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ORNL-5388 - the Molten Salt Energy Technologies Web Site

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L<br />

1<br />

L<br />

u<br />

without benefit of U.S. experience.<br />

overriding criterion and could be sacrificed in favor of a more moderate level of<br />

technology.<br />

centrifuge designs to guide mechanically competent engineers with access to adequate<br />

facilities.<br />

technology than prototype construction.<br />

7-5<br />

For a military program, economics would not be an<br />

Moreover, <strong>the</strong> open literature contains sufficient information concerning <strong>the</strong><br />

Replication of an economic design would require a somewhat higher level of<br />

The following particular points regarding <strong>the</strong> enrichment of denatured 233U fuel<br />

should be noted:<br />

Because of <strong>the</strong> lower mass of 233U, separating 23% from 238U would require only 9/25<br />

of <strong>the</strong> effort required to separate 235U from 238U, assuming equal feed enrichments.<br />

Since <strong>the</strong> fast critical mass of 23% is less than that of 235U, less enrichment<br />

capacity would be required to produce a 23% weapon from 233U/238U feed than would<br />

be required to produce a 235U weapon from 235Uf238U feed, again assuming equal<br />

enrichments of <strong>the</strong> feed material.<br />

The higher <strong>the</strong> enrichment of <strong>the</strong> source material, <strong>the</strong> less separative work that would<br />

have to be done to upgrade <strong>the</strong> material to 90% enrichment.<br />

natural uranium to a 10% level consumes 90% of <strong>the</strong> separative work required to<br />

achieve a 90% level. It is to be noted that <strong>the</strong> enrichment of denatured 23% fuel<br />

is approximately 12%, whereas <strong>the</strong> enrichment of currently used LWR 235U fuel is<br />

around 3-4%.<br />

For example, enriching<br />

With respect to items (2) and (3), a rough comparison can be made of <strong>the</strong> feed<br />

requirements and <strong>the</strong> number of centrifuges that would be necessary to produce 90% enriched<br />

material from various fuels in one year (normalized to 1 kg of product):<br />

Number of Centrifuges Required<br />

- Fuel<br />

Feed Required<br />

(kg)<br />

0.3 kg SWUfyr<br />

Capacity<br />

5 kg SWUfyr<br />

Capacity<br />

12% 233u 8 55 3<br />

20% 2351) 5 50 3<br />

3.2% 235U 30 292 17<br />

Natural Uranium 178 779 46<br />

The above values do not consider measures to eliminate <strong>the</strong> 232U contamination and <strong>the</strong>y<br />

assume that a reasonable tails assay will be maintained (%0.2% 235U).<br />

assay were acceptable, <strong>the</strong> number of centrifuges could be reduced but <strong>the</strong> feed material<br />

required would be increased.<br />

If a higher tails<br />

One year, of course, is a long time when compared to a period of weeks that would<br />

be needed to obtain approximately 10 kg of plutonium by chemically reprocessing two to<br />

three spent LWR-LEU fuel elements.<br />

It would be possible to speed up <strong>the</strong> process time for<br />

<strong>the</strong> centrifuge method ei<strong>the</strong>r by increasing <strong>the</strong> individual machine capacity, by adding<br />

additional centrifuges, or by operating at a higher tails assay.<br />

Increasing <strong>the</strong> capacity

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