chemical thermodynamics of neptunium and plutonium - U.S. ...

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LIST OF CITED AUTHORS 561Table 23.1: (continued)AuthorPopov, M. M.Portanova, R.Porthault, M.Porto, R.Posokhov, A. K.Potemkina, T. I.Potter, P. E.Pozharskii, B. G.Poznyakov, A. N.Pratopo, M. I.Prins, G.Prussin, T.Pryke, D. C.Puigdomènech, I.Pushlenkov, M. F.Pytkowicz, R. M.Rabideau, S. W.Rabinowitch, E.Rae, H. K.Raghavan, R.Rai, D.Ramakrishna, V. V.Ramanujam, A.Rananiah, M. V.R<strong>and</strong>, M. H.R<strong>and</strong>all, M.Rao, C. L.Rao, L. F.Rao, P. R. V.Rard, J. A.Raspopin, S. P.Rauh, E. G.References[57POP/IVA], [59POP/GAL][72CAS/MAG], [72CAS/MAG2][73MUS/POR][87CIA/IUL][91POS/ROV][89BUD/FED][80POT/SPE], [90COR/KON2][59KRE/NIK], [59KRE/NIK2], [60LIP/POZ], [64POZ/FED][78MOS/POZ], [79MOS/POZ][89MOR/PRA], [89PRA/MOR], [90PRA/MOR], [91PRA/YAM],[91YAM/PRA], [93PRA], [93PRA/MOR], [93PRA/YAM],[95MOR/PRA][90COR/KON2][96ROB/SIL][86PRY/REE][95GRE/PUI], [95SIL/BID], [97PUI/RAR], [98SPA/PUI][68KRY/KOM], [68KRY/KOM2], [69KRY/KOM3],[69KRY/KOM4][79JOH/PYT], [79PYT][51RAB/LEM], [53RAB], [55RAB/COW], [56RAB], [57RAB],[60RAB/KLI], [61RAB/MAS][51KAT/RAB][56MAN/RAE][75RAG/RAM][80RAI/SER], [80RAI/SER2], [81RAI/SWA], [82RAI/RYA],[84RAI], [85KRU/RAI], [85RAI/RYA], [87RAI/SWA],[87RYA/RAI], [89FEL/RAI], [90RAI/FEL], [92RAI/FEL],[95RAI/FEL], [97FEL/RAI], [98RAI/FEL], [99RAI/HES],[99RAI/HES2][73PAT/RAM], [73PAT/RAM2], [75PAT/RAM], [75RAG/RAM],[76BAG/RAM], [76BAG/RAM2], [76PAT/RAM], [77BAG/RAM],[78PAT/RAM], [78RAO/BAG], [78RAO/BAG2], [79KUS/GAN],[81PAT/RAM][79KUS/GAN][78PAT/RAM][62RAN/FOX], [63RAN/KUB], [66MAR/RAN], [66RAN],[76OET/RAN], [80RAN], [81CHI/AKH], [84HOL/RAN],[90COR/KON2], [95GRE/PUI], [95SIL/BID], [99RAR/RAN],[2000RAN/FUG][61LEW/RAN][67NAI/RAO][84CHO/RAO], [91SUL/CHO], [94RIZ/RAO][78RAO/BAG], [78RAO/BAG2], [78RAO/PAT], [79KUS/GAN],[79RAO/GUD][97PUI/RAR], [99RAR/RAN][69LEB/BAB], [84LEB/KOB][66ACK/FAI], [75ACK/RAU](Continued on next page)
562 LIST OF CITED AUTHORSTable 23.1: (continued)AuthorRausch, M. P.Reavis, J. G.Rebizant, J.Reddy, J. F.Reed, D. T.Reedy, G. T.Rees, J. H.Rees, T. F.Richards, R. R.Richter, K.Riglet, C.Riley, B. F.Rizkalla, E. N.Rizvi, G. H.Robbins, J. L.Roberts, K. E.Roberts, L. E. J.Roberts, M. M.Roberts, R. A.Robinson, H. P.Robinson, R. A.Robouch, P.Robouch, P. B.Rolon, C. E.Rossotti, H.Roullet, G.Rovnyi, S. I.Rudolph, G.Rukov, A. G.Runde, W.Russo, R. E.Ryan, J. L.Rykov, A. G.Ryukov, A. G.Rösch, F.Sabau, C. A.Saito, A.Sakamoto, Y.Saltelli, A.Saluja, P. P. S.Salvatore, F.References[75ALE/OGD][59BJO/REA][88BLA/HAL], [94AMA/BRA][79MUE/LAN][90OKA/REE], [91OKA/REE], [93OKA/REE], [93WEG/OKA][78GRE/REE][86PRY/REE][84REE/DAN][85SCH/FRI][87RIC/SAR][86GRE/RIG], [87RIG/VIT], [89RIG/ROB], [90RIG][70RIL][94RIZ/RAO][85SAW/CHA], [85SAW/RIZ][76ALE/CLA][94NEU/HOF], [95NOV/ROB], [96ROB/SIL][63ROB/WAL][82ALC/ROB][86CHO/ROB][49ROB], [49ROB/WES], [49WES/ROB][51ROB/LIM], [59ROB/STO][86GRE/ROB], [87ROB/VIT], [89BRU/GRE], [89RIG/ROB],[89ROB][95SIL/BID][81ROL/GAL][69ROS][71ROU][91POS/ROV][95NEC/FAN][81VOL/VIS], [81VOL/VIS2][92RUN/MEI], [93PAS/RUN], [94NEC/RUN], [94RUN/KIM],[95NEC/RUN], [96CLA/CON2], [96RUN/NEU][92BEN/HOF][82RAI/RYA], [85RAI/RYA], [87RAI/SWA], [87RYA/RAI],[89FEL/RAI], [90RAI/FEL][66RYK/YAK], [71RYK/BLO], [73RYK/BLO], [76FRO/CHI],[76FRO/CHI2], [79VOL/VIS], [79VOL/VIS2], [81VOL/VIS3],[81VOL/VIS4][75VAS/AND], [75VAS/AND2][87RÖS/MIL], [89RÖS/DIT], [90RÖS/HUN][90OKA/REE], [91OKA/REE][75UEN/SAI], [77SAI/UEN], [78SAI/UEN][94YAM/SAK][79SAL/AVO][93LEM/CAM][81CIA/FER], [83FER/GRE], [85FER/GRE](Continued on next page)
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4VOLUMECHEMICALTHERMODYNAMICSCHEMIC
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CHEMICAL THERMODYNAMICSVol. 1. Chem
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Published under the imprint NORTH-H
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viPREFACEviewed several of the othe
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viiiACKNOWLEDGEMENTSand Whiteshell
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xFOREWORDsending comments on the TD
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xiiCONTENTSIII Discussion of neptun
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xivCONTENTS11.1.4.2 Solid neptunium
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CONTENTSxvii20.5.1 PuSb(cr) . . . .
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List of Tables2.1 Symbols and termi
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LIST OF TABLESxxi20.2 Experimental
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List of Figures2.1 Standard order o
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Part IIntroductory material1
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4 1. IntroductionInorganic Complexe
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6 1. Introductionlected, but form a
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Chapter 2Standards, Conventions, an
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2.1 Symbols, terminology and nomenc
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2.2 Units and conversion factors 23
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2.2 Units and conversion factors 25
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2.3 Standard and reference conditio
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2.3 Standard and reference conditio
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2.5 Uncertainty estimates 31Table 2
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2.7 Presentation of the selected da
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2.7 Presentation of the selected da
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Chapter 3Selected neptunium dataThi
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41Table 3.1: Selected thermodynamic
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43Table 3.1: (continued)Compound f
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49Table 3.2: (continued)SpeciesReac
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Chapter 4Selected plutonium dataThi
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61SpeciesPu(OH) 3 (cr)ReactionTable
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Chapter 5Selected auxiliary dataThi
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(footnotes continued)(p) Data from
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79Table 5.2: (continued)Species Rea
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81Table 5.2: (continued)Species Rea
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Chapter 6Elemental neptunium6.1 Nep
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6.1 Neptunium crystal and liquid 87
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6.2 Neptunium ideal monatomic gas 8
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92 7. Neptunium aqua ionsE ◦′ (
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94 7. Neptunium aqua ionsto the sta
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96 7. Neptunium aqua ions(∂ E ◦
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98 7. Neptunium aqua ionsnon-system
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100 7. Neptunium aqua ionsto the re
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102 7. Neptunium aqua ionsTable 7.4
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Chapter 8Neptunium oxygen andhydrog
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8.1 Aqueous neptunium hydroxide com
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8.2 Crystalline and amorphous neptu
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132 9. Neptunium group 17 (halogen)
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178 10. Neptunium group 16 compound
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Chapter 11Neptunium group 15compoun
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11.1 Neptunium nitrogen compounds a
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11.2 Neptunium phosphorus compounds
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11.2 Neptunium phosphorus compounds
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Chapter 12Neptunium group 14compoun
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12.1 Neptunium carbon compounds and
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cal 0.3-1.6 M Na 2 SO 4 25 r H m =
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vlt 0 25 (0.340±0.002) (k) [95OFF/
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sol K + ,CO 2−3 , 20 −(2.31±0.
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sp 0.1 M NaCl 23 (4.68±0.03) [96RU
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dis 0.2 M NaClO 25 2.93 (3.42±1.0)
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sol 1 M NaCl 23 (2.06±0.13) [96RUN
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sol 0.15 M Na 2 CO 3 −(2.58±0.64
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sol 1 M NaClO 30 −(4.0±0.2) [93L
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sol 3 M NaClO 25 −(2.14±0.18)
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(f) Values selected in this review
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(V vs. SHE) (V vs. SHE) (V · K −
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(h) 1MK 2 CO 3 is written in Table
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2 3 r H m (5.0±2.0)log 10 β 2 MO
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290 13. Neptunium group 2 (alkaline
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292 14. Neptunium group 1 (alkali)
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Part IVDiscussion of plutonium data
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298 15. Elemental plutoniumTable 15
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300 15. Elemental plutoniumfrom 298
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302 16. Plutonium aqua ionsthe prop
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304 16. Plutonium aqua ions298.15 K
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306 16. Plutonium aqua ionsE ◦ =
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308 16. Plutonium aqua ionsSm ◦ (
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310 16. Plutonium aqua ionsstandard
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312 16. Plutonium aqua ions r H ◦
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314 16. Plutonium aqua ionsE ◦′
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316 16. Plutonium aqua ionsFigure 1
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318 17. Plutonium oxygen and hydrog
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1:1 pot RT 1 M NaClO 4 −5.71 [49K
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Chapter 18Plutonium group 17 (halog
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18.1 Plutonium halide compounds 347
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18.2 Aqueous plutonium group 17 (ha
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PuO 2+2+ 3F − Å PuO 2 F − (b)3
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390 19. Plutonium group 16 compound
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Chapter 20Plutonium group 15 compou
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20.1 Plutonium nitrogen compounds a
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Pu + NO 3Å PuNO 3sp 2 M HClO 4 20
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3 3 3dis, TTA 6 M (? HCl or HClO 4
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20.2 Plutonium phosphorus compounds
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20.2 Plutonium phosphorus compounds
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20.3 Solid plutonium phosphorus com
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20.4 Plutonium arsenic compounds 42
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20.6 The plutonium-bismuth system 4
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20.6 The plutonium-bismuth system 4
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446 22. Plutonium group 2 (alkaline
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Chapter 23Plutonium group 1 (alkali
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452 BIBLIOGRAPHY[47GIN/COR][48KRA/N
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454 BIBLIOGRAPHY[49MAG/LAC][49ROB][
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456 BIBLIOGRAPHY[51WES/EYR][51WES/W
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458 BIBLIOGRAPHY[55COH/SUL]Cohen, D
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460 BIBLIOGRAPHYmetals in connectio
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462 BIBLIOGRAPHY[59SHE/TIM][59STU][
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464 BIBLIOGRAPHY[61SCH][61STO/FRY][
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466 BIBLIOGRAPHY[63ROB/WAL] Roberts
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468 BIBLIOGRAPHY[64SIL/MAR][65CHO/K
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470 BIBLIOGRAPHY[66DAN/ORL][66FRO/K
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472 BIBLIOGRAPHY[67ERM/STA][67FRL/C
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474 BIBLIOGRAPHY[68KRU/SAV][68KRY/K
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476 BIBLIOGRAPHY[69KEN/LEA][69KRY/K
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478 BIBLIOGRAPHY[70HIN/COB][70KRO/G
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480 BIBLIOGRAPHY[71MOS][71MOS2][71M
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482 BIBLIOGRAPHY[72MET/GUI][72NIK/S
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484 BIBLIOGRAPHY[73PAT/RAM2][73PIT]
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486 BIBLIOGRAPHY[74SAV][74SIM/VOL][
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488 BIBLIOGRAPHY[75OSB/FLO][75PAT/R
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490 BIBLIOGRAPHY298.15 K”, J. Che
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492 BIBLIOGRAPHY[76VOL/VIS][77BAG/R
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494 BIBLIOGRAPHY[78HAL/LEE][78HUR][
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496 BIBLIOGRAPHYof plutonium(IV)”
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498 BIBLIOGRAPHYNa 0.6 NpO 2 (CO 3
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500 BIBLIOGRAPHY[81CHI/AKH][81CIA/F
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502 BIBLIOGRAPHY[81WOO][82ALC/ROB][
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504 BIBLIOGRAPHY[83ALL][83BES/LIN][
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506 BIBLIOGRAPHY[83SCH/GOR]Schmidt,
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508 BIBLIOGRAPHY[84LEM][84LIE/KIM][
Page 535 and 536: 510 BIBLIOGRAPHY[85CÔM][85EIS/KIM]
Page 537 and 538: 512 BIBLIOGRAPHY[85NEW/SUL][85RAI/R
Page 539 and 540: 514 BIBLIOGRAPHY[86FAH][86FRE/KEL]F
Page 541 and 542: 516 BIBLIOGRAPHY[87BEN][87BEN/HOF][
Page 543 and 544: 518 BIBLIOGRAPHY[88HIR/LIE][88ITU][
Page 545 and 546: 520 BIBLIOGRAPHYGeochim. Cosmochim.
Page 547 and 548: 522 BIBLIOGRAPHY[90BEN][90CAP/VIT][
Page 549 and 550: 524 BIBLIOGRAPHY254, 258, 258, 264,
Page 551 and 552: 526 BIBLIOGRAPHY[91MEI][91NIT][91OK
Page 553 and 554: 528 BIBLIOGRAPHYment”, Waste Mana
Page 555 and 556: 530 BIBLIOGRAPHY[93ERI/NDA][93GIF/V
Page 557 and 558: 532 BIBLIOGRAPHY[93TAY/LEM][93WEG/O
Page 559 and 560: 534 BIBLIOGRAPHYpages 222, 223, 226
Page 561 and 562: 536 BIBLIOGRAPHYK, gas-phase infrar
Page 563 and 564: 538 BIBLIOGRAPHY[96ALL/VEI][96CAP/V
Page 565 and 566: 540 BIBLIOGRAPHY[97CAP/VIT][97FEL/R
Page 567 and 568: 542 BIBLIOGRAPHY[99RAI/HES2][99RAR/
Page 569 and 570: 544 LIST OF CITED AUTHORSTable 23.1
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Page 596 and 597: Appendix ADiscussion of selected re
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A. Discussion of selected reference
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5 −10.63±0.11 (g) −12.48±0.23
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dataarein1MNa + media, except as no
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Appendix BIonic strength correction
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B.1 The specific ion interaction eq
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B.2 Ion interaction coefficients ve
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B.3 Tables of ion interaction coeff
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Appendix CAssigned uncertainties
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C.2 Two or more independent source
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C.2 Two or more independent source
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C.3 Several data at different ionic
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C.3 Several data at different ionic
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C.4 Procedures for data handling 83
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C.4 Procedures for data handling 83
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Index837
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INDEX - GENERAL 839standard state p
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INDEX - NEPTUNIUM 841elemental nept
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INDEX - PLUTONIUM 843Index - pluton
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INDEX - PLUTONIUM 845monobismuthide
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