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National Technical Information Service U.S. Department of Commerce 5285 Port Royal Road, Springfield, Virginia 22161 Price: Printed Copy $1 1.75; Microfiche $3.00 This report was prepared as an account of work sponsored by an agency of the United States Government. Neither the United States Government norany agency thereof, nor any of their employees, contractors, subcontractors, or their employees, makes any warranty, express or implied, nor assumes any legal liability or responsibility for any third party's use or the results of such use of any information, apparatus, product or process disclosed in this report, nor represents that its use by such third party would not infringe privately owned rights. u
i L i b I, i L L bi L L Contract No. W-7405-eng-26 Engineering Physics Di vi s ion INTERIM ASSESSMENT OF THE DENATURED 23% FUEL CYCLE: FEASIBILITY AND NONPROLIFERATION CHARACTERISTICS Edited by L. S. Abbott, D. E. Bartine, T. J. Burns With Contributions from Argonne National Laboratory Brookhaven National Laboratory Combustion Engineering, Inc. Hanf ord Engineering De vel opment Laboratory Oak Ridge Gaseous Diffusion Plant Oak Ridge National Laboratory C. Sege DOE Program Manager D. E. Bartine ORNL Program Manager I. Spiewak ORNL Program Director December, 1978 OAK RIDGE NATIONAL LABORATORY Oak Ridge, Tennessee 37830 operated by UNION CARBIDE CORPORATION for the DEPARTMENT OF ENERGY DISTRIB~ION c OF THIS DOCUMENT 19 UN ORNL-5388 Distribution Category UC-80 NOTICE Ihh nport was prepared u m account of wok vponsond by the United Sates Gwemmnt. Neither the United Sulci nor the United States Depvtmcnt of Fnerw, nor MY of their amployus. nor MY of their wnlnnon, wbcontnc:mr, or meir employas, mkn my warranty, cxpnn or implied. or p~ymcs my kgnl liability or mpmIJility for the -cy. cnnpleteneu OT Urefulnnr of my infomution. ap1an:uI. product or proocn dirlacd. or rcpnrnb du: itr we would no: hfrhlEC DriWClV omd dhb.
Page 1: Interim Assessment of the Denatured
Page 7 and 8: 1, L L t i Ltr 1 L L V PREFACE AND
Page 9 and 10: L i Li 1, I b k b id ii t L id b i
Page 11 and 12: I L bi i; L 7.3.1. Possible Procedu
Page 13 and 14: i xi I b L ABSTRACT A fuel cycle th
Page 15 and 16: I b .- i, hd t t CHAPTER 1 INTRODUC
Page 17 and 18: - - I 4d _- t .- ! Lili L Ld id .-
Page 19 and 20: L .- k id .- I L: _ - I iclr .- i b
Page 21 and 22: I, G - -- I id ..- ! I _. I: L _.-
Page 23 and 24: huJ -- AI I ' b --- I bl --- t L L
Page 25 and 26: -- t Li - I' b -. c (u I i ai L i i
Page 27 and 28: L - i' u i Lt L r- L t- b L 2-7 den
Page 29 and 30: 2-9 1. Nuclear power is limited to
Page 31: e Isr i L i- b t CHAPTER 3 ISOTOPIC
Page 34 and 35: 232" Fig. 3.0-1. Decay of 232U. ORN
Page 36 and 37: 3-6 3.1. ESTIMATED U CONCENTRATIONS
Page 38 and 39: 3-8 The values in Table 3.1-2 are a
Page 40 and 41: 3-1 0 3.2. RADIOLOGICAL HAZARDS OF
Page 42 and 43: 3-1 2 232u IN RECYCLED HTGR FUEL (p
Page 44 and 45: 3-14 3.2.2 Toxicity of 232Th Given
Page 46 and 47: 1. 2. 3. 4. 5. 6. 7. 8. 9. 10. 11.
Page 48 and 49: 3.18 There are three approaches whi
Page 50 and 51: 1 i i 3-20 3.3.2. Fabrication and H
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The 3-22 3.3.3 Detection and Assay
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3-24 3.3.4. Potential Circumvention
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3-26 - either large centrifuge pilo
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! 3-28 Table 3.3-3. Enriched Proauc
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3-30 The high alpha activity of ura
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3- 32 Table 3.3-7. Sumry of Results
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3-34 statistical redundancy through
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introduce time, cost and visibility
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3-38 An additional factor relative
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I b t I t L 1; L t ki 4.0. 4.1. CHA
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L L _ _ { i J _- \ I b B u il c _.
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Y m I I I . aro ID0 10.00 4-5 ORNL-
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t .. -. F 4d -- I ' L 0- 122, L _-
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L L; L t -I I ' b L -- t i b -- I;
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_- I -- L i d .-- L 4-1 1 Reference
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_- id L t I , 4d i, L id L 5 bi t h
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-- - . & I I ' h I ' Y 61 L -- I( L
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u -- x i I*i 1- bi 4-1 7 The use of
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la - i , I br -_ t c c L e L 4-1 9
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4-21 Case B" is a modification of C
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c 4-23 L i a L L 4.2. SPECTRAL-SHIF
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4-25 Initial analyses of spectral-s
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h 1' b t c i--; & I- & 1: i f 4-27
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c- i L L e I b 4-29 . safeguards fo
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L t i- bi L L t i 4-31 a significan
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~ kc'l c" -1 r-"! r! r-'i c Table 4
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F-- I iJ L ii - L c c 4-35 Referenc
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c r- L i] L h L __ f; t 4-37 trons
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Table 4.4-1. Fuel Utilization Chara
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L I 1 I Ld I ie i-- 1 t' 4-41 4.4.2
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4-43 Table 4.4-4. PBR Coated Partic
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HEU/Th 0.59 Seed i3 Breed 0.58 HEU/
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L i; 1 I i; i 1. 2. 3. 4. 5. 6. 7.
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4-49 Table 4.5-1. Fuel Utilization
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ments. 4-51 The calculations for LM
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1. 2. 3. 4. 5. 6. 7. 8. 4-53 0 77-1
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Table 4.6-1. Comparison of Fuel Uti
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4-57 _I 10 10' 2 2' CASE NUMBER -.
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4-59 Most of the information availa
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- i b k L L -- I , b -- I .- I Li L
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4-63 on only the preliminary data p
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c e E c
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! 5-4 5.1. REACTOR RESEARCH AND DEV
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5-6 As has been pointed out above,
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5-8 the LMFBR on its reference cycl
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5-10 The fuel performance program u
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. 5.1.2. Government Research and De
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5-1 4 The first aspect of large pla
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5-1 6 and should also address metho
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I DATA BASE DEMu)pMENT DEMO DESIGN
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j ~ 5-20 The R,D&D costs are highes
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5-22 In the case of metal-clad oxid
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5-24 5.2.2. Research, Development,
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5-26 program, including hot testing
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c c
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6-4 persed areas ensured - a fact w
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6-6 6.1.2. Reactor Options The reac
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Reactor/Cycl ea LWR-U5(LE)/U-S LUR-
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6-10 6.1.3. Nuclear Policy Options,
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Table 6.1-4. Nuclear Policy Options
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SWU SWU 6-14 UZJS USILEINS WYI U5IL
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6-16 n nM MEDL nows.1 Option 4: In
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6-18 HM HEDL7OOl.70.3 Option 6: In
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SRCIFIED CONSTRUCTION LlMllLD INTRO
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50- 40 6-22 c Y \ VL - :-: F 30- -
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6-24 The potential nuclear contribu
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%- f $400 J 2 s 2, 1 THE LWR FOLLOW
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141.6 ST - U308 4 7.2 lo3 swu ENRIC
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6-30 reactor. Since this increase i
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‘9. ,1 ST ‘3O8 6-32 12 Kg HM I
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6-34 1HE LWR WITH FISSILE UUNIUM PC
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THE LWR WITH PURONIUM MlNUllUTlON A
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6-38 be located in energy centers a
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6-40 installed capacity must be han
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lm, 1 I I I I mf RR WITH UGHT rwrmi
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6-44 6.2.7. Converter-Breeder Syste
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25.2 ST swu 6-46 19 Kg fir Pu 13 Kg
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6-48 Table 6.3-2. Summary of Result
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6-50 (4) If all plutonium produced
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I d r-- 1 > w I r- k z r L id r- .
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L 1 L u without benefit of U.S. exp
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L a, - L i -- k; L t IJ L 7-7 While
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7-9 Viewed solely from the plutoniu
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L L i; i; 7-1 1 routinely in LWRs a
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'I 7-1 3 t I: k: The isotopic compo
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U L L L L ld 1 i" * required 233U m
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I I, i 7-1 7 ii I 1 I L L k L i Thr
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li i i L Li L & I ' i kr ii L i h i
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7-21 7.3. PROSPECTS FOR IMPLEMENTAT
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L I L t L i L i 1 L 7-23 7.3.1. Pos
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7-25 7.3.2. Considerations in Comme
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.. I b k; L; i b b 1J I L 7-27 cycl
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7-29 7.4. ADEQUACY OF NUCLEAR POWER
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L i' hd .- - I ' i t L i' b i -' b
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x ibd 1 .. I i, L -- i t Table 7.4-
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7-35 cycled in Pu/Th converters, th
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L 1' b I_- ,- i b -- I ' b L 7-37 T
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..a 4 I- 1 ' u c1 Y u L 7-39 betwee
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L e, I I ' lb t 7-41 Systems that u
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e-. . ! hr L3 z i- b: i- b L c i li
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7-45 j I Table 7.5-1. Integrated As
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- isi. c ‘Id i L c 7-47 Although
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e Other e e e On the e 7-49 technol
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t a APPENDICES
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A-3 Appendix A. ISOTOPE SEPARATION
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I] 1- $i ill 8 LI b' The Gas Centri
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id A- 7 The Component Preparation L
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i ?L 1- U t L fl bi L c u La -- ti
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p; ‘U i-- L ,c c Japan A-1 1 Tabl
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13 A-13 L" efficient of the units d
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L L L t I h h u L; _- t f is throug
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u A-1 Aerodynamic Methods 7 Both th
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i i d .- I . ii hi L i: i t ' Li 1
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la t L I I, lj ir 1 Li c I L L' B-1
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i; 1 t u 1 1 B-3 Table 8.5. Reactor
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Table 6-7. Marginal Costs of U308 a
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LJ L L1 a .E 4' P Y W 5 18 2 16 : 0
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Appendix C. DETAILED RESULTS FROM E
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1 i; Li b L lkd t L L I hd I ' L; i
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L c-5 The introduction of the class
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i ' ibd 1 b i L L i L I Li . . b b
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E , 1 ' b _. I ' L 1 b _- i G i' b
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-, ii I ; b i- ii L b 4 i L L i‘
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_- I ii I _ _ I L I td C i b L i, L
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Qulatiw klur W i t y hilt (*I thrmg
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L c c b - i ii L r D-1 Appendix D.
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L L L L [i i” Table D -2. Maximum
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Fig. D-2 (cont.) 25W I I I I I (I)
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[i energy center. It can be seen fr
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L L i il L t W 0-9 Table D-4. Summa
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-- Lid c i' .- .b) i Internal Distr
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It e L L L t u I' f ' ki Federal Ag
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u 1' 1" Outside Organizations (cont
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