26.02.2013 Views

Program - Brookhaven National Laboratory

Program - Brookhaven National Laboratory

Program - Brookhaven National Laboratory

SHOW MORE
SHOW LESS

You also want an ePaper? Increase the reach of your titles

YUMPU automatically turns print PDFs into web optimized ePapers that Google loves.

section of 241 Am was deduced for a neutron energy region between 0.01 and 20 eV. The obtained cross<br />

section and the Westcott factor are compared with the preceding experiments and evaluated values. This<br />

work was supported by JSPS KAKENHI Grant Number 22226016.<br />

NA 2 11:00 AM<br />

Neutron-Induced Cross Sections Measurements Of Calcium<br />

K. H. Guber, Oak Ridge <strong>National</strong> <strong>Laboratory</strong>, P.O. Box 2008, Oak Ridge, TN 37831, USA. S. Kopecky,<br />

Nuclear Physics Unit, EC-JRC-IRMM, Retieseweg 111, 2440 Geel, Belgium. P. Schillebeeckx, Nuclear<br />

Physics Unit, EC-JRC-IRMM, Retieseweg 111, 2440 Geel, Belgium. K. Kauwenberghs, Nuclear Physics<br />

Unit, EC-JRC-IRMM, Retieseweg 111, 2440 Geel, Belgium. P. Siegler, Nuclear Physics Unit,<br />

EC-JRC-IRMM, Retieseweg 111, 2440 Geel, Belgium.<br />

Among its many applications, calcium is a constituent of concrete and is very frequently found in combination<br />

with uranium and/or mixed with radioactive waste. The US Department of Energy Nuclear Criticality<br />

Safety <strong>Program</strong> (NCSP) has identified calcium as a nuclide needing improvement for supporting criticality<br />

safety analyses. In particular, a consistent set of covariance data is needed in the evaluation to support<br />

sensitivity/uncertainty analyses. As a result, the NCSP initiated new neutron-induced cross section<br />

measurements on calcium to support the development of a new cross-section evaluation in the resonance<br />

region.. The objective of this paper is to present the results of the calcium cross-section measurements<br />

and data analysis. Two types of experiments were performed at the Geel Electron Linear Accelerator<br />

(GELINA) of the Institute for Reference Material and Measurements of the Joint Research Centers, European<br />

Union. A metallic calcium target was placed in Flight Path 14 at a distance of 60 m from the<br />

neutron production target to measure neutron capture with 4 C6D6 detectors. Due to its reactivity with<br />

air, the metallic calcium sample was encapsulated in a thin-wall aluminum container. To correct for the<br />

effect of the aluminum, an empty container of the exact same dimensions was also measured. The same<br />

sample was used in a transmission experiment to determine the total cross section. The sample was placed<br />

in Flight Path 4 at a distance of 50 m from the neutron target. A 1.27-cm thick 6Li glass detector was<br />

used to detect the sample-transmitted neutron. The empty aluminum container served in the open beam<br />

as a compensator for the aluminum in the sample. The final paper will provide the experimental details<br />

and compare the measured cross-section data for calcium with cross sections calculated from the latest<br />

evaluated data files. ORNL is managed by UT-Battelle, LLC, for the U.S. Department of Energy under<br />

Contract No. DE-AC05-00OR22725. The U.S. Department of Energy Nuclear Criticality Safety <strong>Program</strong><br />

sponsored the work that is presented in this paper<br />

NA 3 11:20 AM<br />

Measurements of keV-Neutron Capture Cross Sections and Capture Gamma-Ray Spectra<br />

of Pd Isotopes<br />

K. Terada, M. Igashira, T. Katabuchi, T. Matsuhashi, B. Hales<br />

Tokyo Institute of Technology<br />

The nuclear transmutation of long-lived fission products (LLFPs) generated in nuclear fission reactors into<br />

stable or short-lived nuclides by neutron capture reaction is expected to reduce the impact of nuclear waste<br />

disposal on the environment. Palladium-107 (half life: 6.5x10 6 y) is one of the most important LLFPs, and<br />

its neutron capture cross sections are important for the study of LLFP transmutation systems. On the<br />

other hands, the capture cross sections of stable Pd isotopes also affect the performance of a transmutation<br />

191

Hooray! Your file is uploaded and ready to be published.

Saved successfully!

Ooh no, something went wrong!