Landfills and waste water treatment plants as sources of ... - GKSS

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SUPPORTING INFORMATION Table S16: Table of recovery rates (%) obtained in particle phase samples from waste water treatment plants WA and WB and the reference sites. 128 18 O2 PFHxS 13 CPFOS 13 C PFBA 13 C PFHxA 13 C PFOA 13 C PFNA 13 C PFDA 13 C PFUDA WA1 - - - - - - - - - 93 90 83 110 113 162 55 104 WA2 42 59 54 32 55 37 58 87 67 88 83 87 110 117 132 93 94 WA3 38 60 39 19 39 35 58 70 54 80 85 76 96 93 129 69 102 WA4 32 88 35 16 45 53 53 47 35 91 87 84 135 122 130 88 119 WA5 44 80 46 28 51 63 73 88 73 85 88 84 113 114 141 106 - WB1 65 63 85 46 77 41 52 63 59 40 44 56 92 116 69 55 76 WB2 - - - - - - - - - 36 36 42 57 56 60 95 40 WB3 47 66 53 18 55 38 45 51 48 54 61 65 110 122 67 99 101 WB4 118 72 44 83 96 70 65 83 79 46 44 49 75 76 47 83 85 WB5 55 87 48 19 58 42 47 64 54 51 57 61 103 99 87 70 81 RF1 48 77 55 40 54 61 76 84 74 60 65 59 70 68 103 - 48 RF2 43 79 35 27 49 57 69 76 68 80 76 80 89 89 150 - 70 RF3 35 56 28 17 36 41 50 59 51 78 76 77 84 84 144 - 66 RF4 31 87 35 17 39 48 52 49 43 70 72 77 79 83 131 - 48 RF5 43 91 35 21 38 55 60 63 53 65 66 61 61 64 113 - 61 RF11 92 85 118 61 111 93 68 27 2 53 49 48 76 75 48 101 97 RF12 48 83 30 18 43 43 55 66 54 52 59 64 73 75 76 78 82 RF13 52 60 48 18 52 44 51 59 55 62 59 63 73 84 82 93 103 RF14 44 62 42 19 49 39 46 58 53 56 52 59 70 73 80 83 89 RF15 91 103 77 82 81 87 91 103 95 65 60 67 75 72 103 49 74 13 C PFDoA MBDE 28 MBDE 47 MBDE 99 MBDE 153 MBDE 183 MBDE 209 AHTN D3 MX D15
SUPPORTING INFORMATION Table S17: PFC concentrations (pg m -3 ) in gas-phase samples from WWTP WA and WB and the corresponding RFs. n.d.: not detected, a values are corrected by mean recovery rates of 13 C 6:2 FTOH as described in section 5.3.7. 4:2 FTOH 6:2 FTOH 8:2 FTOH 10:2 FTOH 12:2 FTOH 6:2 FTA 8:2 FTA WB1 n.d. 112 a 216 51 34 n.d. 20 28 n.d. 55 27 16 n.d. 7 n.d. 3 WB2 n.d. 12 a 124 35 14 n.d. 3 4 n.q. 51 23 6 n.d. 4 5 9 WB3 n.d. 120 a 143 31 17 n.d. 7 8 n.d. 31 34 8 n.d. 2 n.d. n.d. WB4 n.d. 225 a 419 66 29 n.d. 35 33 n.d. 69 61 10 n.d. 4 7 3 WB5 n.d. 259 a 350 77 30 n.d. 49 56 n.d. 61 60 54 n.d. 2 5 n.d. WA1 n.d. 16 59 27 55 11 4 21 n.d. 4 n.d. 9 n.d. 1 n.d. 2 WA2 7 29 85 22 33 8 4 15 n.d. 11 n.d. 10 n.d. 2 n.d. 3 WA3 n.d. 15 41 11 6 10 3 2 n.d. 3 n.d. 4 n.d. 1 3 n.d. WA4 n.d. 0 36 19 6 n.d. n.d. 2 n.d. 18 n.d. 5 n.d. 2 5 3 WA5 n.d. 25 91 22 12 11 3 3 n.d. 3 n.d. n.d. 6 7 2 RF1 n.d. 13 34 14 8 n.d. 3 3 n.d. 3 n.d. 6 n.d. 1 5 n.d. RF2 n.d. 9 130 19 8 4 4 3 n.d. 3 n.d. 4 n.d. 1 5 1 RF3 n.d. 7 62 11 6 5 1 2 n.d. 3 n.d. 4 n.d. 1 3 n.d. RF4 n.d. 8 31 12 3 9 1 1 n.d. 2 n.d. n.d. 3 3 1 RF5 n.d. 8 26 9 5 n.d. n.d. n.d. n.d. 9 n.d. 10 n.d. 1 5 3 RF12 n.d. 34 a 75 48 20 n.d. 3 2 n.d. 1 3 3 n.d. 2 3 n.d. RF13 n.d. 4 a 45 14 7 7 4 2 n.d. 2 3 4 n.d. n.d. n.d. n.d. RF14 n.d. 45 176 58 24 13 6 3 n.d. 3 4 9 n.d. 4 n.d. 2 RF15 n.d. 4 a 7 3 2 n.d. 3 n.d. n.d. 1 n.d. n.d. n.d. 2 n.d. n.d. Table S18: PFC concentrations (pg m -3 ) in particle-phase samples from WWTP WA and WB and the corresponding RFs. n.d.: not detected, n.q.: not quantified PFBS PFHxS PFOS PFBA PFPA PFHxA WA2 n.d. n.d. 0.2 8.4 0.0 0.5 0.1 1.3 n.d. 0.2 0.1 0.2 1.9 WA3 n.d. n.d. 0.5 6.5 0.1 0.2 n.d. 1.1 0.1 0.1 0.1 0.1 1.5 WA4 n.d. n.d. 0.4 1.4 n.d. n.d. n.d. n.d. 0.1 n.d. n.d. 0.1 0.6 WA5 0.2 0.7 0.9 6.5 0.2 0.4 0.1 0.5 0.3 0.0 0.1 0.1 0.9 WB1 n.d. n.d. 0.0 0.5 n.d. 0.0 n.d. n.d. 0.2 0.3 n.d. n.d. 0.6 WB3 0.1 n.d. 0.2 2.8 n.d. n.d. n.d. 0.6 0.3 0.2 n.d. n.d. 0.9 WB4 n.d. n.d. n.d. n.d. n.d. n.d. n.d. n.d. n.d. n.d. n.d. n.d. n.d. WB5 0.2 n.d. 0.5 0.0 n.d. n.d. n.d. 1.1 0.5 0.6 n.d. n.d. 0.9 RF2 n.d. 0.0 0.1 2.6 0.4 0.3 0.1 0.3 0.3 0.1 0.1 0.2 0.2 RF3 0.1 0.2 0.6 5.6 0.4 0.3 0.1 0.2 0.0 0.1 0.1 0.1 0.3 RF4 n.d. n.d. 0.1 n.d. n.d. n.d. n.d. n.d. 0.0 n.d. n.d. n.d. 0.0 RF5 0.9 2.0 1.8 5.4 1.8 1.6 1.0 3.4 0.9 2.1 0.8 1.1 1.7 RF11 1.9 n.d. 2.9 15.7 4.7 3.3 2.8 7.1 1.9 1.7 n.d. n.d. n.d. RF13 0.2 n.d. 0.6 7.2 n.d. 0.5 0.1 0.4 n.d. n.d. n.d. n.d. n.d. RF14 n.d. n.d. 1.0 6.6 1.2 0.6 n.d. 0.5 n.d. n.d. n.d. n.d. n.d. RF15 n.q. n.d. n.d. 1.7 n.d. n.q. n.d. n.q. n.d. n.d. n.d. n.d. n.d. 10:2 FTA PFHpA Me2FOSA PFOA EtFOSA PFNA MeFBSA MeFOSA PFDA PFOSA PFUnDA MeFOSE PFDoDA MeFBSE EtFOSE PFOSA 129
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ISSN 0344-9629 Landfills and waste
Page 4 and 5:
Die Berichte der GKSS werden kosten
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Deponien und Kläranlagen als Quell
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TABLE OF CONTENTS VI 4.2.5 Extracti
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LIST OF FIGURES Figure 20: Proporti
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LIST OF TABLES Table S6: Table of r
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ABBREVIATIONS BDE47 2,2',4,4'-Tetra
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ABBREVIATIONS MW molecular weight M
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2 INTRODUCTION
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INTRODUCTION 175 chemicals classifi
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INTRODUCTION Table 1 cont. Analytes
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INTRODUCTION Table 3: Polycyclic mu
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INTRODUCTION Mabury 2006). This inc
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INTRODUCTION 1.3 Physico-chemical p
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INTRODUCTION 1.4 Environmental conc
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INTRODUCTION Chen et al. 2007a; Har
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INTRODUCTION prevent xenobiotica fr
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INTRODUCTION al. 2009c) and being d
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INTRODUCTION Table 6: Selection of
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INTRODUCTION 1.5 Sources Sources of
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OBJECTIVES 2. Objectives In recent
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METHOD OPTIMISATION Simonich et al.
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METHOD OPTIMISATION used as carrier
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METHOD OPTIMISATION 3.3 Extraction
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METHOD OPTIMISATION 3.3 Results 3.3
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METHOD OPTIMISATION AHMI). For less
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METHOD OPTIMISATION 3.3.5 Extractio
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METHOD OPTIMISATION 3.4 Discussion
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METHOD OPTIMISATION partly due to h
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METHOD OPTIMISATION Figure 7: Final
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STUDY 1: LANDFILLS AS SOURCES volat
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STUDY 1: LANDFILLS AS SOURCES On ea
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STUDY 1: LANDFILLS AS SOURCES (Supe
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STUDY 1: LANDFILLS AS SOURCES Table
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STUDY 1: LANDFILLS AS SOURCES 52 c
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STUDY 1: LANDFILLS AS SOURCES 4.3.2
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STUDY 1: LANDFILLS AS SOURCES 4.5 D
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STUDY 1: LANDFILLS AS SOURCES conce
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STUDY 1: LANDFILLS AS SOURCES influ
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STUDY 2: WASTE WATER TREATMENT PLAN
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Page 96 and 97: STUDY 2: WASTE WATER TREATMENT PLAN
Page 106 and 107: CONCLUSIONS AND OUTLOOK BDE183 were
Page 108 and 109: REFERENCES wastewater treatment/pol
Page 110 and 111: REFERENCES Capuano, F. Cavalchi, B.
Page 112 and 113: REFERENCES Dreyer, A. Temme, C. Stu
Page 114 and 115: REFERENCES Harada, K. Nakanishi, S.
Page 116 and 117: REFERENCES Kallenborn, R. Gatermann
Page 118 and 119: REFERENCES sexual development, and
Page 120 and 121: REFERENCES Oros, D. R. Hoover, D. R
Page 122 and 123: REFERENCES Rimkus, G. (1995): Nitro
Page 124 and 125: REFERENCES Smithwick, M. Mabury, S.
Page 126 and 127: REFERENCES USEPA (2006): 2010/2015
Page 128 and 129: REFERENCES Zhao, Y.-X. Qin, X.-F. L
Page 130 and 131: SUPPORTING INFORMATION Figure S3: H
Page 132 and 133: SUPPORTING INFORMATION Table S1: Ta
Page 134 and 135: SUPPORTING INFORMATION Table S2: Ma
Page 136 and 137: SUPPORTING INFORMATION Table S5: Ta
Page 138 and 139: SUPPORTING INFORMATION Table S7: Bl
Page 140 and 141: SUPPORTING INFORMATION Table S11: P
Page 142 and 143: SUPPORTING INFORMATION Figure S7: S
Page 144 and 145: SUPPORTING INFORMATION Figure S7 co
Page 148 and 149: SUPPORTING INFORMATION Table S19: M
Page 154: ERKLÄRUNG DER SELBSTSTÄNDIGEN VER
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