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Program - Brookhaven National Laboratory

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The European Spallation Source (ESS) is the European common effort in designing and building a next<br />

generation large-scale user facility for studies of the structure and dynamics of materials. The ESS target,<br />

moderators and reflectors system through interactions with 5 MW proton beam (2.5 GeV, 20 Hz) will<br />

produce long pulse (2.8 ms width) neutrons in subthermal and thermal energy range. These neutrons are<br />

further transported to a variety of neutron scattering instruments. The aim of this work is to assess the<br />

strategy to be used for safely handling and shipping of the high activated components of ESS target station.<br />

For safe maintenance, during operation as well as handling, transport and storage of the components of the<br />

ESS target station after their lifetime, detailed knowledge about the activation induced by the impinging<br />

protons and secondary radiation fields is required. The Monte Carlo transport code MCNPX2.6.0 was<br />

coupled with CINDER90 version 07.4 to calculate the residual nuclide production in the main items of the<br />

system: target wheel and the shaft, moderator-reflector plug, beam window plug, shutters. Dose equivalent<br />

rates due to the residual radiation were further calculated with the MICROSHIELD and MCNPX<br />

codes using photon sources resulting from CINDER. Various decay times after ceasing operation of each<br />

component were considered. The activation and decay heat density distributions of all these components<br />

together with the derived dose rates were analyzed to assess the best strategy to be used for their safely<br />

remove and transport to a hotcell, eventual dismantling, storage on-site and shipping off-site as intermediate<br />

level waste packages. The derived photon sources were used afterwards to design the shielded exchange<br />

flasks that are needed to remove and transport each component after its lifespan to a hotcell. Design of<br />

a multi-purpose cask able to accommodate the different highly activated components and shipping them<br />

to external conditioning facility was further developed. For this purpose, the photon source term of each<br />

of the analyzed item was derived taken into consideration previously estimated decay time on-site prior<br />

the cask loading. The main criterion used for optimization of the thickness and material selection of the<br />

shielding of the flasks, in agreement with Swedish legislation and ADR provisions, is that the dose rate<br />

must not exceed 2 mSv h −1 on the outer surface and 0.1 mSv h −1 at a distance of 1 m. The calculated<br />

parameters for the shield of the components with high dose rates will be used for detailed design and<br />

manufacturing of the exchange flasks. Obtained results for the off-site shipping cask are discussed in order<br />

to derive the requirements to be fulfilled for the type B(U) package design approval.<br />

KE 3 2:20 PM<br />

Distribution of Radionuclides in MEGAPIE, a Proton Irradiated LBE Target<br />

Bernadette Hammer, Dorothea Schumann, Jörg Neuhausen, Viktor Boutellier, Hans-Peter Linder,<br />

Natalia Shcherbina, Michael Wohlmuther, Andreas Türler<br />

Paul Scherrer Institute<br />

Christof Vockenhuber<br />

ETH Zurich<br />

At the moment, several technologies are developed to reduce the amount and the radiotoxicity of residual<br />

waste from nuclear power plants. Promising techniques that could be employed for this purpose are fast<br />

reactors or Accelerator Driven Systems (ADS) that use liquid heavy metal as reactor coolants and/or<br />

material for generating fast neutrons in spallation targets. In some of these innovative reactor designs,<br />

lead or lead-bismuth eutectic (LBE) is used as the liquid metal. In an ADS, additional radioactivity<br />

is formed in the spallation unit by interactions of high energy and secondary particles with the target<br />

material. Data on this residue nuclide production are essential for benchmark theoretical predictions as<br />

well as analyzing safety hazards of future LBE cooled nuclear facilities during and after operation, including<br />

the options of intermediate or final disposal [1]. A prototype of a lead-bismuth spallation target, MEGAPIE<br />

(MEGAwatt PIlot Experiment) [2], was operated close to the megawatt regime (0.8 MW) in the spallation<br />

159

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