FATE OF MERCURY IN THE ARCTIC Michael Evan ... - COGCI

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Fate of Mercury in the Arctic Paper 1: Goodsite, M.E., Brooks, S.B., Lindberg, S.E. Meyers, T.P Skov, H. and Larsen, M.R.B. (2003) The Fluxes of Reactive Gaseous Mercury measured with a newly developed method using Relaxed Eddy Accumulation. Submitted to Atmospheric Environment, June 2003.
Submitted to Atmospheric Environment The Fluxes of Reactive Gaseous Mercury Measured with a Newly Developed Method using Relaxed Eddy Accumulation Michael E. Goodsite a,b,d,e* , Henrik Skov a , Steve B. Brooks c , Steve E. Lindberg d , Tilden P. Meyers e , Matt Landis f , Michael R.B. Larsen a,e , Glen McConville g a National Environmental Research Institute, Frederiksborgvej 399, 4000 Roskilde, Denmark b Present address: MEG: Department of Chemistry University of Southern Denmark, Campusvej 55, 5230 Odense M., Denmark c Oak Ridge Associated Universities, P.O. Box 117, Oak Ridge, Tennessee 37831-0117 d Environmental Sciences Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831-6038 e Atmospheric Turbulence and Diffusion Division, National Oceanic and Atmospheric Administration, Oak Ridge, Tennessee 37831-0117 f U.S. EPA, 79 TW Alexander Drive, Human Exposure Analysis Branch, MD-56, Research Triangle Park, North Carolina 27711 g CLIMATE MONITORING AND DATA LABORATORY, National Oceanic and Atmospheric Administration,Barrow, Alaska * Corresponding author. Tel.: +45 65 50 25 57; fax: +45- 65 50 12 14. E-mail address: meg@chem.sdu.dk (Mike Goodsite). 1
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Page 149 and 150: 1. Introduction Mercury in the atmo
Page 151 and 152: For all flux measurements, heating
Page 153 and 154: esponse switching valves supplied b
Page 155 and 156: 3.1 RGM flux measurements The resul
Page 157 and 158: estimating for Alert an average spr
Page 159 and 160: References 1. Businger J.A. and Onc
Page 161 and 162: Table captions Table 1. RGM mass ra
Page 163 and 164: Figure 2. RGM pg m-3 350 300 250 20
Page 165 and 166: Table 2 DAYHOURMON avg.temp avg.WS
Page 167 and 168: Fate of Mercury in the Arctic Paper
Page 169 and 170: FIGURE 1. Schematic diagram of the
Page 171 and 172: mass flow controller to 10 L/min an
Page 173 and 174: FIGURE 3. Trends in Hg 0 (upper plo
Page 175 and 176: FIGURE 6. Trends in several Hg spec
Page 177 and 178: FIGURE 7. Spatial patterns in month
Page 179 and 180: (51) Ebinghaus, R.; Kock, H. H.; Te
Page 181 and 182: The fate of elemental mercury in Ar
Page 183 and 184: Ozone was measured with an UV absor
Page 185 and 186: demonstrating that BrO and ClO with
Page 187 and 188: In the model the removal of GEM lea
Page 189 and 190: 15. Kemp, K. and Wåhlin, P. Applic
Page 191 and 192: GEM, ng/m 3 Fig 3. GEM against ozon
Page 194 and 195: Fig. 6 Comparison of measured surfa
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Fate of Mercury in the Arctic Paper
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Introduction The perennial oxidatio
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Ariya et al. (11) have shown recent
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Table 1 lists the binding energies
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and a classical densities of states
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The third point demonstrated in Fig
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7. Lamborg, C. H.; Fitzgerald, W.;
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Figure 1. k rec / cm 3 molecule -1
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Asian Chemistry Letters vol. XX, No
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496 M E Goodsite et al. In the pres
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498 M E Goodsite et al. Figure 1 Th
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500 M E Goodsite et al. observed a
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502 M E Goodsite et al. Table 1 14C
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504 M E Goodsite et al. annual reso
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506 M E Goodsite et al. Table 2b Sa
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508 M E Goodsite et al. Going from
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510 M E Goodsite et al. dry mass. T
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512 M E Goodsite et al. Figure 4 Hg
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514 M E Goodsite et al. Koenig B, L
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130 F. Roos-Barraclough et al. / Th
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ABSTRACT Mercury concentrations are
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INTRODUCTION Atmospheric pollution
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and the relative importance of natu
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corresponding to the alkaline igneo
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edges cut off the slices were dried
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Age dating using 14 C Plant macrofo
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espectively (Naucke et al., 1993).
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200 was in the range 1 to 3 :g/m 2
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unpublished data for these paramete
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leachable fraction, and 32.1 µg/g
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indicator of the concentration of a
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caused by the introduction of gasol
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porewaters reveals the influence of
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For example, Hg may become adsorbed
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of the GL profile. Comparison with
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further improve our knowledge of pr
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which are derived from them. In con
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ACKNOWLEDGEMENTS We are grateful to
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Bindler, R. (2003) Estimating the n
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of Southern Denmark. Goodsite, M.E.
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MacKenzie AB, Farmer JG, Sugden CL.
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Schroeder, W.H. and Munthe, J. (199
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Table 1. AMS 14 C dating of plant m
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Table 3. Pb isotope data of leachat
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esidual fractions of the “B” co
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Depth (cm) Depth (cm) a b 0 -10 -20
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Hg accumulation rate (µg/m2/yr) 10
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Depth (cm) a Pb/Zr = UCC Depth (cm)
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Depth (cm) a Depth (cm) b 0 -10 -20
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Depth (cm) Depth (cm) a b 0 -10 -20
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Saturday, 28 December 2002 (Revised
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INTRODUCTION Recent research utiliz
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In addition, the coring system incl
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and testing prior to the Carey Isla
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ACKNOWLEDGEMENTS Development of thi
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Fig. 5. The stainless steel (AISI 3
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Fig. 2. 13
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Fig. 4. 15
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Fig. 6. 17
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FATE OF MERCURY IN THE ARCTIC Michael Evan ... - COGCI

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