Coherent Backscattering from Multiple Scattering Systems - KOPS ...
Coherent Backscattering from Multiple Scattering Systems - KOPS ...
Coherent Backscattering from Multiple Scattering Systems - KOPS ...
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4 Samples<br />
3 0<br />
2 5<br />
n u m b e r o f p a rtic le s<br />
2 0<br />
1 5<br />
1 0<br />
5<br />
0<br />
1 0 0 1 5 0 2 0 0 2 5 0 3 0 0 3 5 0 4 0 0 4 5 0<br />
p a rtic le d ia m e te r [n m ]<br />
Figure 4.1: Particle size and polydispersity. From the electron microscope image<br />
(left) the distribution of the particle sizes of R700 (right) was obtained by measuring the<br />
diameters of approximately 150 particles [47].<br />
and can quite easily be calculated by measuring the weight m and the spatial dimensions r<br />
and h of the sample, while the mass density ρ of the scattering material can be obtained <strong>from</strong><br />
numerous literature sources.<br />
For strong scattering and low mean free paths, the sample should be as dense as possible. If<br />
however the filling fraction is larger than a certain value (which depends on the mismatch of<br />
the refractive indices of scatterers and surrounding medium) [20], scattering takes place at the<br />
holes rather than the particles, so that there is no use increasing the volume fraction beyond<br />
this value.<br />
4.1.3 Effective refractive index<br />
The refractive index mismatch between the particles and the surrounding medium determines<br />
the effectiveness of the scattering. In contrast, the effective refractive index, which is an average<br />
over the indices of the scatterers, n scat , and the medium in between, n surr , describes<br />
the sample as a whole and is for example needed to calculate the reflectivity of the sample<br />
surface.<br />
Linear approach<br />
The most simple and straightforward approach to calculate the effective refractive index n eff<br />
of a sample is to establish an average medium with an averaged refractive index<br />
36<br />
n eff = f · n scat + (1− f ) · n surr