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A. ATES et al./ ISEM2016 Alanya – Turkey Şekil 5.HFO-Si5 ile kolon çıkış derişim oranı (a) Şekil 6. HFO-Si5 ile pseudo second order kinetik model (b) Tartışmalar Silika jelin HFO partikülleriyle yüklenmesiyle gerçekleştirilen adsorbent ile yüksek verimde arsenik giderimi başarılmıştır. Silika- jelin yüksek derişimlerde demir ile modifiye edilebilme özelliği onu diğer adsorbentlere göre üstün tutmuştur. Adsorpsiyon sonrası adsorbent, NaOH + NaCl ile başarılı bir şekilde rejenere edilebilmektedir. Ayrıca kolon çalışmaları, yaklaşık 24000 yatak hacmine kadar arsenik ayrımını sağlayabilmiştir. Teşekkür Bu çalışma Cumhuriyet Üniversitesi Araştırma fonunun (M-585) finansal desteği ile gerçekleştirilmiştir. 880
A. ATES et al./ ISEM2016 Alanya – Turkey Kaynaklar [1] Muhammad S, Shah M.T., Khan S. Arsenic health risk assessment in drinking water and source apportionment using multivariate statistical techniques in Kohistan region, northern Pakistan. Food and Chemical Toxicology 2010;48:2855-2864. [2] Rahman M.M., Naidu R., Bhattacharya P. Arsenic contamination in groundwater in the Southeast Asia region. Environmental Geochemistry and Health 2009; 31:9-21. [3]Thundiyil J., Yuan Y., Smith A.H., Steinmaus C., Seasonal variation of arsenic concentration in wells in Nevada. Environmental Research 2007;104: 367-373. [4] Lamm S.H., Kruse M.B. Arsenic ingestion and bladder cancer mortality - What do the doseresponse relationships suggest about. Hum Ecol Risk Assess 2005;11:433-450. [5] McArthur J.M., Ravenscroft P., Banerjee D.M., Milsom J., Hudson-Edwards K.A., Sengupta S., Bristow C., Sarkar A., Tonkin S., Purohit R. How paleosols influence groundwater flow and arsenic pollution: A model from the Bengal Basin and its worldwide implication. Water Resources Research 2008;44 :1-30. [6] Sengupta S., McArthur J.M., Sarkar A., Leng M.J., Ravenscroft P., Howarth R.J., Banerjee D.M. Do ponds cause arsenic-pollution of groundwater in the Bengal Basin? An answer from West Bengal. Environ Sci Technol 2008;42:5156-5164. [7] Celebi A., Sengorur B., Klove B. Human health risk assessment of dissolved metals in groundwater and surface waters in the Melen watershed, Turkey. Journal of Environmental Science and Health Part a-Toxic/Hazardous Substances & Environmental Engineering 2014;49:153-161. [8] Mohan D., Pittman C.U., Arsenic removal from water/wastewater using adsorbents - A critical review. J Hazard Mater 2007, 142:1-53. [9] Navarro P., Alguacil F.J., Adsorption of antimony and arsenic from a copper electrorefining solution onto activated carbon. Hydrometallurgy 2002;66 :101-105. [10] Carvalho W.A., Mandelli D., Dal Bosco S.M., Jimenez R.S., Figueiredo F.C.A., Uses of Brazilian natural zeolite in the removal of toxic metal cations from wastewater. Stud Surf Sci Catal 2005;158:2105-2112. [11] Chuang C.L., Fan M., Xu M., Brown R.C., Sung S., Saha B., Huang C.P., Adsorption of arsenic(V) by activated carbon prepared from oat hulls. Chemosphere 2005;61 :478-483. [12] Daus B., Wennrich R., Weiss H., Sorption materials for arsenic removal from water: A comparative study. Water Research 2004;38:2948-2954. [13] Zeng L. A method for preparing silica-containing iron(III) oxide adsorbents for arsenic removal. Water Res 2003;37:4351-4358. [14] Zeng L. Arsenic adsorption from aqueous solutions on an Fe(III)-Si binary oxide adsorbent. Water Qual Res J Can 2004;39:267-275. [15] Raven K.P., Jain A. Loeppert R.H. Arsenite and arsenate adsorption on ferrihydrite: Kinetics, equilibrium, and adsorption envelopes. Environ Sci Technol 1998;32:344-349. [16] Jain A., Loeppert R.H. Effect of competing anions on the adsorption of arsenate and arsenite by ferrihydrite. J Environ Qual 2000;29:1422-1430. [17] Pierce M.L., Moore C.B. Adsorption of Arsenite and Arsenate on Amorphous Iron Hydroxide. Water Res 1982;16:1247-1253. [18] Wilkie J.A., Hering J.G. Adsorption of arsenic onto hydrous ferric oxide: Effects of adsorbate/adsorbent ratios and co-occurring solutes. Colloid Surface A 1996;107:97-110. 881
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ISBN 9786054735846

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