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Nonlinear Fiber Optics - 4 ed. Agrawal

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432 Chapter 11. Highly <strong>Nonlinear</strong> <strong>Fiber</strong>s<br />

Figure 11.5: Values of n 2 as a function of the relative index difference Δ when fiber core is dop<strong>ed</strong><br />

with GeO 2 (fill<strong>ed</strong> circles) or cladding is dop<strong>ed</strong> with fluorine (empty circles). Straight lines show<br />

a linear fit to the data (After Ref. [27]; c○2002 IEEE.)<br />

beyond 1.6 μm. Inde<strong>ed</strong>, the measur<strong>ed</strong> values of n 2 are close to 4×10 −20 m 2 /W for the<br />

DCFs [25].<br />

The dopant dependence of n 2 does not explain fully the spread in n 2 seen in Table<br />

11.1. It turns out that the length of the fiber us<strong>ed</strong> in the experiment also affects the<br />

measurements. The reason is relat<strong>ed</strong> to the fact that most optical fibers do not maintain<br />

the state of polarization during propagation of light. If the polarization state changes<br />

randomly along the fiber length, one measures an average value of γ that is r<strong>ed</strong>uc<strong>ed</strong> by<br />

a factor of 8/9 (see Section 6.6.3), compar<strong>ed</strong> with the value expect<strong>ed</strong> for bulk samples<br />

that maintain the linear polarization of the incident light [29]. If the standard relation<br />

γ = 2πn 2 /(λA eff ) is us<strong>ed</strong> to d<strong>ed</strong>uce n 2 , the resulting value would be smaller by a factor<br />

of 8/9. Of course, one can account for the polarization effects by simply multiplying<br />

this value by 9/8.<br />

The measur<strong>ed</strong> value of n 2 is also affect<strong>ed</strong> by the width of optical pulses us<strong>ed</strong> during<br />

the experiment. It turns out that the n 2 value is considerably larger under CW or quasi-<br />

CW conditions in which pulse width exce<strong>ed</strong>s 10 ns. The reason is that two other<br />

mechanisms, relat<strong>ed</strong> to molecular motion (Raman scattering) and excitation of acoustic<br />

waves through electrostriction (Brillouin scattering), also contribute to n 2 . However,<br />

their relative contributions depend on whether the pulse width is longer or shorter than<br />

the response time associat<strong>ed</strong> with the corresponding process. For this reason, one<br />

should be careful when comparing measurements made using different pulse widths.<br />

The Raman contribution to the nonlinear susceptibility has been discuss<strong>ed</strong> in Section<br />

2.3.2. The first and second terms in Eq. (2.3.38) represent the electronic (Kerr)<br />

and the nuclear (Raman) contributions, respectively. When pulse width is much larger<br />

than the duration of the Raman response function h R (t), we can treat h R (t) as a delta<br />

function, and the electrons and nuclei contribute to n 2 fully. This is the case in practice<br />

for pulses with widths >1 ps. In contrast, the Raman contribution nearly vanishes

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