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VERS UNE MEMOIRE QUANTIQUE AVEC DES IONS PIEGES

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tel-00430795, version 1 - 9 Nov 2009<br />

122 CHAPITRE 5. CHARGEMENT DU PIÈGE<br />

Photoionisation loading of large Sr + ion clouds with ultrafast pulses. 5<br />

1000 trapped ions. In fact, with TPPI an optimum of<br />

4 × 10 4 trapped Sr + ions is obtained for Vrf = 125 V.<br />

In the case of EB it is impossible to explore the same<br />

range for the parameter Vrf without affecting the sample<br />

purity, since too many spurious ionic species, of mass<br />

lower than Sr, are produced and trapped at low Vrf .<br />

This effect is clearly visible in the mass spectra of Figure<br />

6b obtained with the two techniques in an intermediate<br />

regime (Vrf = 350 V). Therefore, in our case of a noncrystalized<br />

regime, the possibility to work at a low Vrf<br />

is crucial in order to obtain a large number of trapped<br />

ions. We interpret this result in terms of rf-heating process<br />

that increases with Vrf [30]. In this situation, and<br />

in the presence of laser-cooling, the ion-density depends<br />

on the balance between cooling and heating. A maximum<br />

density is then achievable by minimizing Vrf (i.e.<br />

the rf heating) within the stability region. But the total<br />

number of trapped ions also depends on the volume<br />

of the trap that is imposed by Vrf and Vec. Numerical<br />

simulations carried-out using Simion R○ software[26] allowed<br />

us to estimate the trap volume as a function of<br />

Vrf for Vec = 500 V. An optimum (maximum) volume<br />

is obtained for Vrf = 180 V, slightly larger than the<br />

experimental value that maximizes the total number of<br />

trapped ions. Let us note that for low-temperature samples<br />

(e.g. in crystallized regime) the ion density increases<br />

by increasing Vrf , provided that the rf-heating remains<br />

low enough to prevent the melting of the crystal.<br />

We also observed that, when working in the regime of<br />

relatively high Vrf , that is optimal for EB (Vrf = 500V ),<br />

1100±5% ions can be trapped by EB to be compared to<br />

1200 ± 5% ions obtained by photoionisation. This small<br />

discrepancy might be explained by space charge effects<br />

due to electrons that can perturb the trap electrostatic<br />

potential. Let us also finally remark that the selectivity<br />

of the TPPI technique allowed us to load pure Sr + clouds<br />

in the trap at very low oven temperatures (on the order<br />

of 120 ◦ C), contrary to the case of EB (on the order<br />

of 165 ◦ C). As mentioned above, this lower temperature<br />

implies a vapour pressure reduction of several orders of<br />

magnitude.<br />

4 Conclusion<br />

We demonstrated the loading of Sr + in a linear Paul trap<br />

using two-photon absorption of ultrafast pulses centered<br />

at 431 nm. We compared this technique to the electron<br />

bombardment loading and observed several advantages,<br />

already mentioned in previous experiments concerning<br />

other species or other photo-excitation paths. In particular<br />

this technique allowed us to selectively load pure<br />

Sr + clouds, to explore trapping regimes with low RF<br />

voltages, to obtain large cooled-ion clouds, and to improve<br />

the vacuum quality by lowering the power in the<br />

Sr oven. Concerning this last point, it has been possible<br />

to reduce the expected Sr partial pressure near the<br />

oven filament by roughly 4 orders of magnitude. Our results<br />

have been obtained with a home-made femtosecond<br />

source that delivers relatively low energy pulses.<br />

We expect an improvement of two orders of magnitudes<br />

in the photoionization rate in the case of commercially<br />

available Ti:Sa oscillators delivering routinely 10 nJ per<br />

pulse. Let us finally mention that the trapping of up to<br />

4 × 10 4 cooled Sr + ions is an important step towards the<br />

realization of an ion-based quantum memory[31].<br />

5 Acknowledgments<br />

We thank P. Lepert for technical support. The authors<br />

would also like to thank M. Joffre for the loan of the femtosecond<br />

oscillator. This work was supported by ANR<br />

“jeunes chercheuses et jeunes chercheurs” research contract<br />

JC05 61454.<br />

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055403 (2007)

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