chemical thermodynamics of neptunium and plutonium - U.S. ...

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BIBLIOGRAPHY 461[59AXE/IHL][59BJO/REA][59DEB/LIC][59EVA/MAR][59GEL/ZAI][59KRE/NIK][59KRE/NIK2][59LEE/MAR][59POP/GAL][59ROB/STO]Axe, Jr., J. D., Ihle, H., “Chemistry division annual progress reportfor June through November, 1958”, Tech. Rep. UCRL–8618, CaliforniaUniversity, California, USA, 1959, Chapter: Calorimetry, p.86. Cited pages 302, 544, 552Bjorklund, C. W., Reavis, J. G., Leary, J. A., Walsh, K. A., “Phaseequilibria in the binary systems PuCl 3 -NaCl and PuCl 3 -LiCl”, J.Phys. Chem., 63 (1959) 1774–1777. Cited pages 356, 356, 367,545, 555, 562, 567DeBethune, A. J., Licht, T. S., Swendeman, N., “The temperaturecoefficients of electrode potentials: the isothermal and thermalcoefficients–the standard ionic entropy of electrochemical transportof the hydrogen ion”, J. Electrochem. Soc., 106 (1959) 616–625.Cited pages 94, 547, 556, 565, 696Evans, J. P., Mardon, P. G., “Some physical properties of neptuniummetal-I. A determination of the specific heat of α-neptunium”, J.Phys. Chem. Solids, 10 (1959) 311–313. Cited pages 86, 87, 548,556Gel’man, A. D., Zaitsev, L. M., “Simple and complex plutonium(IV)carbonates”, Russ. J. Inorg. Chem., 4 (1959) 1243–1246.Cited pages 550, 568, 589Krevinskaia, M. E., Nikol’ski, V. D., Pozharskii, B. G., Zastenker,Y. Y., “The properties of nitric acid solutions of the plutonyl ion.I. Hydrolysis of plutonyl nitrate”, Sov. Radiochem., 1 (1959) 238–244. Cited pages 326, 413, 413, 414, 414, 414, 555, 559, 561, 568,589Krevinskaia, M. Y., Nikol’ski, V. D., Pozharskii, B. G., Zastenker,Y. Y., “The preparation and properties of plutonyl nitrate”, Sov. Radiochem.,1 (1959) 253–257. Cited pages 414, 415, 555, 559, 561,568Lee, J. A., Mardon, P. G., Pearce, J. H., Hall, R. O. A., “Somephysical properties of neptunium metal. II. A study of the allotropictransformations in neptunium”, J. Phys. Chem. Solids, 11 (1959)177–181. Cited pages 85, 85, 86, 551, 555, 556, 560Popov, M. M., Gal’chenko, G. L., Senin, M. D., “Specific heats andheats of fusion of UCl 4 and UI 4 and heat of transformation of UI 4 ”,Russ. J. Inorg. Chem., 4 (1959) 560–562. Cited pages 145, 146,550, 561, 563Robinson, R. A., Stokes, R. H., Electrolyte solutions, London: Butterworths,2nd edn., 1959, 559 p. Cited pages 329, 562, 565, 666,706, 730, 767, 784, 803
462 BIBLIOGRAPHY[59SHE/TIM][59STU][59SUL/HIN][59WEI/WEA][59ZIE][60DEN/MOS][60DEN/MOS2][60GRE/NOR][60IHL/AXE][60LIP/POZ]Shevchenko, V. B., Timoshev, V. G., Volkova, A. A., “Stability constantsof nitrate complexes of trivalent plutonium in aqueous andtributyl phosphate solutions”, Sov. J. At. Energy, 6 (1959) 293–296.Cited pages 405, 405, 405, 405, 563, 566, 567, 589Sturtevant, J. M., Technique of organic chemistry, vol. I of Physicalmethods of organic chemistry, chap. “Calorimetry, Chapter X”,New York: Interscience Publ. Inc., 3rd edn., 1959, pp. 523–654.Cited pages 120, 125, 339, 341, 565Sullivan, J. C., Hindman, J. C., “The hydrolysis of neptunium(IV)”,J. Phys. Chem., 63 (1959) 1332–1333. Cited pages xxiii, 111, 111,111, 112, 112, 112, 112, 112, 113, 552, 565, 590, 627, 627Weinstock, B., Weaver, E. E., Malm, J. G., “Vapour pressures ofNpF 6 ,andPuF 6 ; thermodynamic calculations with UF 6 ,NpF 6 ,andPuF 6 ”, J. Inorg. Nucl. Chem., 11 (1959) 104–14. Cited pages 134,138, 139, 139, 140, 352, 352, 352, 556, 567, 567Zielen, A. J., “Thermodynamics of the sulfate complexes ofthorium”, J. Am. Chem. Soc., 81 (1959) 5022–5028. Cited pages568, 616, 661Denotkina, R. G., Moskvin, A. I., Shevchenko, V. B., “The compositionand dissociation constants of phosphate complexes of plutonium(VI)determined by the solubility method”, Russ. J. Inorg.Chem., 5 (1960) 731–734. Cited pages 198, 416, 416, 548, 558,563, 590, 594, 615, 615Denotkina, R. G., Moskvin, A. I., Shevchenko, V. B., “The solubilityproduct of plutonium(IV) hydrogen phosphate and its solubilityin various acids”, Russ. J. Inorg. Chem., 5 (1960) 387–389. Citedpages xxiv, 198, 198, 416, 417, 548, 558, 563, 590, 591, 591, 593,615, 615Grenthe, I., Norén, B., “On the stability of nitrate and chloride complexesof plutonium(IV)”, Acta Chem. Scand., 14 (1960) 2216–2229. Cited pages 380, 380, 381, 381, 381, 382, 383, 407, 408,409, 411, 412, 551, 559, 592, 592, 592, 607Ihle, H. R., Axe, Jr., J. D., “Neubestimmung der Entropie desPlutonylions in wäßriger Lösung”, Z. Elektrochem., 64 (1960)1051, in German. Cited pages 302, 544, 552Lipis, L. V., Pozharskii, B. G., Fomin, V. V., “Spectrophotometricstudy of the complex formation: processes of tetravalent plutoniumin nitric acid solutions”, J. Struct. Chem. USSR, 1 (1960) 135–144.Cited pages 549, 556, 561, 594
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4VOLUMECHEMICALTHERMODYNAMICSCHEMIC
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CHEMICAL THERMODYNAMICSVol. 1. Chem
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Published under the imprint NORTH-H
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viPREFACEviewed several of the othe
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viiiACKNOWLEDGEMENTSand Whiteshell
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xFOREWORDsending comments on the TD
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xiiCONTENTSIII Discussion of neptun
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xivCONTENTS11.1.4.2 Solid neptunium
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CONTENTSxvii20.5.1 PuSb(cr) . . . .
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List of Tables2.1 Symbols and termi
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LIST OF TABLESxxi20.2 Experimental
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List of Figures2.1 Standard order o
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Part IIntroductory material1
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4 1. IntroductionInorganic Complexe
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6 1. Introductionlected, but form a
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Chapter 2Standards, Conventions, an
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2.1 Symbols, terminology and nomenc
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2.2 Units and conversion factors 23
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2.2 Units and conversion factors 25
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2.3 Standard and reference conditio
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2.3 Standard and reference conditio
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2.5 Uncertainty estimates 31Table 2
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2.7 Presentation of the selected da
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2.7 Presentation of the selected da
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Chapter 3Selected neptunium dataThi
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41Table 3.1: Selected thermodynamic
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43Table 3.1: (continued)Compound f
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49Table 3.2: (continued)SpeciesReac
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Chapter 4Selected plutonium dataThi
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61SpeciesPu(OH) 3 (cr)ReactionTable
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Chapter 5Selected auxiliary dataThi
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(footnotes continued)(p) Data from
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79Table 5.2: (continued)Species Rea
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81Table 5.2: (continued)Species Rea
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Chapter 6Elemental neptunium6.1 Nep
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6.1 Neptunium crystal and liquid 87
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6.2 Neptunium ideal monatomic gas 8
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92 7. Neptunium aqua ionsE ◦′ (
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94 7. Neptunium aqua ionsto the sta
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96 7. Neptunium aqua ions(∂ E ◦
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98 7. Neptunium aqua ionsnon-system
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100 7. Neptunium aqua ionsto the re
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102 7. Neptunium aqua ionsTable 7.4
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Chapter 8Neptunium oxygen andhydrog
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8.1 Aqueous neptunium hydroxide com
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8.2 Crystalline and amorphous neptu
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132 9. Neptunium group 17 (halogen)
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178 10. Neptunium group 16 compound
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Chapter 11Neptunium group 15compoun
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11.1 Neptunium nitrogen compounds a
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11.2 Neptunium phosphorus compounds
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11.2 Neptunium phosphorus compounds
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Chapter 12Neptunium group 14compoun
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12.1 Neptunium carbon compounds and
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cal 0.3-1.6 M Na 2 SO 4 25 r H m =
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vlt 0 25 (0.340±0.002) (k) [95OFF/
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sol K + ,CO 2−3 , 20 −(2.31±0.
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sp 0.1 M NaCl 23 (4.68±0.03) [96RU
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dis 0.2 M NaClO 25 2.93 (3.42±1.0)
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sol 1 M NaCl 23 (2.06±0.13) [96RUN
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sol 0.15 M Na 2 CO 3 −(2.58±0.64
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sol 1 M NaClO 30 −(4.0±0.2) [93L
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sol 3 M NaClO 25 −(2.14±0.18)
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(f) Values selected in this review
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(V vs. SHE) (V vs. SHE) (V · K −
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(h) 1MK 2 CO 3 is written in Table
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2 3 r H m (5.0±2.0)log 10 β 2 MO
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290 13. Neptunium group 2 (alkaline
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292 14. Neptunium group 1 (alkali)
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Part IVDiscussion of plutonium data
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298 15. Elemental plutoniumTable 15
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300 15. Elemental plutoniumfrom 298
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302 16. Plutonium aqua ionsthe prop
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304 16. Plutonium aqua ions298.15 K
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306 16. Plutonium aqua ionsE ◦ =
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308 16. Plutonium aqua ionsSm ◦ (
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310 16. Plutonium aqua ionsstandard
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312 16. Plutonium aqua ions r H ◦
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314 16. Plutonium aqua ionsE ◦′
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316 16. Plutonium aqua ionsFigure 1
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318 17. Plutonium oxygen and hydrog
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1:1 pot RT 1 M NaClO 4 −5.71 [49K
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Chapter 18Plutonium group 17 (halog
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18.1 Plutonium halide compounds 347
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18.2 Aqueous plutonium group 17 (ha
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PuO 2+2+ 3F − Å PuO 2 F − (b)3
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390 19. Plutonium group 16 compound
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Chapter 20Plutonium group 15 compou
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20.1 Plutonium nitrogen compounds a
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20.1 Plutonium nitrogen compounds a
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Pu + NO 3Å PuNO 3sp 2 M HClO 4 20
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3 3 3dis, TTA 6 M (? HCl or HClO 4
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Page 453 and 454: 428 21. Plutonium group 14 compound
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Page 474: Chapter 23Plutonium group 1 (alkali
Page 477 and 478: 452 BIBLIOGRAPHY[47GIN/COR][48KRA/N
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Page 481 and 482: 456 BIBLIOGRAPHY[51WES/EYR][51WES/W
Page 483 and 484: 458 BIBLIOGRAPHY[55COH/SUL]Cohen, D
Page 485: 460 BIBLIOGRAPHYmetals in connectio
Page 489 and 490: 464 BIBLIOGRAPHY[61SCH][61STO/FRY][
Page 491 and 492: 466 BIBLIOGRAPHY[63ROB/WAL] Roberts
Page 493 and 494: 468 BIBLIOGRAPHY[64SIL/MAR][65CHO/K
Page 495 and 496: 470 BIBLIOGRAPHY[66DAN/ORL][66FRO/K
Page 497 and 498: 472 BIBLIOGRAPHY[67ERM/STA][67FRL/C
Page 499 and 500: 474 BIBLIOGRAPHY[68KRU/SAV][68KRY/K
Page 501 and 502: 476 BIBLIOGRAPHY[69KEN/LEA][69KRY/K
Page 503 and 504: 478 BIBLIOGRAPHY[70HIN/COB][70KRO/G
Page 505 and 506: 480 BIBLIOGRAPHY[71MOS][71MOS2][71M
Page 507 and 508: 482 BIBLIOGRAPHY[72MET/GUI][72NIK/S
Page 509 and 510: 484 BIBLIOGRAPHY[73PAT/RAM2][73PIT]
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Page 513 and 514: 488 BIBLIOGRAPHY[75OSB/FLO][75PAT/R
Page 515 and 516: 490 BIBLIOGRAPHY298.15 K”, J. Che
Page 517 and 518: 492 BIBLIOGRAPHY[76VOL/VIS][77BAG/R
Page 519 and 520: 494 BIBLIOGRAPHY[78HAL/LEE][78HUR][
Page 521 and 522: 496 BIBLIOGRAPHYof plutonium(IV)”
Page 523 and 524: 498 BIBLIOGRAPHYNa 0.6 NpO 2 (CO 3
Page 525 and 526: 500 BIBLIOGRAPHY[81CHI/AKH][81CIA/F
Page 527 and 528: 502 BIBLIOGRAPHY[81WOO][82ALC/ROB][
Page 529 and 530: 504 BIBLIOGRAPHY[83ALL][83BES/LIN][
Page 531 and 532: 506 BIBLIOGRAPHY[83SCH/GOR]Schmidt,
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Page 535 and 536: 510 BIBLIOGRAPHY[85CÔM][85EIS/KIM]
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512 BIBLIOGRAPHY[85NEW/SUL][85RAI/R
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514 BIBLIOGRAPHY[86FAH][86FRE/KEL]F
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516 BIBLIOGRAPHY[87BEN][87BEN/HOF][
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518 BIBLIOGRAPHY[88HIR/LIE][88ITU][
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520 BIBLIOGRAPHYGeochim. Cosmochim.
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522 BIBLIOGRAPHY[90BEN][90CAP/VIT][
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524 BIBLIOGRAPHY254, 258, 258, 264,
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526 BIBLIOGRAPHY[91MEI][91NIT][91OK
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528 BIBLIOGRAPHYment”, Waste Mana
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530 BIBLIOGRAPHY[93ERI/NDA][93GIF/V
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532 BIBLIOGRAPHY[93TAY/LEM][93WEG/O
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534 BIBLIOGRAPHYpages 222, 223, 226
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536 BIBLIOGRAPHYK, gas-phase infrar
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538 BIBLIOGRAPHY[96ALL/VEI][96CAP/V
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540 BIBLIOGRAPHY[97CAP/VIT][97FEL/R
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542 BIBLIOGRAPHY[99RAI/HES2][99RAR/
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544 LIST OF CITED AUTHORSTable 23.1
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Appendix ADiscussion of selected re
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A. Discussion of selected reference
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5 −10.63±0.11 (g) −12.48±0.23
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dataarein1MNa + media, except as no
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Appendix BIonic strength correction
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B.1 The specific ion interaction eq
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B.2 Ion interaction coefficients ve
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B.3 Tables of ion interaction coeff
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Appendix CAssigned uncertainties
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C.2 Two or more independent source
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C.2 Two or more independent source
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C.3 Several data at different ionic
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C.3 Several data at different ionic
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C.4 Procedures for data handling 83
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C.4 Procedures for data handling 83
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Index837
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INDEX - GENERAL 839standard state p
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INDEX - NEPTUNIUM 841elemental nept
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INDEX - PLUTONIUM 843Index - pluton
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INDEX - PLUTONIUM 845monobismuthide
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