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ORNL-5388 - the Molten Salt Energy Technologies Web Site

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4-48<br />

4.5. LIQUID-METAL FAST BREEDER REACTORS<br />

T. J. Burns<br />

Oak Ridge National Laboratory<br />

A preliminary analysis of <strong>the</strong> impact of denatured fuel on breeder reactors was<br />

performed by Argonne National Laboratory, Hanford Engineering Development Laboratory,2<br />

and Oak Ridge National Laboratory3 for a variety of fissile/fertile fuel options.<br />

analysis concentrated principally on oxide-fueled LMFBRs due to <strong>the</strong>ir advanced state of<br />

development relative to o<strong>the</strong>r potential breeder concepts.<br />

Table 4.5-1 summarizes some of <strong>the</strong> significant design and performance parameters<br />

for <strong>the</strong> various LMFBR designs considered. The procedure followed by each analysis group<br />

in assessing <strong>the</strong> impact of alternate fuel cycles was essentially <strong>the</strong> same.<br />

The<br />

A reference<br />

design (for <strong>the</strong> Pu/~~*U cycle) was selected and analyzed, and <strong>the</strong>n <strong>the</strong> performance para-<br />

meters of alternate fissile/fertile combinations were calculated by replacing <strong>the</strong> refer-<br />

ence core and blanket material by <strong>the</strong> appropriate alternative material (s).<br />

As indicated by Case 1 in Table 4.5-1, a different reference design was selected<br />

by each group, emphasizing different design characteristics. The three basic designs do<br />

share certain characteristics, however. Each is a "classical" LMFBR design consisting of<br />

two core zones of different fissile enrichments surrounded by blankets (axial and radial)<br />

of fertile material. In assessing <strong>the</strong> performance impact of various fissile/fertile com-<br />

binations, no attempt was made to modify or optimize any of <strong>the</strong> designs to account for<br />

<strong>the</strong> better <strong>the</strong>rmophysical properties (e.g., me1 ting point, <strong>the</strong>rmal conductivity, etc.)<br />

of <strong>the</strong> alternate materials relative to <strong>the</strong> reference system. (Note: The question of<br />

selection and subsequent optimization of proliferation-resistant LMFBR core designs is<br />

currently being addressed as part of <strong>the</strong> more detailed Proliferation-Resistant Core<br />

Design study being carried out by DOE and its contractor^.)^<br />

In all cases ENDF/B-IV nuclear data5 were utilized in <strong>the</strong> calculations. The ade-<br />

quacy of <strong>the</strong>se nuclear data relative to detailed evaluation of <strong>the</strong> denatured fuel cycle<br />

fast systems is open to some question. Recent measurements of <strong>the</strong> capture cross section<br />

of 232Th,6 <strong>the</strong> primary fertile material in <strong>the</strong> denatured fuel cycle, indicate significan<br />

discrepancies between <strong>the</strong> measured and tabulated ENDF/B-IV cross sections for <strong>the</strong> energy<br />

range of interest. Additionally, <strong>the</strong> adequacy of <strong>the</strong> nuclear data for <strong>the</strong> primary de-<br />

natured fissile species, 233U, for <strong>the</strong> LMFBR spectral range has also been questioned.'<br />

Due to <strong>the</strong>se possible nuclear data uncertainties and also to <strong>the</strong> lack of design optimiza-<br />

tion of <strong>the</strong> reactors <strong>the</strong>mselves, it is prudent to regard <strong>the</strong> results tabulated in<br />

Table 4.5-1 as preliminary evaluations, subject to revision as more data become available.<br />

The compound system fissile doubling time given in Table 4.5-1 was calculated using<br />

<strong>the</strong> simple approximation that<br />

C.S.D.T =<br />

0.693 s (Initial Core + Eq. Cycle Charge)<br />

(RF x Eq. Cycle Discharge - Eq. Cycle Charge) '<br />

n<br />

L;<br />

I:

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