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Program - Brookhaven National Laboratory

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Session JF Neutron Cross Section Measurements<br />

Wednesday March 6, 2013<br />

Room: Central Park East at 10:30 AM<br />

JF 1 10:30 AM<br />

Measurement of Neutron Induced Fission Cross Sections by Surrogate Methods<br />

V.V. Desai, B.K. Nayak, A. Saxena and S. Kailas<br />

Nuclear Physics Division, Bhabha Atomic Research Centre, Mumbai-400085, India<br />

The neutron induced compound nuclear fission cross section data are required for nuclear energy, national<br />

security and nuclear astrophysics applications [1]. Unfortunately, for a large number of reactions the<br />

relevant data cannot be directly measured in the laboratory, since the desired nuclei are often too difficult<br />

to produce with currently available experimental techniques or too short-lived to serve as target in present<br />

day setups. The Surrogate method provides an access to such nuclear data indirectly. In recent years,<br />

the surrogate reaction methods in various forms such as: (i) direct surrogate method, (ii) surrogate ratio<br />

method and (iii) hybrid surrogate ratio method, have been employed to get indirect estimate of the neutron<br />

induced fission reaction cross sections of many compound nuclear systems in actinide region, which are<br />

not accessible for direct measurements. In an earlier work, the 233Pa(n,f) cross sections in the equivalent<br />

neutron energy range 11.0 MeV to 16.0 MeV have been determined employing the Hybrid Surrogate Ratio<br />

Method (HSRM)[2]. In a recent work, we have determined the 234Pa(n,f), 239Np(n,f), and 240Np(n,f) cross<br />

sections by HSRM in the equivalent neutron energy range 9.0 MeV to 16.0 MeV, by measuring ratios of<br />

fission decay probabilities of the compound nuclear residues produced in [ 232Th( 7Li, α) 235Pa/ 232Th( 7Li, t) 236U], [ 238U( 6Li, α) 240Np / 238U( 6Li, d) 242Pu], and [ 238U( 7Li, α) 241Np / 238U( 7Li, t) 242Pu] transfer<br />

reactions respectively. We have also determined 241Pu(n,f) cross sections using 238U ( 6Li, d) 242Pu and<br />

232Th ( 6Li, d) 236U transfer reactions by employing surrogate ratio method. Details of experiments and<br />

results for various reactions will be presented.<br />

Corresponding author: B.K. Nayak<br />

[1] J.E. Escher et al. Rev. of Mod. Phys. 84, 354 (2012). [2] B.K. Nayak et al. Phys. Rev. C78, 061602<br />

(R) (2008).<br />

JF 2 11:00 AM<br />

Neutron-induced Capture Cross Sections of Actinides via the Surrogate-Reaction Method<br />

Q. Ducasse, B. Jurado, M. Aiche, L. Mathieu, I. Companis, S. Czajkowski, J. Matarranz, I.<br />

Tsekhanovich, CENBG, Chemin du Solarium B. P. 120, 33175 Gradignan, France. T.Tornyi, F.<br />

Giacoppo, A. Goergen, M. Guttormsen, A. C. Larsen, T. Renstrom, S. Rose, S. Siem, G. M. Tveten, T.<br />

Wiborg-Hagen, University of Oslo, Department of Physics, 0316 Oslo, Norway. F. Gunsing,<br />

CEA/Saclay, 91191Gif-sur-Yvette, France. M. Lebois, J. N. Wilson, IPN, 91406 Orsay, France. M.<br />

Wiedeking, iThemba LABS, 7129 Somerset West, South Africa. O. Serot, CEA/Cadarache, 13108 Saint<br />

Paul lez Durance, France. G. Boutoux, V. Meot, O. Roig, CEA/DAM, 91297 Arpajon, France.<br />

Neutron-induced cross sections of short-lived nuclei are crucial for reactor physics. In particular, (n, γ) cross<br />

sections on minor actinides are one of the largest sources of uncertainty in modeling new reactors for nuclear<br />

waste transmutation using fast neutrons. However, very often the high radioactivity of the actinide samples<br />

makes the direct measurement of these cross sections extremely difficult. The surrogate-reaction method<br />

148

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