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Chapter I Brief Introduction...<br />

the crystal. These methods are called temperature tuning method and quasi –<br />

phase matching. In temperature tuning, the pump (laser) frequency<br />

polarization is selected orthogonal to the signal and idler frequency<br />

polarization. The birefringence in some crystals, for example, Lithium niobate<br />

is highly temperature dependent. The crystal is controlled at a certain<br />

temperature to achieve phase matching conditions. In quasi – phase matching<br />

the frequencies involved are not constantly locked in phase with each other,<br />

instead the crystal axis is altered at a regular interval. Hence, these crystals<br />

are called periodically poled. This results in the polarization response of the<br />

crystal to be shifted back in phase with the pump beam by reversing the<br />

Nonlinear susceptibility. This allows net positive energy flow from pump into<br />

the signal idler frequencies. In this case, the crystal itself provides the<br />

additional wave vector K = 2/ to satisfy the phase matching condition. The<br />

quasi – phase matching can be expanded to chipped pulse as it is done in a<br />

dazzler.<br />

Group Velocity Mismatching<br />

For NLO processes of ultrafast lasers such as Ti:Sapphire and Dye<br />

lasers with femto second (fs) pulse width, the main limitation to conversion<br />

efficiency is group velocity mismatching(GVM). The GVM is caused by group<br />

velocity dispersion of NLO crystal.<br />

Damage Threshold<br />

Damage threshold is a property of the crystal to withstand the laser<br />

radiation without damage. The damage threshold is a function of the<br />

wavelength of fundamental and harmonic radiation, pulse duration, beam<br />

16

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