Heiss W.D. (ed.) Quantum dots.. a doorway to - tiera.ru
Heiss W.D. (ed.) Quantum dots.. a doorway to - tiera.ru
Heiss W.D. (ed.) Quantum dots.. a doorway to - tiera.ru
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36 J.M. Elzerman et al.<br />
a b c d<br />
µ( N+ 1)<br />
µ S µ( N)<br />
µ D<br />
µ( N-1)<br />
E add<br />
Γ L<br />
µ( N+ 1)<br />
µ( N )<br />
Γ R<br />
eV SD<br />
µ( N )<br />
∆E<br />
µ( N+ 1)<br />
µ( N)<br />
Fig. 7. Schematic diagrams of the electrochemical potential of the quantum dot<br />
for different electron numbers. (a) No level falls within the bias window between<br />
µS and µD, sotheelectronnumberisfix<strong>ed</strong>atN − 1 due <strong>to</strong> Coulomb blockade.<br />
(b) Theµ(N) level is align<strong>ed</strong>, so the number of electrons can alternate between N<br />
and N − 1, resulting in a single-electron tunneling current. The magnitude of the<br />
current depends on the tunnel rate between the dot and the reservoir on the left,<br />
ΓL, andontheright, ΓR. (c) Both the ground-state transition between N − 1and<br />
N electrons (black line), as well as the transition <strong>to</strong> an N-electron excit<strong>ed</strong> state<br />
(gray line) fall within the bias window and can thus be us<strong>ed</strong> for transport (though<br />
not at the same time, due <strong>to</strong> Coulomb blockade). This results in a current that is<br />
different from the situation in (b). (d) The bias window is so large that the number<br />
of electrons can alternate between N − 1, N and N + 1, i.e. two electrons can tunnel<br />
on<strong>to</strong> the dot at the same time<br />
electrons on the dot remains fix<strong>ed</strong> and no current flows through the dot. This<br />
is known as Coulomb blockade.<br />
Fortunately, there are many ways <strong>to</strong> lift the Coulomb blockade. First,<br />
we can change the voltage appli<strong>ed</strong> <strong>to</strong> the gate electrode. This changes the<br />
electrostatic potential of the dot with respect <strong>to</strong> that of the reservoirs, shifting<br />
the whole “ladder” of electrochemical potential levels up or down. When a level<br />
falls within the bias window, the current through the device is switch<strong>ed</strong> on. In<br />
Fig. 7b µ(N) is align<strong>ed</strong>, so the electron number alternates between N − 1and<br />
N. This means that the Nth electron can tunnel on<strong>to</strong> the dot from the source,<br />
but only after it tunnels off <strong>to</strong> the drain can another electron come on<strong>to</strong> the<br />
dot again from the source. This cycle is known as single-electron tunnelling.<br />
By sweeping the gate voltage and measuring the current, we obtain a trace<br />
as shown in Fig. 8a. At the positions of the peaks, an electrochemical potential<br />
level is align<strong>ed</strong> with the source and drain and a single-electron tunnelling<br />
current flows. In the valleys between the peaks, the number of electrons on<br />
the dot is fix<strong>ed</strong> due <strong>to</strong> Coulomb blockade. By tuning the gate voltage from<br />
one valley <strong>to</strong> the next one, the number of electrons on the dot can be precisely<br />
controll<strong>ed</strong>. The distance between the peaks corresponds <strong>to</strong> EC + ∆E, and can<br />
therefore give information about the energy spect<strong>ru</strong>m of the dot.<br />
A second way <strong>to</strong> lift Coulomb blockade is by changing the source-drain<br />
voltage, VSD (see Fig. 7c). (In general, we keep the drain potential fix<strong>ed</strong>, and<br />
change only the source potential.) This increases the bias window and also<br />
“drags” the electrochemical potential of the dot along, due <strong>to</strong> the capacitive<br />
coupling <strong>to</strong> the source. Again, a current can flow only when an electrochemical