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H. NADAROGLU et al./ ISEM2016 Alanya – Turkey 120 Boya giderimi (%) 100 80 60 40 20 3 5 7 9 11 pH Şekil 4. Acid kırmızısı 37 (AR37) azo boyasının TiO 2 nanopartikül varlığında UV katalitik olarak gideriminin pH’ya bağlı değişimi Çalışmada farklı sıcaklıkların etkisi denenmiş ancak oda sıcaklığında yüksek verim elde edildiği için tüm boya giderimi çalışması oda sıcaklığında yapılmıştır. Elde edilen bulgulardan, pH 4.0’da %99.9 oranında Acid kırmızısı 37 (AR37) azo boyasının TiO2 nanopartiküllerinin varlığında UV katalitik olarak giderildiği belirlenmiştir. Çalışmada kısa sürede etkili bir sonucun elde edildiği ve tekrarlanabilir olduğu anlaşılmıştır. Sonuç olarak; AR37 azo boyarmaddesinin TiO2 nanopartikülleri varlığında %99.9 gibi yüksek oranda başarılı ve yan ürün oluşturmadan giderilebildiği belirlenmiştir. Kaynaklar [1] Gupta VK, Suhas Application of low-cost adsorbents for dye removal -A review. Journal of Environmental Management 2009; 90(8): 2313-2342. [2] Georgiou D, Melidis P, Aivasidis A, Gimouhopoulos K. Degradation of azo-reactive dyes by ultraviolet radiation in the presence of hydrogen peroxide, Dyes Pigm. 2002; 52: 69-78. [3] Taslimi P, Adiguzel A, Nadaroglu H, Bozoglu C, Gulluce M. Removal of some textile dyes from aquous solution by using a catalase-peroxidase from Aeribacillus pallidus (P26). Journal of Pure and Applied Microbiology 2013; 7 (4): 2629-2640. [4] Nadaroglu H, Kalkan E, Celebi N. Equilibrium, kinetic and thermodynamic studies on adsorption of Reactive Black 5 dye by laccase modified-red mud from aqueous solutions Fresenius Environmental Bulletin 2014;23 (1) 70-83. [5] Gungor AA, Nadaroglu H, Celebi N. Fenton process for Basic red 9 degradation: ımmobilized apolaccase on a nanomagnetite system. Environmental and Experimental Biology 2014; 12: 121-129. [6] Kalkan E, Nadaroglu H, Celebi N, Tozsin G. Removal of textile dye Reactive Black 5 from aqueous solution by adsorption on laccase-modified silica fume. Desalination and Water Treatment 2014; 52 (31-33): 6122-6134. [7] Kalkan E, Nadaroglu H, Celebi N, Celik H, Tasgin E. Experimental study to remediate of acid fuchsin dye using laccase-modified zeolite from aqueous solutions. Polish Journal of Environmental Studies 2015; 24 (1): 115-124. [8] Nadaroglu H, Gungor AA, Celebi N. Removal of Basic Red 9 (BR9) in aqueous solution by using silica with nano-magnetite by enzymatic with fenton process. International Journal of Environmental Research 2015; 9(3):991-1000. 4 947
H. NADAROGLU et al./ ISEM2016 Alanya – Turkey [9] Nadaroglu H, Kalkan E, Celebi N, Tasgin E. Removal of Reactive Black 5 from wastewater using natural clinoptilolite modified with apolaccase. Clay minerals 2015; 50: 65- 76. [10] Gungor, AA, Celebi N, Nadaroglu H. Removal of basic red 9 in wastewater using green fenton reaction, Fresenius Environmental Bulletin 24 (5b), 2015, 1947-1957. [11] Nadaroglu H, Kalkan E, Demir N. Removal of copper from aqueous solution using red mud, Desalination 2010; 251 (1-3): 90-95. 5 948
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