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Program - Brookhaven National Laboratory

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Shintaro Hashimoto, Osamu Iwamoto, Yosuke Iwamoto, Tatsuhiko Sato<br />

Japan Atomic Energy Agency, Ibaraki-ken, 319-1195, Japan<br />

Koji Niita<br />

Research Organization for Information Science and Technology, Ibaraki-ken, 319-1196, Japan<br />

Monte Carlo simulation codes such as PHITS, MCNP, FLUKA and MARS play an important role in<br />

prediction of radiation damage to materials and human bodies under irradiation. As these codes can<br />

describe the transport of many particles, e.g. photons, electrons, nucleons, and heavy ions, using various<br />

physical processes, we can obtain deposit energies and particle fluxes in materials for many purposes. In<br />

particular, nuclear reaction processes are essential parts for the production of secondary particles in a high<br />

energy region. Recently, there are plans to utilize accelerator-based neutron sources using the reaction<br />

between proton or deuteron beams and Li, Be or C target for Boron Neutron Capture Therapy (BNCT)<br />

or the material test under irradiation at the International Fusion Materials Irradiation Facility (IFMIF)<br />

project. For neutron source design, evaluation of neutron yields created by nuclear reactions at incident<br />

energies from 10 to 100 MeV is indispensable. However, as nuclear reaction models of the Intra-Nuclear<br />

Cascade type used in most of the simulation codes cannot describe quantum mechanical effects, discrete<br />

neutron peaks in the neutron energy spectrum are neglected. Although the use of the evaluated nuclear<br />

data can give detailed and complex spectra, the energy of the incident particle has been generally limited,<br />

e.g. less than 20 MeV. In this study, we obtain cross sections of the discrete states using the Distorted Wave<br />

Born Approximation (DWBA) method, which is a theoretical model based on quantum mechanics, and<br />

combine the cascade type calculation with the event generator using the DWBA results. This combined<br />

model gives not only a broad peak but also discrete peaks of the neutron spectrum for deuteron induced<br />

reactions on Li, Be, and C targets. We will show results for proton induced reactions on the targets, and<br />

discuss effects of neutron spectra by different nuclear reaction models on the dose estimation.<br />

HC 2 4:00 PM<br />

Calculations of Compound Nucleus Spin-Parity Distributions Populated via the (P,T)<br />

Reaction in Support of Surrogate Reaction Measurements<br />

James Benstead<br />

AWE, UK<br />

Prof Jeff Tostevin<br />

University of Surrey, UK<br />

The surrogate reaction method may be used to determine the cross section for neutron induced reactions<br />

not accessible through standard experimental techniques. This is achieved by creating the same compound<br />

nucleus as would be expected in the desired reaction, but through a different incident channel, generally<br />

a direct transfer reaction. So far, the surrogate technique has been applied with reasonable success to<br />

determine the fission cross section for a number of actinides [1], but has been less successful when applied<br />

to other reactions, e.g. (n,γ), due to a ”spin-parity mismatch” [2]. This mismatch, between the distributions<br />

of the excited levels of the compound nucleus populated in the desired and surrogate channels, leads to<br />

differing decay probabilities and hence reduces the validity of using the surrogate method to infer the cross<br />

section in the desired channel. A greater theoretical understanding of the expected distribution of levels<br />

excited in both the desired and surrogate channels is therefore required in order to attempt to address this<br />

mismatch and allow the method to be utilised with greater confidence. Two neutron transfer reactions,<br />

e.g. (p,t), which allow the technique to be utilised for isotopes further removed from the line of stability,<br />

are the subject of this study. Preliminary results will be presented for calculations of the distribution of<br />

compound nucleus states populated, via the (p,t) reaction, at excitation energies consistent with those<br />

115

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