Plutonium Biokinetics in Human Body A. Luciani - Kit-Bibliothek - FZK

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JOURNALS OWN PUBLICATIONS RELATED TO THE SUBJECT � Luciani, A., Polig, E., Doerfel, H. An age-related model derived from ICRP 67 model for Plutonium dose assessments: application to an updated case of contamination, Oral Presentation at the 8th International Conference on Low level measurements of actinides and long-lived radionuclides in biological and environmental samples, Oarai, Japan, 16-20 October 2000, Proceedings of the Conference, Journal of Radioanalytical and Nuclear Chemistry 252(2):301-307, 2002. � Luciani, A. Plutonium dose assessments based on a new model derived from ICRP 67, Health Phys. 80(6):618-619, 2001 � Luciani, A., Doerfel, H., Polig, E. Sensitivity analysis of the urinary excretion of Plutonium, Rad. Prot. Dosim. 93(2):179-183, 2001. � Luciani, A., Polig, E. Verification and modification of the ICRP-67 model for plutonium dose calculation, Health Phys. 78(3):303-310, 2000. TECHNICAL AND ANNUAL REPORTS � Luciani, A. and Castellani, C.M. Biocinetica del Plutonio nell’organismo umano: analisi e modifica del modello ICRP 67. Rapporto Tecnico ENEA, RT/AMB/PRO/2001/5, ENEA, Roma, 2001. � Luciani, A. Dosisabschätzungen mit einem neuen altersabhängingen Modell für Plutonium, In Jahresbericht 1999 der Hauptabteilung Sichereit, Forschungszentrum Karlsruhe, Redaktion W. Kölzer, Wissenschaftliche Berichte, FZKA 6430, 2000. � Luciani, A. Ein optimiertes biokinetisches Modell für Plutonium, In Jahresbericht 1998 der Hauptabteilung Sichereit, Forschungszentrum Karlsruhe, Redaktion W. Kölzer, Wissenschaftliche Berichte, FZKA 6230, 1999. WORK IN PROGRESS • Luciani, A. Doerfel, H. And Polig, E. Uncertainty analysis of the Plutonium urinary excretion. Accepted as contribution to the Workshop on Internal Dosimetry of Radionuclides – Occupational, Public and Medical Exposure, Oxford, United Kingdom, 9-12 September 2002, Proceedings of the Conference will be published in Radiation Protection Dosimetry. 175
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Forschungszentrum Karlsruhe in der
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Für diesen Bericht behalten wir un
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i ABSTRACT The biokinetic model pre
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ZUSAMMENFASSUNG Das von der Interna
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1 INDEX OF CONTENTS INDEX OF SYMBOL
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3 INDEX OF SYMBOLS Here a short glo
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Chapter 1 Introduction 5
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the duties of the Department for Ra
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adionuclide. Therefore only isotope
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stabilise the +4 oxidation state [1
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techniques adopted in the early pha
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present in spent and MOX reactor fu
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INTRAVENOUS INJECTION skin WOUND bl
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functions, defined as retained and
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the contamination event, of such as
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Table 1.3.2 Indicative 239 Pu detec
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The kinetics of Plutonium in the ki
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1.4.2 COMMENTS ON THE ICRP 67 MODEL
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Chapter 2 Data and measurements 31
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Therefore the radiolysis process, m
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Recent technologic developments in
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eu(t) = 0.19e −0.272t + 0.023e
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function for each of the considered
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the minimum detectable activity of
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2.2.2 AVAILABLE MEASUREMENTS Immedi
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Table 2.2.4 Daily fecal excretion o
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elements the spectral distribution
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The phoswich detector is based on t
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HPGe crystals are produced in cylin
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This quantity is normally expressed
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The peak is located in the region B
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To introduce the second quantity, t
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117 cm 3 h -1 for the incoming and
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Figure 2.3.8 The Lawrence Livermore
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three detectors are used. Two detec
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Table 2.3.4 Efficiency factors of p
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• the necessity of performing mea
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Table 2.3.7 Impulses in the measure
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2.4 ACTIVITY MEASUREMENTS IN BIOASS
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If more then one radionuclide is ma
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L A is the air layer in µgcm -2 ;
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The electrodeposition cell used for
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Table 2.4.1 238 Pu, 239 Pu and 241
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3.1.1 MATHEMATICAL TOOLS 3.1.1.1 So
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calculating the amount of Plutonium
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3.1.2 ANALYSIS OF THE ICRP 67 MODEL
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empirical curves given by Langham,
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the worst performance of the group.
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leave the total clearance from the
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Figure 3.1.4 shows that the use of
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3.1.3 MODIFICATION OF ICRP 67 MODEL
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The structure of Polig’s skeleton
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Percentage daily urinary excretion
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of 0.693d -1 . The values of the F
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Percentage daily urinary excretion
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the basis of all the reference data
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Table 3.1.10 Transfer rates of the
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3.1.4 VERIFICATION OF THE OPTIMIZED
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Table 3.1.13 Intakes and percentage
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soft tissue ST2 soft tissue ST0 sof
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For the routine application of Mode
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excreted by individuals aged sixty
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Table 3.1.20 Exponents and coeffici
Page 133 and 134: tract [57] to consider a contaminat
Page 135 and 136: The sensitivity coefficients for th
Page 137 and 138: Sensitivity coefficients S i Figure
Page 139 and 140: transfer rates on the Plutonium uri
Page 141 and 142: Geometric standard deviations rangi
Page 143 and 144: Percentage daily urinary excretion
Page 145 and 146: Percentage daily urinary excretion
Page 147 and 148: 3.2 APPLICATION OF THE OPTIMIZED MO
Page 149 and 150: lymph nodes, as in the LLNL phantom
Page 151 and 152: Americium in the lungs [Bq] 1000 10
Page 153 and 154: Daily urinary excretion [Bqd -1 ] 1
Page 155 and 156: long time is not yet described by t
Page 157 and 158: excretion that is one of the main i
Page 159 and 160: The comparison of model’s predict
Page 161 and 162: Americium in the lungs [Bq] 1000 10
Page 163 and 164: 153 CONCLUSIONS The optimized model
Page 165 and 166: Annex Quantities used in Radiologic
Page 167 and 168: present. As the radiation weighting
Page 169 and 170: w R is the radiation weighting fact
Page 171 and 172: 161 BIBLIOGRAPHY 1. Plutonium. W. K
Page 173 and 174: 29. Nenot, J.-C. and Stather, J. W.
Page 175 and 176: 55. International Atomic Energy Age
Page 177 and 178: 81. Crowley, J., Lanz, H., Scott, K
Page 179 and 180: 107. Hempelmann, L.H., Langham,W.H.
Page 181 and 182: 137. Breitestein, B.D., Newton, C.E
Page 183: 167. Harrison, J.D., Khursheed, A.,
Page 187 and 188: 177 ACKNOWLEDGEMENTS Special thanks
Page 189 and 190: Name: Andrea Luciani Date and place
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Plutonium Biokinetics in Human Body A. Luciani - Kit-Bibliothek - FZK

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