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ORNL-5388 - the Molten Salt Energy Technologies Web Site

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4-50<br />

where RF is <strong>the</strong> reprocessing recovery factor (0.98). While such an expression i s not<br />

absolutely correct, it does provide a measure of <strong>the</strong> relative growth capability of each<br />

reactor. Since <strong>the</strong> data sumnarized in Table 4.5-1 are based on three separate reference<br />

LMFBRs operating with a variety of design differences and fuel management schemes, <strong>the</strong><br />

above expression was used simply to provide relative values for each system. It should<br />

also be noted that sane reactor configurations listed have dissimilar core and axial<br />

blanket materials and thus would probably require modifications to standard reprocessing<br />

procedures.<br />

The data presented in Table 4.5-1, although preliminary, do serve to indicate cer-<br />

tain generic characteristics regarding <strong>the</strong> impact of <strong>the</strong> alternate LMFOR fuel options.<br />

considering those cases in which similar core materials but different blanket materials<br />

By<br />

are utilized it is clear that <strong>the</strong> choice of <strong>the</strong> blanket material has only a ra<strong>the</strong>r small<br />

effect on <strong>the</strong> reactor physics parameters. On <strong>the</strong> o<strong>the</strong>r hand, <strong>the</strong> impact of changes in <strong>the</strong><br />

core fissile and fertile materials is considerable, particularly on <strong>the</strong> breeding ratio.<br />

Utilizing 233U as <strong>the</strong> fissile material results in a significant decrease in <strong>the</strong> breeding<br />

ratio relative to <strong>the</strong> corresponding Pu-fueled case (ranging from 0.10 to 0.15, depending<br />

on <strong>the</strong> system). This decrease is due primarily to <strong>the</strong> lower value of v (neutrons produced<br />

per fission) of 2% relative to 239Pu and 241Pu. Somewhat compensating for <strong>the</strong> difference<br />

in v is <strong>the</strong> fact that <strong>the</strong> capture-to-fission ratio of 233U is significantly less than that<br />

of <strong>the</strong> two plutonium isotopes. The differences in breeding ratios given in Table 4.5-1<br />

reflect <strong>the</strong> net result of <strong>the</strong>se two effects, <strong>the</strong> decrease in v clearly dominating. Use of<br />

233U as <strong>the</strong> fissile material also results in a slight decrease in <strong>the</strong> fissile inventory<br />

required for criticality. This is due to two effects, <strong>the</strong> lower capture-to-fission ratio<br />

of 233U relative to <strong>the</strong> plutonium isotopes, and <strong>the</strong> obvious decrease in <strong>the</strong> atomic weight<br />

of 233U relative to Pu (% 2.5%).<br />

. The replacement of 2j*U by zs2Th as <strong>the</strong> core fertile material also has a significant<br />

impact on <strong>the</strong> overall breeding ratio regardless of <strong>the</strong> fissile material utilized. As <strong>the</strong><br />

data in Table 4.5-1 indicate, <strong>the</strong>re is a substantial breeding ratio penalty associated<br />

with <strong>the</strong> use of 232Th as a core material in an LMFBR. This penalty is due to <strong>the</strong> much<br />

lower fast fission effect in 232Th relative to that in 2s*li (roughly a factor of 4 lower).<br />

The fertile fast fission effect is reflected in <strong>the</strong> breeding ratio in two ways. First,<br />

although <strong>the</strong> excess neutrons generated by <strong>the</strong> fission of a fertile nucleus can be sub-<br />

sequently captured by fertile material. <strong>the</strong>ir production is not at <strong>the</strong> expense of a<br />

fissile nucleus. Moreover, <strong>the</strong> fertile fission effect produces energy, <strong>the</strong>reby reducing<br />

<strong>the</strong> fission rate required of <strong>the</strong> fissile material to maintain a given power level. Since<br />

both <strong>the</strong>se effects act to improve <strong>the</strong> breeding ratio, it is not surprising that use of<br />

Th-based fuels result in significant degradation in <strong>the</strong> breeding ratio. A fur<strong>the</strong>r<br />

consequence of <strong>the</strong> reduced fast fission effect of 232Th is a marked increase in fissile<br />

inventory required for criticality, evident from <strong>the</strong> values given in Table 4.5-1 for <strong>the</strong><br />

required initial loadings.<br />

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