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ORNL-5388 - the Molten Salt Energy Technologies Web Site

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4-3<br />

4.0. INTRODUCTION<br />

L. S. Abbott, T. J. Burns, and J. C. Cleveland<br />

Oak Ridge National Laboratory<br />

The three preceding chapters have introduced <strong>the</strong> concept of 233U fuel and its use in<br />

nuclear power systems that include secure (guarded) energy centers supporting dispersed power<br />

reactors, <strong>the</strong> rationale for such systems being that <strong>the</strong>y would allow for <strong>the</strong> production and<br />

use of fissile material in a manner that would reduce weapons proliferation risks relative<br />

to power systems that are increasingly based on plutonium-fueled reactors. Throughout <strong>the</strong><br />

discussion it has been assumed that <strong>the</strong> use of denatured 233U fuel in power reactors is<br />

feasible; however, up to this point <strong>the</strong> validity of that assumption has not been addressed.<br />

A number of calculations have been performed by various organizations to estimate <strong>the</strong><br />

impact that conversion to <strong>the</strong> denatured cycle (and also to o<strong>the</strong>r "alternate" fuel cycles)<br />

would have on power reactors, using as models both existing reactors and reactors whose<br />

designs have progressed to <strong>the</strong> extent that <strong>the</strong>y could be deployed before or shortly after<br />

<strong>the</strong> turn of <strong>the</strong> century. This chapter presents pertinent results from <strong>the</strong>se calculations<br />

which, toge<strong>the</strong>r with <strong>the</strong> predictions given in Chapter 5 on <strong>the</strong> availability of <strong>the</strong> various<br />

reactors and <strong>the</strong>ir associated fuel cycles, have been used to postulate specific symbiotic<br />

nuclear power systems utilizing denatured fuel. The adequacy of such systems for meeting<br />

projected electrical energy demands is <strong>the</strong>n <strong>the</strong> subject of Chapter 6.<br />

The impact of an alternate fuel cycle on <strong>the</strong> performance of a reactor will, of<br />

course, be reactor specific and will largely be determined by <strong>the</strong> differences between <strong>the</strong><br />

neutronic properties of <strong>the</strong> fissile and fertile nuclides included in <strong>the</strong> alternate cycle<br />

and those included in <strong>the</strong> reactor's reference cycle.<br />

fuel, <strong>the</strong> fissile nuclide is 233U and <strong>the</strong> primary fertile nuclide is 232Th, with fertile<br />

238U included as <strong>the</strong> 233U denaturant. If LWRs such as those currently providing nuclear<br />

power in <strong>the</strong> United States were to be <strong>the</strong> reactors in which <strong>the</strong> denatured fuel is deployed,<br />

<strong>the</strong>n <strong>the</strong> performance of <strong>the</strong> reactors using <strong>the</strong> denatured fuel must be compared with <strong>the</strong>ir<br />

performance using a fuel comprised of <strong>the</strong> fissile nuclide 23% and <strong>the</strong> fertile isotope<br />

238U.<br />

denatured fuel must also be compared with LWRs in which Pu is recycled. Similarly, if<br />

FBRs were to be <strong>the</strong> reactors in which <strong>the</strong> denatured fuel is deployed, <strong>the</strong>n <strong>the</strong> performance<br />

of FBRs operating on 233U/238U or 233U/238U/232Th and including 232Th i n <strong>the</strong>ir blankets<br />

must be compared with <strong>the</strong> performance of FBRs operating on surrounded by a 238U<br />

blanket.<br />

In <strong>the</strong> case of <strong>the</strong> proposed denatured<br />

And since <strong>the</strong> use of 233U assumes recycle, <strong>the</strong>n <strong>the</strong> performance of <strong>the</strong> LWRs using<br />

A significant poht in <strong>the</strong>se two examples is that <strong>the</strong>y represent <strong>the</strong> two generic<br />

types of power reactors -- <strong>the</strong>ma2 and fast -- and that <strong>the</strong> neutronic properties of <strong>the</strong><br />

fissile and fertile nuclides in a <strong>the</strong>rmal-neutron environment differ from <strong>the</strong>ir properties<br />

in a fast-neutron environment. Thus while one fissile material may be <strong>the</strong> optimum fuel in<br />

a' reactor operating on <strong>the</strong>rmal neutrons (e,g., LWRS) it may be <strong>the</strong> least desirable fuel<br />

for a reactor operating on fast neutrons (e.g., FBRs).

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