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Coherent Backscattering from Multiple Scattering Systems - KOPS ...

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2.5 Photon flux <strong>from</strong> a surface<br />

The main contribution of the flux comes <strong>from</strong> the immediate neighborhood of dS, so that<br />

the photon density can be replaced by its first-order Taylor expansion around the origin.<br />

Evaluation of the integral then yields<br />

j ∓ = ρ 0v<br />

4 ± vl∗<br />

6<br />

( ) ∂ρ<br />

∂z<br />

0<br />

where the photon density and its derivative have to be taken at the origin.<br />

If dS is located at a boundary, there will be no flux <strong>from</strong> outside the sample, but internal<br />

reflections will create an apparent flux <strong>from</strong> this direction, which is related to the outgoing<br />

flux by the reflectivity R of the surface: j in = R · j out . This gives the boundary conditions<br />

ρ − 2l∗<br />

3<br />

ρ + 2l∗<br />

3<br />

1 + R<br />

1 − R · ∂ρ<br />

∂z = 0 for an upper boundary, i.e. j + = R · j − and<br />

1 + R<br />

1 − R · ∂ρ<br />

∂z = 0 for a lower boundary, i.e. j − = R · j +<br />

The point where the photon density drops to zero is not located at the boundary but at a<br />

distance 2l∗ 1+R<br />

3 1−R · ∂ρ<br />

∂z<br />

in front of it. We can identify this distance with the average penetration<br />

depth z 0 which we have used above for the image point method, as this also is the point where<br />

the photon density vanishes. Assuming a constant gradient of the photon density distribution<br />

close to the surface, one obtains |z 0 | = 2l∗ 1+R 1+R<br />

3 1−R<br />

≈ 0.67<br />

1−R l∗ . Other solutions are mostly of the<br />

order of |z 0 | ≈ 0.7 for the limit of non-reflective surfaces (see e.g. [53], [54]).<br />

2.5 Photon flux <strong>from</strong> a surface<br />

The experimentally accessible quantity in multiple scattering experiments is not the photon<br />

density distribution inside the sample, but the light intensity emitted <strong>from</strong> a sample surface.<br />

It is obvious that this intensity (or photon flux density) is proportional to the number of<br />

photons, i.e. the photon density, at the surface. One can therefore easily calculate the expected<br />

intensities for the various experimental situations <strong>from</strong> eqns. 2.9 and 2.10.<br />

2.5.1 <strong>Backscattering</strong> geometry<br />

<strong>Backscattering</strong> experiments are usually performed with thick samples, where the influence of<br />

the rear and side surfaces on the photon density distribution can be neglected, and the sample<br />

is well described as an infinite half-space.<br />

In backscattering geometry, photon paths of all lengths contribute to the intensity at the surface,<br />

so that the latter is not fully described by the solution of the diffusion equation, which is<br />

valid only for long photon paths. It has been shown however [44] that correct results can be<br />

15

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