluted and unpolluted regions.<br />
Correlations between data of one of these<br />
groups and data of Halifax are around 0.97 in<br />
polluted areas and about 0.55 in the less NO2enriched<br />
region between −50 ◦ and −10 ◦ latitude.<br />
Outlook/Future work Level 2 data of the<br />
DLR have to be included in the comparison study.<br />
Also VCDs and air mass factors have to be considered,<br />
the number of selected orbits has to be<br />
extended.<br />
Main publication Publication is planned later<br />
on in an advanced stage of the comparison study.