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Heiss W.D. (ed.) Quantum dots.. a doorway to - tiera.ru

Heiss W.D. (ed.) Quantum dots.. a doorway to - tiera.ru

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Semiconduc<strong>to</strong>r Few-Electron <strong>Quantum</strong> Dots as Spin Qubits 35<br />

the discrete energy spect<strong>ru</strong>m is independent of the number of electrons on the<br />

dot. Under these assumptions the <strong>to</strong>tal energy of a N-electron dot with the<br />

source-drain voltage, VSD, appli<strong>ed</strong> <strong>to</strong> the source (and the drain ground<strong>ed</strong>), is<br />

given by<br />

U(N) = [−|e|(N − N0)+CSVSD + CgVg] 2<br />

2C<br />

+<br />

N�<br />

En(B) (1)<br />

where −|e| is the electron charge and N0 the number of electrons in the<br />

dot at zero gate voltage, which compensates the positive background charge<br />

originating from the donors in the heterost<strong>ru</strong>cture. The terms CSVSD and<br />

CgVg can change continuously and represent the charge on the dot that is<br />

induc<strong>ed</strong> by the bias voltage (through the capacitance CS) and by the gate<br />

voltage Vg (through the capacitance Cg), respectively. The last term of (1)<br />

is a sum over the occupi<strong>ed</strong> single-particle energy levels En(B), which are<br />

separat<strong>ed</strong> by an energy ∆En = En −En−1. These energy levels depend on the<br />

characteristics of the confinement potential. Note that, within the CI model,<br />

only these single-particle states depend on magnetic field, B.<br />

To describe transport experiments, it is often more convenient <strong>to</strong> use the<br />

electrochemical potential. This is defin<strong>ed</strong> as the energy requir<strong>ed</strong> <strong>to</strong> add an<br />

electron <strong>to</strong> the quantum dot:<br />

µ(N) ≡ U(N) − U(N − 1) =<br />

�<br />

N − N0 − 1<br />

2<br />

�<br />

n=1<br />

EC − EC<br />

|e| (CSVSD + CgVg)+EN<br />

where EC = e 2 /C is the charging energy. The electrochemical potential for<br />

different electron numbers N is shown in Fig. 7a. The discrete levels are spac<strong>ed</strong><br />

by the so-call<strong>ed</strong> addition energy:<br />

Eadd(N) =µ(N +1)− µ(N) =EC + ∆E . (2)<br />

The addition energy consists of a purely electrostatic part, the charging energy<br />

EC, plus the energy spacing between two discrete quantum levels, ∆E. Note<br />

that ∆E can be zero, when two consecutive electrons are add<strong>ed</strong> <strong>to</strong> the same<br />

spin-degenerate level.<br />

Of course, for transport <strong>to</strong> occur, energy conservation ne<strong>ed</strong>s <strong>to</strong> be satisfi<strong>ed</strong>.<br />

This is the case when an electrochemical potential level falls within the “bias<br />

window” between the electrochemical potential (Fermi energy) of the source<br />

(µS) and the drain (µD), i.e. µS ≥ µ ≥ µD with −|e|VSD = µS − µD. Only<br />

then can an electron tunnel from the source on<strong>to</strong> the dot, and then tunnel<br />

off <strong>to</strong> the drain without losing or gaining energy. The important point <strong>to</strong><br />

realize is that since the dot is very small, it has a very small capacitance<br />

and therefore a large charging energy – for typical <strong>dots</strong> EC ≈ afewmeV.<br />

If the electrochemical potential levels are as shown in Fig. 7a, this energy is<br />

not available (at low temperatures and small bias voltage). So, the number of

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