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Heiss W.D. (ed.) Quantum dots.. a doorway to - tiera.ru

Heiss W.D. (ed.) Quantum dots.. a doorway to - tiera.ru

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Semiconduc<strong>to</strong>r Few-Electron <strong>Quantum</strong> Dots as Spin Qubits 87<br />

We also have the possibility <strong>to</strong> initialize the dot <strong>to</strong> a mix<strong>ed</strong> state, where<br />

the spin is probabilistically in |↑〉or |↓〉. In Sect. 5, mix<strong>ed</strong>-state initialization<br />

was demonstrat<strong>ed</strong> in a parallel field by first emptying the dot, follow<strong>ed</strong> by<br />

placing both spin levels below EF during the “injection stage” (Fig. 37c).<br />

The dot is then randomly fill<strong>ed</strong> with either a spin-up or a spin-down electron.<br />

This is very useful, e.g. <strong>to</strong> test two-spin operations (see paragraph 6.6).<br />

In a large perpendicular field providing a strong spin-selectivity, initialization<br />

<strong>to</strong> the |↑〉 state is possible via spin relaxation (Fig. 37a) or via direct<br />

injection (Fig. 37d). Initialization <strong>to</strong> a mix<strong>ed</strong> state (or in fact <strong>to</strong> any state other<br />

than |↑〉) is very difficult due <strong>to</strong> the spin-selectivity. It probably requires the<br />

ability <strong>to</strong> coherently rotate the spin from |↑〉<strong>to</strong> |↓〉(see paragraph 6.5).<br />

6.4 Coherence Times<br />

The long-term potential of GaAs quantum <strong>dots</strong> as electron spin qubits clearly<br />

depends c<strong>ru</strong>cially on the spin coherence times T1 and T2. In Sect. 5, wehave<br />

shown that the single-spin relaxation time, T1, can be very long – on the order<br />

of 1 ms at 8 T. This implies that the spin is only very weakly disturb<strong>ed</strong> by the<br />

environment. The dominant relaxation mechanism at large magnetic field is<br />

believ<strong>ed</strong> <strong>to</strong> be the coupling of the spin <strong>to</strong> phonons, m<strong>ed</strong>iat<strong>ed</strong> by the spin-orbit<br />

interaction [22].<br />

The fundamental quantity of interest for spin qubits is the decoherence<br />

time of a single electron spin in a quantum dot, T2, which has never been measur<strong>ed</strong>.<br />

Experiments with electrons in 2DEGs have establish<strong>ed</strong> an ensembleaverag<strong>ed</strong><br />

decoherence time, T ∗ 2 , of ∼100 ns [89]. Recently, a similar lower<br />

bound on T2 has been claim<strong>ed</strong> for a single trapp<strong>ed</strong> electron spin, bas<strong>ed</strong> on the<br />

linewidth of the observ<strong>ed</strong> electron spin resonance [90]. Theoretically, it has<br />

been suggest<strong>ed</strong> that the real value of T2 can be much longer [22], and under<br />

certain circumstances could even be given by T2 =2T1, limit<strong>ed</strong> by the same<br />

spin-orbit interactions that limit T1.<br />

To build a scalable quantum computer, a sufficiently long T2 (corresponding<br />

<strong>to</strong> more than 10 4 times the gate operation time) is essential in order <strong>to</strong><br />

reach the “accuracy threshold”. However, for experiments in the near future,<br />

we only ne<strong>ed</strong> <strong>to</strong> perform a few spin rotations within T2, which might already<br />

be possible for much shorter T2, on the order of a µs. This should also be long<br />

enough <strong>to</strong> perform two-spin operations, which are likely <strong>to</strong> be much faster. To<br />

find the actual value of T2, the ability <strong>to</strong> perform coherent spin operations is<br />

requir<strong>ed</strong>. This is discuss<strong>ed</strong> in the next paragraphs.<br />

6.5 Coherent Single-Spin Manipulation: ESR<br />

We have not yet satisfi<strong>ed</strong> the key requirement for an actual spin qubit: coherent<br />

manipulation of one- and two-spin states. To controllably create superpositions<br />

of |↑〉and |↓〉, we can use the well-known electron spin resonance

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