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Contents - Max-Planck-Institut für Physik komplexer Systeme

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|| 2<br />

1<br />

0.8<br />

0.6<br />

0.4<br />

0.2<br />

0 2 4 6 8 10<br />

1<br />

0<br />

0 50 100 150 200<br />

t (fs)<br />

0.95<br />

Figure2: Survivalprobabilityofa2svacancy<br />

inNe5H + (solidline)-theexponentialdecay<br />

isshownwithadashedline. Theinset(logarithmicscale)showsthedeviationfromtheexponentialdecayatshorttimes.<br />

Note,thatfor<br />

timesbeyondthatoftheinsetthebeginning<br />

motionofthenucleiwillchangethepresentresultswhichisbasedonstaticnuclei.<br />

0.9<br />

Electronic decay in charged environment While<br />

thepresenceofasinglechargecanmodifytherate<br />

oftheexponentialdecayofacore-ionizedstate, a<br />

multiplepositiveenvironmentcandramaticallychange<br />

thedecayandevenleadtoanoscillatorybehavior[3].<br />

ThisisduetothefactthattheAugerelectronisnot<br />

ejectedintoatruecontinuum,butratherintoamanifoldofshake-upboundstates.Asaconsequence,the<br />

outgoingelectronwaveiseventuallyreflectedfrom<br />

theeffectivepotentialboundary. Asimilarproblem<br />

wasencounteredbyBixonandJortnerinthecontextofnon-radiativedecay[13]andsolvedtherefor<br />

amodelproblem.WehavedevelopedanADC-based<br />

time-dependentfirst-principlesapproachthatisable<br />

topredictthetruedynamicsofelectronicdecayina<br />

givenhighlyionizedsystem. ForCoster-Kronigdecayof<br />

(2s −1 )Ar + ArinmultiplyionizedAr13cluster,<br />

wefindaroughlyexponentialdecayinthebeginning<br />

whichiseventuallysuppressedbytheoscillatorywavepacketdynamicsatlatertimes,seeFig.1.<br />

Forthe<br />

muchslowerexponentialICDinadoublyionizedNe6<br />

cluster,wefindasub-exponentialdecayinthecharged<br />

environment(Fig.2).<br />

[1] S.Kopelke,K.Gokhberg,L.S.CederbaumandV.Averbukh,J.Chem.Phys.130,144103(2009).<br />

[2] V.AverbukhandP.Kolorenč,Phys.Rev.Lett.103,183001(2009).<br />

[3] V.Averbukh,U.SaalmannandJ.M.Rost,Phys.Rev.Lett.104,233002(2010).<br />

[4] See,e.g.M.A.Kornberg,A.L.Godunov,S.Itza-Ortiz,D.L.Ederer,J.H.McGuireandL.Young,J.SynchrotronRad.9,298(2002).<br />

[5] U.SaalmannandJ.M.Rost,Phys.Rev.Lett.89,143401(2002).<br />

[6] K.Gokhberg,V.AverbukhandL.S.Cederbaum,J.Chem.Phys.126,154107(2007).<br />

[7] R.SantraandL.S.Cederbaum,Phys.Rev.Lett.90,153401(2003).<br />

[8] Y.Morishita,X.-J.Liu,N.Saito,T.Lischke,M.Kato,G.Prümper,M.Oura,H.Yamaoka,Y.Tamenori,I.H.Suzuki,Phys.Rev.Lett.<br />

96,243402(2006).<br />

[9] P.Kolorenč,V.Averbukh,K.GokhbergandL.S.Cederbaum,J.Chem.Phys.129,244102(2008).<br />

[10] V.Averbukh,P.Kolorenč,K.GokhbergandL.S.Cederbaum,ProgressinTheoreticalChemistryandPhysics(Springer),2009,Volume<br />

20,PartII,155-181,ProceedingsofThirteenthInternationalWorkshoponQuantumSystemsChemistryandPhysics,editedbyP.<br />

Piecuchetal.<br />

[11] V.Averbukh,U.SaalmannandJ.M.Rost,inpreparation.<br />

[12] R.Neutze,R.Wouts,D.vanderSpoel,E.WeckertandJ.Hajdu,Nature406,752(2000).<br />

[13] M.BixonandJ.Jortner,J.Chem.Phys.48,715(1967).<br />

Thephysicsofproteinaggregationphenomena<br />

(Dr.ChiuFanLee)<br />

Thephysicsofproteinaggregationphenomena Mycurrentmainresearchinterestsconcernthe<br />

phenomenaofproteinaggregation,andtheirrelationstohumanpathologyanddevelopmentalbiology.<br />

Specifically,Iaminvestigatingtheaggregationphenomenaof(i)proteinamyloids,whicharelinearselfassembledstructureofproteinsthatareintimatelyrelatedtoagreatvarietyofhumandiseasessuchastheAlzheimer’sdiseaseandtypeIIdiabetes,and(ii)Pgranules,whicharegermcellgranulesintheonecellembryooftheroundwormC.elegans.<br />

Thesegranulesareinstrumentaltotheproperdevelopment<br />

ofthegametesoftheorganism.<br />

104 DetailsandData

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