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BIBLIOGRAPHY 493[77MUS/MAR] Musikas, C., Marteau, M., “Complexes thiocyaniques du neptunium(V)en milieu aqueux”, Radiochem. Radioanal. Lett., 30(1977) 271–280. Cited pages 286, 286, 286, 287, 287, 287, 287,287, 557, 558, 665[77MYE/GRA] Myers, C. E., Graves, D. T., “Vaporization thermodynamics oflanthanide trihalides”, J. Chem. Eng. Data, 22 (1977) 440–445.Cited pages 370, 550, 558[77SAI/UEN] Saito, A., Ueno, K., “The precipitation of some actinide elementcomplex ions by using hexammine cobalt(III) cation: V. Absorptionspectra and the precipitation of Np(IV), (V) and (VI) carbonatecomplex ions”, J. Inorg. Nucl. Chem., 39 (1977) 315–318. Citedpages 235, 235, 235, 254, 282, 282, 562, 566, 631, 666, 688, 765,784[77SIM] Simakin, G. A., “Real oxidation potentials of the couples AmO 2+2 -AmO + 2 ,NpO2+ 2 -NpO+ 2in solutions of potassium and sodium carbonates”,Sov. Radiochem., 19 (1977) 424–426. Cited pages 204,207, 207, 207, 207, 207, 207, 207, 207, 208, 208, 212, 212, 214,214, 214, 220, 220, 235, 273, 277, 279, 279, 564, 608, 632, 650,655, 655, 656, 656, 656, 656, 657, 668, 669, 670, 671, 671, 671,671, 671, 671, 688, 692, 700, 708, 744, 747, 761, 765, 781[77VOL/VIS] Volkov, Y. F., Visyashcheva, G. I., Kapshukov, I. I., “Study ofcarbonate compounds of pentavalent actinides with alkali metalcations: V. Production and identification of hydrate forms ofsodium monocarbonatoneptunylate”, Sov. Radiochem., 19 (1977)263–266. Cited pages 276, 553, 567, 567, 671, 682, 683, 688, 761,774[77WEI/WIS] Weigel, F., Wishnevsky, V., Hauske, H., “The vapor phase hydrolysisof PuCl 3 and CmCl 3 : heats of formation of PuOCl andCmOCl”, J. Less-Common Met., 56 (1977) 113–123. Cited pages360, 360, 551, 567, 568[78BED/FID] Bednarczyk, L., Fidelis, I., “Determination of stability constants ofU(VI), Np(VI) and Pu(VI) with chloride ions by extraction chromatography”,J. Radioanal. Chem., 45 (1978) 325–330. Cited pages169, 170, 171, 171, 384, 384, 544, 549, 672, 672, 672, 672[78DRO/SER] Drobyshevskii, Y. V., Serik, V. F., Sokolov, V. B., Tul’skii, M. N.,“Synthesis and certain properties of NpOF 4 and NpF 5 ”, Sov. Radiochem.,20 (1978) 200–204. Cited pages 137, 137, 548, 563,564, 566[78GRE/REE] Green, D. W., Reedy, G. T., “Infra-red spectra of matrix isolatedplutonium nitrides”, J. Chem. Phys., 69 (1978) 552–555. Citedpages 404, 550, 562
494 BIBLIOGRAPHY[78HAL/LEE][78HUR][78LLO/HAI][78MOS/POZ][78MUS][78MUS/MAR][78MUS/MAR2][78OET][78PAT/RAM][78PIT/PET]Hall, R. O. A., Lee, J. A., Martin, D. J., Mortimer, M. J., Sutcliffe,P. W., “Heat capacity of plutonium nitride at low temperatures”, J.Chem. Thermodyn., 10 (1978) 935–940. Cited pages 401, 401,402, 403, 551, 555, 557, 558, 565Hurtgen, C., Preparative thermodynamic and spectral studies onlanthanide and actinide halides, oxyhalides, and halogenocomplexes,Ph.D. thesis, University of Liège, Belgium, 1978. Citedpages 151, 155, 552Lloyd, M. H., Haire, R. G., “The chemistry of plutonium in sol-gelprocesses”, Radiochim. Acta, 25 (1978) 139–148. Cited pages 342,551, 556Moskvin, A. I., Poznyakov, A. N., “Investigation of the complexformation of Neptunium(V) and Plutonium(V) in aqueous solutionsby the coprecipitation method”, Sov. J. Coord. Chem., 4 (1978)811–819. Cited pages xxi, 177, 177, 178, 178, 558, 561, 672,680, 680, 680, 680Musikas, C., Contribution à la chimie de coordination des ions 5fpenta, hexa et heptavalents, Ph.D. thesis, Université de Paris-Sud,Orsay, France, 1978, 142 p., in French. Also published as CEA-R-4901, Commisariat à l’énergie atomique, France. Cited pages 123,126, 558, 672, 719, 728Musikas, C., Marteau, M., “Complexes cyanures du neptunium(V)en solutions aqueuses”, Radiochem. Radioanal. Lett., 33 (1978) 41–52, in French. Cited pages 283, 557, 558, 665, 672Musikas, G., Marteau, M., “Complex ions of neptunium(V) withnitrogen-containing ligands”, Sov. Radiochem., 20 (1978) 213–216.Cited pages 189, 189, 557, 558, 665Oetting, F. L., “The chemical thermodynamic properties of nuclearmaterials: III. Plutonium mononitride”, J. Chem. Thermodyn., 10(1978) 941–948. Cited pages 188, 402, 403, 559Patil, S. K., Ramakrishna, V. V., Rananiah, M. V., “Aqueous coordinationcomplexes of neptunium”, Coord. Chem. Rev., 25 (1978)133–171. Cited pages 172, 173, 174, 174, 174, 174, 192, 482, 483,560, 561, 561, 617, 627Pitzer, K. S., Peterson, J. R., Silvester, L. F., “Thermodynamics ofelectrolytes: IX. Rare earth chlorides, nitrates, and perchlorates”, J.Solution Chem., 7 (1978) 45–56. Cited pages 560, 560, 564, 802
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4VOLUMECHEMICALTHERMODYNAMICSCHEMIC
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CHEMICAL THERMODYNAMICSVol. 1. Chem
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Published under the imprint NORTH-H
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viPREFACEviewed several of the othe
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viiiACKNOWLEDGEMENTSand Whiteshell
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xFOREWORDsending comments on the TD
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xiiCONTENTSIII Discussion of neptun
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xivCONTENTS11.1.4.2 Solid neptunium
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CONTENTSxvii20.5.1 PuSb(cr) . . . .
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List of Tables2.1 Symbols and termi
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LIST OF TABLESxxi20.2 Experimental
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List of Figures2.1 Standard order o
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Part IIntroductory material1
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4 1. IntroductionInorganic Complexe
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6 1. Introductionlected, but form a
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Chapter 2Standards, Conventions, an
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2.1 Symbols, terminology and nomenc
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2.2 Units and conversion factors 23
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2.2 Units and conversion factors 25
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2.3 Standard and reference conditio
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2.3 Standard and reference conditio
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2.5 Uncertainty estimates 31Table 2
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2.7 Presentation of the selected da
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2.7 Presentation of the selected da
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Chapter 3Selected neptunium dataThi
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41Table 3.1: Selected thermodynamic
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43Table 3.1: (continued)Compound f
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49Table 3.2: (continued)SpeciesReac
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Chapter 4Selected plutonium dataThi
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61SpeciesPu(OH) 3 (cr)ReactionTable
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Chapter 5Selected auxiliary dataThi
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(footnotes continued)(p) Data from
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79Table 5.2: (continued)Species Rea
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81Table 5.2: (continued)Species Rea
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Chapter 6Elemental neptunium6.1 Nep
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6.1 Neptunium crystal and liquid 87
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6.2 Neptunium ideal monatomic gas 8
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92 7. Neptunium aqua ionsE ◦′ (
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94 7. Neptunium aqua ionsto the sta
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96 7. Neptunium aqua ions(∂ E ◦
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98 7. Neptunium aqua ionsnon-system
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100 7. Neptunium aqua ionsto the re
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102 7. Neptunium aqua ionsTable 7.4
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Chapter 8Neptunium oxygen andhydrog
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8.1 Aqueous neptunium hydroxide com
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8.2 Crystalline and amorphous neptu
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132 9. Neptunium group 17 (halogen)
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178 10. Neptunium group 16 compound
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Chapter 11Neptunium group 15compoun
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11.1 Neptunium nitrogen compounds a
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11.2 Neptunium phosphorus compounds
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11.2 Neptunium phosphorus compounds
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Chapter 12Neptunium group 14compoun
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12.1 Neptunium carbon compounds and
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cal 0.3-1.6 M Na 2 SO 4 25 r H m =
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vlt 0 25 (0.340±0.002) (k) [95OFF/
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sol K + ,CO 2−3 , 20 −(2.31±0.
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sp 0.1 M NaCl 23 (4.68±0.03) [96RU
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dis 0.2 M NaClO 25 2.93 (3.42±1.0)
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sol 1 M NaCl 23 (2.06±0.13) [96RUN
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sol 0.15 M Na 2 CO 3 −(2.58±0.64
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sol 1 M NaClO 30 −(4.0±0.2) [93L
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sol 3 M NaClO 25 −(2.14±0.18)
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(f) Values selected in this review
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(V vs. SHE) (V vs. SHE) (V · K −
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(h) 1MK 2 CO 3 is written in Table
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2 3 r H m (5.0±2.0)log 10 β 2 MO
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290 13. Neptunium group 2 (alkaline
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292 14. Neptunium group 1 (alkali)
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Part IVDiscussion of plutonium data
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298 15. Elemental plutoniumTable 15
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300 15. Elemental plutoniumfrom 298
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302 16. Plutonium aqua ionsthe prop
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304 16. Plutonium aqua ions298.15 K
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306 16. Plutonium aqua ionsE ◦ =
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308 16. Plutonium aqua ionsSm ◦ (
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310 16. Plutonium aqua ionsstandard
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312 16. Plutonium aqua ions r H ◦
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314 16. Plutonium aqua ionsE ◦′
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316 16. Plutonium aqua ionsFigure 1
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318 17. Plutonium oxygen and hydrog
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1:1 pot RT 1 M NaClO 4 −5.71 [49K
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Chapter 18Plutonium group 17 (halog
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18.1 Plutonium halide compounds 347
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18.2 Aqueous plutonium group 17 (ha
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PuO 2+2+ 3F − Å PuO 2 F − (b)3
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390 19. Plutonium group 16 compound
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Chapter 20Plutonium group 15 compou
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20.1 Plutonium nitrogen compounds a
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Pu + NO 3Å PuNO 3sp 2 M HClO 4 20
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3 3 3dis, TTA 6 M (? HCl or HClO 4
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20.2 Plutonium phosphorus compounds
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20.2 Plutonium phosphorus compounds
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20.3 Solid plutonium phosphorus com
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20.4 Plutonium arsenic compounds 42
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20.6 The plutonium-bismuth system 4
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20.6 The plutonium-bismuth system 4
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Page 467 and 468: 442 21. Plutonium group 14 compound
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Page 474: Chapter 23Plutonium group 1 (alkali
Page 477 and 478: 452 BIBLIOGRAPHY[47GIN/COR][48KRA/N
Page 479 and 480: 454 BIBLIOGRAPHY[49MAG/LAC][49ROB][
Page 481 and 482: 456 BIBLIOGRAPHY[51WES/EYR][51WES/W
Page 483 and 484: 458 BIBLIOGRAPHY[55COH/SUL]Cohen, D
Page 485 and 486: 460 BIBLIOGRAPHYmetals in connectio
Page 487 and 488: 462 BIBLIOGRAPHY[59SHE/TIM][59STU][
Page 489 and 490: 464 BIBLIOGRAPHY[61SCH][61STO/FRY][
Page 491 and 492: 466 BIBLIOGRAPHY[63ROB/WAL] Roberts
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Page 507 and 508: 482 BIBLIOGRAPHY[72MET/GUI][72NIK/S
Page 509 and 510: 484 BIBLIOGRAPHY[73PAT/RAM2][73PIT]
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Page 513 and 514: 488 BIBLIOGRAPHY[75OSB/FLO][75PAT/R
Page 515 and 516: 490 BIBLIOGRAPHY298.15 K”, J. Che
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Page 521 and 522: 496 BIBLIOGRAPHYof plutonium(IV)”
Page 523 and 524: 498 BIBLIOGRAPHYNa 0.6 NpO 2 (CO 3
Page 525 and 526: 500 BIBLIOGRAPHY[81CHI/AKH][81CIA/F
Page 527 and 528: 502 BIBLIOGRAPHY[81WOO][82ALC/ROB][
Page 529 and 530: 504 BIBLIOGRAPHY[83ALL][83BES/LIN][
Page 531 and 532: 506 BIBLIOGRAPHY[83SCH/GOR]Schmidt,
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Page 535 and 536: 510 BIBLIOGRAPHY[85CÔM][85EIS/KIM]
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Page 545 and 546: 520 BIBLIOGRAPHYGeochim. Cosmochim.
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Page 549 and 550: 524 BIBLIOGRAPHY254, 258, 258, 264,
Page 551 and 552: 526 BIBLIOGRAPHY[91MEI][91NIT][91OK
Page 553 and 554: 528 BIBLIOGRAPHYment”, Waste Mana
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Page 557 and 558: 532 BIBLIOGRAPHY[93TAY/LEM][93WEG/O
Page 559 and 560: 534 BIBLIOGRAPHYpages 222, 223, 226
Page 561 and 562: 536 BIBLIOGRAPHYK, gas-phase infrar
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Page 565 and 566: 540 BIBLIOGRAPHY[97CAP/VIT][97FEL/R
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544 LIST OF CITED AUTHORSTable 23.1
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Appendix ADiscussion of selected re
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A. Discussion of selected reference
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5 −10.63±0.11 (g) −12.48±0.23
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dataarein1MNa + media, except as no
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Appendix BIonic strength correction
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B.1 The specific ion interaction eq
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B.2 Ion interaction coefficients ve
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B.3 Tables of ion interaction coeff
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Appendix CAssigned uncertainties
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C.2 Two or more independent source
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C.2 Two or more independent source
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C.3 Several data at different ionic
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C.3 Several data at different ionic
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C.4 Procedures for data handling 83
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C.4 Procedures for data handling 83
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Index837
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INDEX - GENERAL 839standard state p
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INDEX - NEPTUNIUM 841elemental nept
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INDEX - PLUTONIUM 843Index - pluton
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INDEX - PLUTONIUM 845monobismuthide
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