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Heiss W.D. (ed.) Quantum dots.. a doorway to - tiera.ru

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36 J.M. Elzerman et al.<br />

a b c d<br />

µ( N+ 1)<br />

µ S µ( N)<br />

µ D<br />

µ( N-1)<br />

E add<br />

Γ L<br />

µ( N+ 1)<br />

µ( N )<br />

Γ R<br />

eV SD<br />

µ( N )<br />

∆E<br />

µ( N+ 1)<br />

µ( N)<br />

Fig. 7. Schematic diagrams of the electrochemical potential of the quantum dot<br />

for different electron numbers. (a) No level falls within the bias window between<br />

µS and µD, sotheelectronnumberisfix<strong>ed</strong>atN − 1 due <strong>to</strong> Coulomb blockade.<br />

(b) Theµ(N) level is align<strong>ed</strong>, so the number of electrons can alternate between N<br />

and N − 1, resulting in a single-electron tunneling current. The magnitude of the<br />

current depends on the tunnel rate between the dot and the reservoir on the left,<br />

ΓL, andontheright, ΓR. (c) Both the ground-state transition between N − 1and<br />

N electrons (black line), as well as the transition <strong>to</strong> an N-electron excit<strong>ed</strong> state<br />

(gray line) fall within the bias window and can thus be us<strong>ed</strong> for transport (though<br />

not at the same time, due <strong>to</strong> Coulomb blockade). This results in a current that is<br />

different from the situation in (b). (d) The bias window is so large that the number<br />

of electrons can alternate between N − 1, N and N + 1, i.e. two electrons can tunnel<br />

on<strong>to</strong> the dot at the same time<br />

electrons on the dot remains fix<strong>ed</strong> and no current flows through the dot. This<br />

is known as Coulomb blockade.<br />

Fortunately, there are many ways <strong>to</strong> lift the Coulomb blockade. First,<br />

we can change the voltage appli<strong>ed</strong> <strong>to</strong> the gate electrode. This changes the<br />

electrostatic potential of the dot with respect <strong>to</strong> that of the reservoirs, shifting<br />

the whole “ladder” of electrochemical potential levels up or down. When a level<br />

falls within the bias window, the current through the device is switch<strong>ed</strong> on. In<br />

Fig. 7b µ(N) is align<strong>ed</strong>, so the electron number alternates between N − 1and<br />

N. This means that the Nth electron can tunnel on<strong>to</strong> the dot from the source,<br />

but only after it tunnels off <strong>to</strong> the drain can another electron come on<strong>to</strong> the<br />

dot again from the source. This cycle is known as single-electron tunnelling.<br />

By sweeping the gate voltage and measuring the current, we obtain a trace<br />

as shown in Fig. 8a. At the positions of the peaks, an electrochemical potential<br />

level is align<strong>ed</strong> with the source and drain and a single-electron tunnelling<br />

current flows. In the valleys between the peaks, the number of electrons on<br />

the dot is fix<strong>ed</strong> due <strong>to</strong> Coulomb blockade. By tuning the gate voltage from<br />

one valley <strong>to</strong> the next one, the number of electrons on the dot can be precisely<br />

controll<strong>ed</strong>. The distance between the peaks corresponds <strong>to</strong> EC + ∆E, and can<br />

therefore give information about the energy spect<strong>ru</strong>m of the dot.<br />

A second way <strong>to</strong> lift Coulomb blockade is by changing the source-drain<br />

voltage, VSD (see Fig. 7c). (In general, we keep the drain potential fix<strong>ed</strong>, and<br />

change only the source potential.) This increases the bias window and also<br />

“drags” the electrochemical potential of the dot along, due <strong>to</strong> the capacitive<br />

coupling <strong>to</strong> the source. Again, a current can flow only when an electrochemical

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