chemical thermodynamics of neptunium and plutonium - U.S. ...

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BIBLIOGRAPHY 463[60RAB/KLI][61BEN/DOU][61BER/GAU][61ELL][61ELL/CRA][61GOL/GOL][61JOH/FIS][61LEW/RAN][61MAN/DAV][61MAR/CHM][61PAU/GAL][61RAB/MAS]Rabideau, S. W., Kline, R. J., “A spectrophotometric study of thehydrolysis of plutonium(IV)”, J. Phys. Chem., 64 (1960) 680–682.Cited pages 322, 322, 322, 322, 322, 323, 325, 329, 329, 554, 561,578, 587, 595Benz, R., Douglass, R. M., “Phase equilibria in the binary systemsPuCl 3 -RbCl and PuCl 3 -CsCl”, J. Phys. Chem., 65 (1961) 1461–1463. Cited pages 362, 367, 544, 548Berger, R., Gaumann, T., “Die Sublimation von Plutoniumtetrafluorid”,Helv. Chim. Acta, 44 (1961) 1084–1088. Cited pages 351,544, 550Ellinger, F. H., The Metal Plutonium, chap. “XXV. A review ofthe intermetallic compounds of plutonium”, University of ChicagoPress, 1961, p. 287. Cited pages 423, 548Elliot, R. O., Cramer, E. M., 1961, cited by [68ELL/MIN]. Citedpages 425, 547, 548Golub, A. M., Golodets, G. I., “Iodide complexes of lead in nonaqueoussolvents”, Ukr. Khim. Zh. (Russ. Ed.), 27 (1961) 141–146,in Russian, Chem. Abstr. 55 (1961): 23150i. Cited pages 407, 408,409, 410, 550, 550Johnson, C. E., Fischer, J., Steindler, M. J., “Reactions of sulfurtetrafluorides with oxides, oxyfluorides, and fluorides of uraniumand plutonium”, J. Am. Chem. Soc., 83 (1961) 1620–2. Cited pages349, 549, 553, 564Lewis, G. N., Randall, M., Thermodynamics, as revised by Pitzer,K. S. and Brewer, L., New York: McGraw-Hill, 2nd edn., 1961, 723p. Cited pages 556, 561, 800, 802, 803, 805Mandleberg, C. J., Davies, D., “The vapour pressure of plutoniumtetrafluoride”, J. Chem. Soc. (1961) 2031–7. Cited pages 351, 351,547, 556Marov, I. N., Chmutova, M. K., “Cation-exchange studies of complexformation by Pu IV and the sulfate ion”, Russ. J. Inorg. Chem.,6 (1961) 1340–1345. Cited pages 391, 393, 393, 546, 556, 595Paul, A. D., Gallo, L. S., VanCamp, J. B., “The fluoride complexingof yttrium(III) in aqueous solution”, J. Phys. Chem., 65 (1961) 441–443. Cited pages 550, 560, 566, 769Rabideau, S. W., Masters, B. J., “Kinetics of the reaction betweenPu(VI) and Sn(II) in chloride perchlorate solution”, J. Phys. Chem.,65 (1961) 1256–1261. Cited pages 384, 384, 385, 385, 385, 385,557, 561, 586, 595, 595, 596, 596, 596
464 BIBLIOGRAPHY[61SCH][61STO/FRY][61SUL/HIN][61TRE/SHI][62BAE/MEY]Schonfeld, F. W., XXII. Plutonium phase diagrams studied at LosAlamos, in: The metal plutonium, University of Chicago Press,1961, pp. 240–254, Coffinberry, A. S. and Miner, W. N., editors.Cited pages 425, 563Stoughton, R. W., Fry, A. J., Barney, J. E., “A study of thoriumiodate complexing in aqueous solutions”, J. Inorg. Nucl. Chem., 19(1961) 286–297. Cited pages 174, 544, 549, 565Sullivan, J. C., Hindman, J. C., Zielen, A. J., “Specific interactionbetween Np(V) and U(VI) in aqueous perchloric acid media”, J.Am. Chem. Soc., 83 (1961) 3373–3378. Cited pages 93, 94, 94, 95,95, 552, 565, 568, 580, 596, 626, 725Trevorrow, L. E., Shinn, W. A., Steunenberg, R. K., “The thermaldecomposition of plutonium hexafluoride”, J. Phys. Chem., 65(1961) 398–402. Cited pages 353, 353, 564, 565, 566Baes, Jr., C. F., Meyer, N. J., “Acidity measurements at elevatedtemperatures: I. Uranium(VI) hydrolysis at 25 and 94 ◦ C”, Inorg.Chem., 1 (1962) 780–789. Cited pages 544, 557, 766[62BEN] Benz, R., “Thermodynamics of PuCl 4 from transpiration data”, J.Inorg. Nucl. Chem., 24 (1962) 1191–1195. Cited pages 358, 359,359, 544[62DAV] Davies, C. W., Ion association, London: Butterworths, 1962, 190p. Cited pages 547, 800[62GEL/MOS][62GRØ/WES][62MOS/ZAI][62RAN/FOX]Gel’man, A. D., Moskvin, A. I., Zaitseva, V. P., “Carbonate compoundsof plutonyl”, Sov. Radiochem., 4 (1962) 138–145. Citedpages 431, 432, 442, 550, 558, 568, 596, 615Grønvold, F., Westrum, Jr., E. F., “Heat capacities and thermodynamicfunctions or iron disulphide (pyrite), iron diselinide, andnickel diselinide from 5 to 350 K: The estimation of standard entropiesof transition metal chalcogenides”, Inorg. Chem., 1 (1962)36–48. Cited pages 423, 551, 567Moskvin, A. I., Zaitseva, V. P., “Hydrolytic behavior of plutonyl inaqueous solution”, Sov. Radiochem., 4 (1962) 63–70. Cited pages317, 319, 320, 326, 338, 338, 558, 568, 597Rand, M. H., Fox, A. C., Street, R. S., “Radiation self-damagein plutonium compounds”, Nature (London), 195 (1962) 567–568.Cited pages 404, 549, 561, 565
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4VOLUMECHEMICALTHERMODYNAMICSCHEMIC
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CHEMICAL THERMODYNAMICSVol. 1. Chem
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Published under the imprint NORTH-H
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viPREFACEviewed several of the othe
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viiiACKNOWLEDGEMENTSand Whiteshell
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xFOREWORDsending comments on the TD
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xiiCONTENTSIII Discussion of neptun
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xivCONTENTS11.1.4.2 Solid neptunium
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CONTENTSxvii20.5.1 PuSb(cr) . . . .
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List of Tables2.1 Symbols and termi
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LIST OF TABLESxxi20.2 Experimental
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List of Figures2.1 Standard order o
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Part IIntroductory material1
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4 1. IntroductionInorganic Complexe
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6 1. Introductionlected, but form a
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Chapter 2Standards, Conventions, an
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2.1 Symbols, terminology and nomenc
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2.2 Units and conversion factors 23
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2.2 Units and conversion factors 25
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2.3 Standard and reference conditio
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2.3 Standard and reference conditio
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2.5 Uncertainty estimates 31Table 2
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2.7 Presentation of the selected da
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2.7 Presentation of the selected da
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Chapter 3Selected neptunium dataThi
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41Table 3.1: Selected thermodynamic
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43Table 3.1: (continued)Compound f
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49Table 3.2: (continued)SpeciesReac
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Chapter 4Selected plutonium dataThi
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61SpeciesPu(OH) 3 (cr)ReactionTable
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Chapter 5Selected auxiliary dataThi
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(footnotes continued)(p) Data from
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79Table 5.2: (continued)Species Rea
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81Table 5.2: (continued)Species Rea
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Chapter 6Elemental neptunium6.1 Nep
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6.1 Neptunium crystal and liquid 87
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6.2 Neptunium ideal monatomic gas 8
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92 7. Neptunium aqua ionsE ◦′ (
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94 7. Neptunium aqua ionsto the sta
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96 7. Neptunium aqua ions(∂ E ◦
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98 7. Neptunium aqua ionsnon-system
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100 7. Neptunium aqua ionsto the re
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102 7. Neptunium aqua ionsTable 7.4
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Chapter 8Neptunium oxygen andhydrog
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8.1 Aqueous neptunium hydroxide com
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8.2 Crystalline and amorphous neptu
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132 9. Neptunium group 17 (halogen)
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178 10. Neptunium group 16 compound
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Chapter 11Neptunium group 15compoun
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11.1 Neptunium nitrogen compounds a
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11.2 Neptunium phosphorus compounds
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11.2 Neptunium phosphorus compounds
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Chapter 12Neptunium group 14compoun
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12.1 Neptunium carbon compounds and
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cal 0.3-1.6 M Na 2 SO 4 25 r H m =
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vlt 0 25 (0.340±0.002) (k) [95OFF/
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sol K + ,CO 2−3 , 20 −(2.31±0.
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sp 0.1 M NaCl 23 (4.68±0.03) [96RU
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dis 0.2 M NaClO 25 2.93 (3.42±1.0)
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sol 1 M NaCl 23 (2.06±0.13) [96RUN
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sol 0.15 M Na 2 CO 3 −(2.58±0.64
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sol 1 M NaClO 30 −(4.0±0.2) [93L
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sol 3 M NaClO 25 −(2.14±0.18)
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(f) Values selected in this review
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(V vs. SHE) (V vs. SHE) (V · K −
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(h) 1MK 2 CO 3 is written in Table
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2 3 r H m (5.0±2.0)log 10 β 2 MO
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290 13. Neptunium group 2 (alkaline
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292 14. Neptunium group 1 (alkali)
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Part IVDiscussion of plutonium data
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298 15. Elemental plutoniumTable 15
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300 15. Elemental plutoniumfrom 298
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302 16. Plutonium aqua ionsthe prop
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304 16. Plutonium aqua ions298.15 K
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306 16. Plutonium aqua ionsE ◦ =
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308 16. Plutonium aqua ionsSm ◦ (
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310 16. Plutonium aqua ionsstandard
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312 16. Plutonium aqua ions r H ◦
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314 16. Plutonium aqua ionsE ◦′
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316 16. Plutonium aqua ionsFigure 1
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318 17. Plutonium oxygen and hydrog
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1:1 pot RT 1 M NaClO 4 −5.71 [49K
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Chapter 18Plutonium group 17 (halog
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18.1 Plutonium halide compounds 347
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18.2 Aqueous plutonium group 17 (ha
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PuO 2+2+ 3F − Å PuO 2 F − (b)3
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390 19. Plutonium group 16 compound
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Chapter 20Plutonium group 15 compou
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20.1 Plutonium nitrogen compounds a
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Pu + NO 3Å PuNO 3sp 2 M HClO 4 20
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3 3 3dis, TTA 6 M (? HCl or HClO 4
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Page 453 and 454: 428 21. Plutonium group 14 compound
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Page 477 and 478: 452 BIBLIOGRAPHY[47GIN/COR][48KRA/N
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Page 481 and 482: 456 BIBLIOGRAPHY[51WES/EYR][51WES/W
Page 483 and 484: 458 BIBLIOGRAPHY[55COH/SUL]Cohen, D
Page 485 and 486: 460 BIBLIOGRAPHYmetals in connectio
Page 487: 462 BIBLIOGRAPHY[59SHE/TIM][59STU][
Page 491 and 492: 466 BIBLIOGRAPHY[63ROB/WAL] Roberts
Page 493 and 494: 468 BIBLIOGRAPHY[64SIL/MAR][65CHO/K
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Page 497 and 498: 472 BIBLIOGRAPHY[67ERM/STA][67FRL/C
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Page 501 and 502: 476 BIBLIOGRAPHY[69KEN/LEA][69KRY/K
Page 503 and 504: 478 BIBLIOGRAPHY[70HIN/COB][70KRO/G
Page 505 and 506: 480 BIBLIOGRAPHY[71MOS][71MOS2][71M
Page 507 and 508: 482 BIBLIOGRAPHY[72MET/GUI][72NIK/S
Page 509 and 510: 484 BIBLIOGRAPHY[73PAT/RAM2][73PIT]
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Page 513 and 514: 488 BIBLIOGRAPHY[75OSB/FLO][75PAT/R
Page 515 and 516: 490 BIBLIOGRAPHY298.15 K”, J. Che
Page 517 and 518: 492 BIBLIOGRAPHY[76VOL/VIS][77BAG/R
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Page 521 and 522: 496 BIBLIOGRAPHYof plutonium(IV)”
Page 523 and 524: 498 BIBLIOGRAPHYNa 0.6 NpO 2 (CO 3
Page 525 and 526: 500 BIBLIOGRAPHY[81CHI/AKH][81CIA/F
Page 527 and 528: 502 BIBLIOGRAPHY[81WOO][82ALC/ROB][
Page 529 and 530: 504 BIBLIOGRAPHY[83ALL][83BES/LIN][
Page 531 and 532: 506 BIBLIOGRAPHY[83SCH/GOR]Schmidt,
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Page 535 and 536: 510 BIBLIOGRAPHY[85CÔM][85EIS/KIM]
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514 BIBLIOGRAPHY[86FAH][86FRE/KEL]F
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516 BIBLIOGRAPHY[87BEN][87BEN/HOF][
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518 BIBLIOGRAPHY[88HIR/LIE][88ITU][
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520 BIBLIOGRAPHYGeochim. Cosmochim.
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522 BIBLIOGRAPHY[90BEN][90CAP/VIT][
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524 BIBLIOGRAPHY254, 258, 258, 264,
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526 BIBLIOGRAPHY[91MEI][91NIT][91OK
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528 BIBLIOGRAPHYment”, Waste Mana
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530 BIBLIOGRAPHY[93ERI/NDA][93GIF/V
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532 BIBLIOGRAPHY[93TAY/LEM][93WEG/O
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534 BIBLIOGRAPHYpages 222, 223, 226
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536 BIBLIOGRAPHYK, gas-phase infrar
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538 BIBLIOGRAPHY[96ALL/VEI][96CAP/V
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540 BIBLIOGRAPHY[97CAP/VIT][97FEL/R
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542 BIBLIOGRAPHY[99RAI/HES2][99RAR/
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544 LIST OF CITED AUTHORSTable 23.1
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Appendix ADiscussion of selected re
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A. Discussion of selected reference
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5 −10.63±0.11 (g) −12.48±0.23
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dataarein1MNa + media, except as no
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Appendix BIonic strength correction
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B.1 The specific ion interaction eq
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B.2 Ion interaction coefficients ve
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B.3 Tables of ion interaction coeff
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Appendix CAssigned uncertainties
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C.2 Two or more independent source
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C.2 Two or more independent source
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C.3 Several data at different ionic
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C.3 Several data at different ionic
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C.4 Procedures for data handling 83
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C.4 Procedures for data handling 83
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Index837
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INDEX - GENERAL 839standard state p
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INDEX - NEPTUNIUM 841elemental nept
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INDEX - PLUTONIUM 843Index - pluton
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INDEX - PLUTONIUM 845monobismuthide
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