Plutonium Biokinetics in Human Body A. Luciani - Kit-Bibliothek - FZK

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Main Publications � Luciani, A., Polig, E., Doerfel, H. "An age-related model derived from ICRP 67 model for Plutonium dose assessments: application to an updated case of contamination", Oral Presentation at the "8th International Conference on Low level measurements of actinides and long-lived radionuclides in biological and environmental samples", Oarai, Japan, 16-20 October 2000, Proceedings of the Conference, Journal of Radioanalytical and Nuclear Chemistry 252(2):301-307, 2002. � Luciani, A. “Plutonium dose assessments based on a new model derived from ICRP 67”, Health Phys. 80(6):618-619, 2001 � Luciani, A., Doerfel, H., Polig, E. "Sensitivity analysis of the urinary excretion of Plutonium", Rad. Prot. Dosim. 93(2):179-183, 2001. � Luciani, A., Polig, E. "Verification and modification of the ICRP-67 model for plutonium dose calculation", Health Phys. 78(3):303-310, 2000. � Luciani, A. “Dosisabschätzungen mit einem neuen altersabhängingen Modell für Plutonium”, In Jahresbericht 1999 der Hauptabteilung Sichereit, Forschungszentrum Karlsruhe, Redaktion W. Kölzer, Wissenschaftliche Berichte, FZKA 6430, 2000. � Luciani, A. “Ein optimiertes biokinetisches Modell für Plutonium”, In Jahresbericht 1998 der Hauptabteilung Sichereit, Forschungszentrum Karlsruhe, Redaktion W. Kölzer, Wissenschaftliche Berichte, FZKA 6230, 1999. � Ceccarelli, C., Battisti, P., Gasperi, M., Fantuzzi, E., Pacini, F., Gualdrini, G.F., Pierantoni, M.C., Luciani, A., Diokich, D., Pinchera., A. "Radiation Dose to the Testes after 131I Therapy for Ablation of Postsurgical Thyroid Remnants in patiens with Differentiated Thyroid Cancer", The Journal of Nuclear Medicine, 40(10):1716-1721, 1999. � Luciani, A., Castellani, C.M., Olivero, L., Donato, R. "Caratterizzazione Granulometrica e Valutazione di Dose da Inalazione per un Aerosol Contaminato da Cs 137" IV Congresso di protezione radiologica dei paesi Europei del mediterraneo occidentale - Barcellona, Spagna.27-29 Maggio 1998 Proceedings in "RADIOPROTECCION" (Sociedad Espanola de Proteccion Radiologica. 1998) - Senda Editorial, S.A., Special Issue Maggio 1998, pagg.224-227, 1998. � Berico, M., Luciani, A., Formignani, M. "Atmospheric aerosol in an urban area: measuremens of TSP and PM10 standards and pulmonary deposition assessment", Atmospheric Environment, 31:3659-3665, 1997. 180
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Forschungszentrum Karlsruhe in der
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Für diesen Bericht behalten wir un
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i ABSTRACT The biokinetic model pre
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ZUSAMMENFASSUNG Das von der Interna
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1 INDEX OF CONTENTS INDEX OF SYMBOL
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3 INDEX OF SYMBOLS Here a short glo
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Chapter 1 Introduction 5
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the duties of the Department for Ra
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adionuclide. Therefore only isotope
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stabilise the +4 oxidation state [1
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techniques adopted in the early pha
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present in spent and MOX reactor fu
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INTRAVENOUS INJECTION skin WOUND bl
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functions, defined as retained and
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the contamination event, of such as
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Table 1.3.2 Indicative 239 Pu detec
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The kinetics of Plutonium in the ki
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1.4.2 COMMENTS ON THE ICRP 67 MODEL
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Chapter 2 Data and measurements 31
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Therefore the radiolysis process, m
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Recent technologic developments in
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eu(t) = 0.19e −0.272t + 0.023e
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function for each of the considered
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the minimum detectable activity of
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2.2.2 AVAILABLE MEASUREMENTS Immedi
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Table 2.2.4 Daily fecal excretion o
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elements the spectral distribution
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The phoswich detector is based on t
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HPGe crystals are produced in cylin
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This quantity is normally expressed
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The peak is located in the region B
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To introduce the second quantity, t
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117 cm 3 h -1 for the incoming and
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Figure 2.3.8 The Lawrence Livermore
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three detectors are used. Two detec
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Table 2.3.4 Efficiency factors of p
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• the necessity of performing mea
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Table 2.3.7 Impulses in the measure
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2.4 ACTIVITY MEASUREMENTS IN BIOASS
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If more then one radionuclide is ma
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L A is the air layer in µgcm -2 ;
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The electrodeposition cell used for
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Table 2.4.1 238 Pu, 239 Pu and 241
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3.1.1 MATHEMATICAL TOOLS 3.1.1.1 So
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calculating the amount of Plutonium
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3.1.2 ANALYSIS OF THE ICRP 67 MODEL
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empirical curves given by Langham,
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the worst performance of the group.
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leave the total clearance from the
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Figure 3.1.4 shows that the use of
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3.1.3 MODIFICATION OF ICRP 67 MODEL
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The structure of Polig’s skeleton
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Percentage daily urinary excretion
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of 0.693d -1 . The values of the F
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Percentage daily urinary excretion
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the basis of all the reference data
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Table 3.1.10 Transfer rates of the
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3.1.4 VERIFICATION OF THE OPTIMIZED
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Table 3.1.13 Intakes and percentage
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soft tissue ST2 soft tissue ST0 sof
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For the routine application of Mode
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excreted by individuals aged sixty
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Table 3.1.20 Exponents and coeffici
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tract [57] to consider a contaminat
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The sensitivity coefficients for th
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Sensitivity coefficients S i Figure
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Page 141 and 142: Geometric standard deviations rangi
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Page 145 and 146: Percentage daily urinary excretion
Page 147 and 148: 3.2 APPLICATION OF THE OPTIMIZED MO
Page 149 and 150: lymph nodes, as in the LLNL phantom
Page 151 and 152: Americium in the lungs [Bq] 1000 10
Page 153 and 154: Daily urinary excretion [Bqd -1 ] 1
Page 155 and 156: long time is not yet described by t
Page 157 and 158: excretion that is one of the main i
Page 159 and 160: The comparison of model’s predict
Page 161 and 162: Americium in the lungs [Bq] 1000 10
Page 163 and 164: 153 CONCLUSIONS The optimized model
Page 165 and 166: Annex Quantities used in Radiologic
Page 167 and 168: present. As the radiation weighting
Page 169 and 170: w R is the radiation weighting fact
Page 171 and 172: 161 BIBLIOGRAPHY 1. Plutonium. W. K
Page 173 and 174: 29. Nenot, J.-C. and Stather, J. W.
Page 175 and 176: 55. International Atomic Energy Age
Page 177 and 178: 81. Crowley, J., Lanz, H., Scott, K
Page 179 and 180: 107. Hempelmann, L.H., Langham,W.H.
Page 181 and 182: 137. Breitestein, B.D., Newton, C.E
Page 183 and 184: 167. Harrison, J.D., Khursheed, A.,
Page 185 and 186: JOURNALS OWN PUBLICATIONS RELATED T
Page 187 and 188: 177 ACKNOWLEDGEMENTS Special thanks
Page 189: Name: Andrea Luciani Date and place
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Plutonium Biokinetics in Human Body A. Luciani - Kit-Bibliothek - FZK

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