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Program - Brookhaven National Laboratory

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Methods have been developed to extrapolate measured first-chance fission-product yields and average fragment<br />

total kinetic energies to higher incident-neutron energies where second, third, and forth chance fission<br />

are of importance. The yields for fragment mass near the asymmetric peaks at A 100 and A 138 decrease<br />

with increasing incident-neutron energy, while the yields for symmetry fragments, and fragments with<br />

masses less than A 96 and more than A 146 increase with increasing incident-neutron energy. Predictions<br />

are made for the energy dependence of plutonium fission-product yields. These are compared to the limited<br />

available data. A prediction is made for the average total kinetic energy of 239 Pu(n,f) fission fragments,<br />

up to a neutron energy of 20 MeV. These predictions will be tested in the next few years by the SPIDER<br />

collaboration at Los Alamos.<br />

Session DA Neutron Cross Section Measurements<br />

Monday March 4, 2013<br />

Room: Met East at 3:30 PM<br />

DA 1 3:30 PM<br />

The Fission Time Projection Chamber Project<br />

Tony Hill, the NIFFTE Collaboration<br />

INL<br />

New high-precision fission experiments have become a priority within the low-energy nuclear community.<br />

Modern sensitivity calculations have revealed unacceptable liabilities in some of the underlying fundamental<br />

nuclear data and have provided target accuracies for new measurements that are well beyond what can<br />

be delivered using current experimental technologies. A potential breakthrough in the precision barrier<br />

for these measurements is the deployment of a Time Projection Chamber (TPC). TPC detector systems<br />

were originally developed within the particle physics community and have played a central role in that<br />

field for nearly 25 years. A group of 6 universities and 4 national laboratories have undertaken the task of<br />

building the first TPC designed specifically for the purpose of measuring fission cross sections. In this talk,<br />

I will present the motivation for the fission TPC concept, a few details of the device and why we think an<br />

improvement on 50 years of fission experiments can be accomplished.<br />

DA 2 4:00 PM<br />

Measuring the α/SF Branching Ratio of 252 Cf with the NIFFTE Time Projection Chamber<br />

Lucas Snyder, the NIFFTE Collaboration<br />

LLNL<br />

Fission reactions are particularly complicated quantum systems and current nuclear theory lacks the necessary<br />

predictive power to calculate many of the fundamental quantities associated with the process. The<br />

neutron induced fission cross section is one experimentally measured value of particular importance in the<br />

calculation and simulation of nuclear fuel cycles. The NIFFTE collaboration is developing a fission Time<br />

Projection Chamber intended to measure energy dependent neutron induced fission cross sections of the<br />

major and minor actinides to an uncertainty of better than 1%. The fission TPC will address many of the<br />

systematic uncertainties associated with past and current detector systems used to measure the neutron<br />

induced fission cross section by providing detailed 3-dimensional images of ionizing particles such as fission<br />

fragments and alpha particles. To establish the particle tracking and identification abilities of the fission<br />

TPC in the development phase, the α-decay and spontaneous fission of 252 Cf was observed with a partial<br />

TPC. Preliminary results of an analysis of the α/SF branching ratio of 252 Cf will be presented.<br />

53

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