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ORNL-5388 - the Molten Salt Energy Technologies Web Site

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production of "denaturable"<br />

operating on conventional and denatured fuel cycles are discussed in Chapter 4 and<br />

summarized in Table 7.1-1, where <strong>the</strong> Light-Water Reactor (LWR) is represented by <strong>the</strong><br />

7-8<br />

3%. The plutonium production rates for various reactors<br />

pressurized-water reactor (PWR); <strong>the</strong> SSCR (Spectral-Shift-Control led Reactor) is a<br />

modified PWR; <strong>the</strong> heavy-water reactor (HWR) is assumed to be a slightly enriched CANDU;<br />

<strong>the</strong> High-Temperature Gas-Cooled Reactor (HTGR) is taken to be <strong>the</strong> Fort St. Vrain plant;<br />

and <strong>the</strong> High-Temperature Reactor (HTR) of <strong>the</strong> Pebble-Bed Reactor (PBR) type is represented<br />

by <strong>the</strong> West German design. Plutonium discharge data for Fast Breeder Reactors (FBRs)<br />

represented by <strong>the</strong> Liquid-Metal Fast Breeder Reactor (LMFBR) are included for comparison.<br />

It is quite clear from Table 7.1-1 that <strong>the</strong> denatured fuel cycle for <strong>the</strong> HWR gives<br />

<strong>the</strong> greatest reduction in plutonium production between <strong>the</strong> regular and denatured cycles.<br />

The HTGR has about <strong>the</strong> same absolute plutonium production for <strong>the</strong> denatured fuel cycle as<br />

<strong>the</strong> HWR and in both cases <strong>the</strong> plutonium amounts are ra<strong>the</strong>r small. The HTR-PBR is best in<br />

absolute minimum plutonium production, yielding only 14 kg/GWe-yr and even less in a highly<br />

optimized design.<br />

Table 7.1-1. Fissile Plutonium Discharge for Various<br />

Reactor and Fuel Cycle Combinations<br />

(Capacity Factor = 0.75)<br />

Fissile Pu Discharge (kg/GWe-yr)<br />

LEU Cycle Pu/U Cycle Denatured Cycle<br />

LWR 7 74 858' 63<br />

SSCR 196 - 72<br />

HWR (CANDU)<br />

HTGR<br />

183b<br />

72 -<br />

32<br />

36<br />

HTR-PBR 63 14<br />

.................................<br />

LMFBR - 991 347<br />

;Plutonium burner.<br />

Slightly enriched CANDU.<br />

For <strong>the</strong> LWR, SSCR and HWR <strong>the</strong> percentage of <strong>the</strong> discharge plutonium that Is fissile<br />

plutonium is approximately <strong>the</strong> same for <strong>the</strong> denatured cycle as for <strong>the</strong> LEU cycle. For<br />

<strong>the</strong> HTGR and PBR, <strong>the</strong> fissile plutonium percentage is only %39% for <strong>the</strong> denatured cycle<br />

(compared to 56% for <strong>the</strong> LEU cycle). Fur<strong>the</strong>r, <strong>the</strong> discharge plutonium from <strong>the</strong> HTGR and PBR,<br />

and also from <strong>the</strong> HWR, is more diluted with o<strong>the</strong>r heavy material by a factor of three to<br />

four than that from <strong>the</strong> LWR or SSCR. Thus, more material must be processed in <strong>the</strong> HTGR,<br />

HTR, and HWR to obtain a given amount of plutonium, which provides an additional prolifera-<br />

tion restraint associated with spent fuel discharged from <strong>the</strong>se reactors. However, <strong>the</strong><br />

on-line refueling feature of <strong>the</strong> CANDU, and also of <strong>the</strong> PBR, may be a disadvantage from a<br />

proliferation viewpoint since low-burnup fuel could be removed and weapons-grade plutonium<br />

extracted from it. On <strong>the</strong> o<strong>the</strong>r hand, premature discharge of low-burnup fuel from <strong>the</strong><br />

reactors would incur economic penalties.<br />

L<br />

L<br />

L<br />

L<br />

I'

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