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Mise en page 1 - Laboratoire National des Champs Magnétiques ...

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2009 METALS, SUPERCONDUCTORS...Transport measurem<strong>en</strong>ts of H c2 and its anisotropy in FeSe 1−x Te x single crystalsExploring the temperature dep<strong>en</strong>d<strong>en</strong>ce of H c2 and itsanisotropy in the new Fe superconductors is an importantexperim<strong>en</strong>tal tool to help revealing the mechanism of superconductivity.For example in LaFeAsO 0.89 F 0.11 , the upturnin curvature for H c2 was observed, which suggeststwo-band superconductivity [Hunte et al, Nature 453, 903(2008)]. The high transition temperatures imply high valuesof H c2 , meaning that it is not easy to obtain the full curvedown to low temperature, and many low temperature valuesof H c2 are in fact extrapolations. However, in order to comparethe real behavior to theoretical models, measurem<strong>en</strong>tsdown to low temperature, and thus at very high field, ar<strong>en</strong>ecessary.A serious limitation at pres<strong>en</strong>t is that the homog<strong>en</strong>eity ofmany samples that are studied is highly questionable, andthe highest T c values are obtained on doped, probably inhomog<strong>en</strong>eous,systems. From this aspect the rec<strong>en</strong>t discoveryof superconductivity in FeSe and FeTe 1−x Se x suggestsa promising new direction as these compounds are close tobeing stoichiometric and have a relatively simple structure.We have rec<strong>en</strong>tly grown single crystals of FeSe [Braithwaiteet al, J. Phys.: Cond<strong>en</strong>s. Matter 21, 232202 (2009)],which so far are not homog<strong>en</strong>eous, and FeTe 1−x Se x whichshow homog<strong>en</strong>eous bulk superconductivity, with T c around14 K, characterized by specific heat measurem<strong>en</strong>ts (figure78), and seem suitable for more detailed studies.In the LNCMI-Gr<strong>en</strong>oble, we have measured the anisotropyof H c2 on our FeTe 1−x Se x single crystals up to 28 T. Thisgives a very precise determination of a large part of thecurve. These measurem<strong>en</strong>ts have be<strong>en</strong> completed by measurem<strong>en</strong>tsin pulsed field in LNCMI-Toulouse where thelow temperature part of the curve was obtained, showingthat H c2 reaches almost 50 T at low temperature (figure 79).Analysis of the data is now in progress but a preliminarystudy suggests that although H c2 significantly exceeds thePauli limit, some Pauli limiting is occurring, and this isquite anisotropic. Refinem<strong>en</strong>ts of the analysis and preparationof a publication are in progress.Figure 78: Specific heat of the single crystal of FeSe 1−x Te xgrown in CEA/Gr<strong>en</strong>oble used in these measurem<strong>en</strong>ts. Inset showsthe electronic part of C/T after subtraction of the phonon contribution.Figure 79: Upper critical field of a FeSe 1−x Te x single crystalgrown in CEA/Gr<strong>en</strong>oble, combining DC field measurem<strong>en</strong>ts upto 9 T made in CEA/Gr<strong>en</strong>oble, DC field measurem<strong>en</strong>ts up to 28T made in LNCMI/Gr<strong>en</strong>oble, and pulsed field measurem<strong>en</strong>ts upto 55 T made in LNCMI/Toulouse. Lines show fits made using aBCS weak coupling model.I. Sheikin, W. KnafoD. Braithwaite , G. Lapertot, C. Marin (CEA/Gr<strong>en</strong>oble, Gr<strong>en</strong>oble, France),59

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