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Ïðåîáëàäàþùèìè ïðè ïèëëàðèðîâàíèè ñòàíîâÿòñÿ ìåçîïîðû ñ ðàäèóñîì 5-8 íì. Äàííûå ÐÔÀ ïîêàçàëè, ÷òî â ñëó÷àå Ìå 1 -ÌÌ êàòèîíû âûçûâàþò ðàçäâèæåíèå ñëîåâ íà 0,5 íì (îò 1,26 äî 1,76 íì). Äëÿ Ìå 2 -ÌÌ íàðÿäó ñ êðèñòàëëè÷åñêîé ôàçîé ôèêñèðóåòñÿ ïîÿâëåíèå àìîðôíîé ôàçû. Äàííûå ïî àêòèâíîñòè ñøèòîãî ìîíòìîðèëëîíèòà â êðåêèíãå ÊÃÔ è ÂÃ ïðèâåäåíû â òàáëèöàõ 1 è 2. Òàáëèöà 1. Êðåêèíã ÊÃÔ Ìå 1 -ÌÌ è Ìå 2 -ÌÌ ïðè 450 î Ñ Îáðàçåö Ìå 1 -ÌÌ Ìå 2 -ÌÌ Ïðîäóêòû êðåêèíãà, % Ãàç Áåíçèíîâàÿ ôðàêöèÿ (í.ê.-205 î Ñ) Òÿæåëûé îñòàòîê (> 205 î Ñ) Êîêñ Ïîòåðè Áåç ó÷åòà Ñ 5+ 14,3 67,0 15,0 1,7 2,0 Ñ ó÷åòîì Ñ 5+ 12,0 69,3 15,0 1,7 2,0 Áåç ó÷åòà Ñ 5+ 8,3 57,3 29,3 3,0 2,1 Ñ ó÷åòîì Ñ 5+ 11,1 60,1 29,3 3,0 2,1 Èòîãî 100 100 Êîíâåðñèÿ, % 83,0 68,6 Îêòàíîâîå ÷èñëî 80 79 Èç äàííûõ òàáëèöû 1 ñëåäóåò, ÷òî ñøèòûå ÌÌ îáëàäàþò çíà÷èòåëüíîé àêòèâíîñòüþ â êðåêèíãå ÊÃÔ, îñîáåííî â ñëó÷àå Ìå 1 -ÌÌ. Âûõîä áåíçèíîâîé ôðàêöèè ñîñòàâëÿåò 69,3 % (ñ ó÷åòîì Ñ 5+ ) Òàáëèöà 2. Êðåêèíã ÂÃ íà Ìå 1 -ÌÌ è Ìå 2 -ÌÌ ïðè 480 î Ñ Îáðàçåö Al-ÏÌ Zr-ÏÌ Ïðîäóêòû êðåêèíãà, Áåç ó÷åòà Ñ ó÷åòîì Áåç ó÷åòà Ñ ó÷åòîì % Ñ 5+ Ñ 5+ Ñ 5+ Ñ 5+ Ãàç 18,2 15,8 14,1 11,0 Áåíçèíîâàÿ ôðàêöèÿ 36,4 38,8 33,1 36,2 (í. ê. –205 î Ñ) Ëåãêèé ãàçîéëü 27,8 27,8 33,3 33,3 (205-350 î Ñ) Òÿæåëûé îñòàòîê 12,0 12,0 12,8 12,8 (>350 î Ñ) Êîêñ 3,6 3,6 4,8 4,8 75
Îáðàçåö Al-ÏÌ Zr-ÏÌ Ïîòåðè 2,0 2,0 1,9 1,9 Èòîãî 100 100 Êîíâåðñèÿ, % 58,2 52,0 Îêòàíîâîå ÷èñëî 83 82 Â êðåêèíãå ÂÃ ñèíòåçèðîâàííûå îáðàçöû ïîêàçàëè áëèçêèå àêòèâíîñòè. Ñäåëàí âûâîä î öåëåñîîáðàçíîñòè èñïîëüçîâàíèÿ ñòîëá÷àòûõ ãëèí â êðåêèíãå ðåàëüíîãî ñûðüÿ. 76
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Èíñòèòóò êàòàëèçà
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Îðãàíèçàòîðû êîíôå
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SINGLE SITE CATALYSTS - IDEAL MODEL
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ÑÒÀÁÈËÈÇÈÐÎÂÀÍÍÛÅ
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ÈÇÓ×ÅÍÈÅ ÌÅÕÀÍÈÇÌÎ
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Ñðàâíåíèå äèíàìèêè
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ÐÎËÜ ÍÎÑÈÒÅËÅÉ Â ÔÎ
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ÒÐÈÈÇÎÁÓÒÈËÀËÞÌÈÍ
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ÏÐÎÃÐÅÑÑ Â ÎÁËÀÑÒÈ
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MOLECULAR DESIGN OF NEW TYPE OF CAT
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PALLADIUM AND COBALT CATALYZED OXID
Page 26 and 27: ÍÎÂÛÉ ÏÎÄÕÎÄ Ê ÔÎÐÌ
Page 28 and 29: Èîííûé îáìåí Al 2O 3 2+
Page 30 and 31: êîòîðûõ èììîáèëèçî
Page 32 and 33: ïðèâåäøàÿ ê ñîçäàí
Page 34 and 35: ÐÀÇÐÀÁÎÒÊÀ ÊÀÒÀËÈÇ
Page 36 and 37: ðàñïðåäåëåíèÿ ÷àñò
Page 38 and 39: ÷òî äåôåêòû ýòîãî â
Page 40 and 41: ÈÇÓ×ÅÍÈÅ ÔÎÐÌÈÐÎÂÀ
Page 42 and 43: Ñîäåðæàíèå äèîêñèä
Page 44 and 45: Òàáë. 1. Äàííûå õåìî
Page 46 and 47: ñëàáîñâÿçàííîì ñîñ
Page 48 and 49: ãèäðîãåíèçàöèè, âå
Page 50 and 51: ÑÅËÅÊÒÈÂÍÀß ÎÊÈÑËÈ
Page 52 and 53: ÌÎÄÈÔÈÖÈÐÎÂÀÍÈÅ ÀË
Page 54 and 55: ãèäðîîêèñüþ àëþìèí
Page 56 and 57: ïðîìûñëîâûõ ìèíè-Í
Page 58 and 59: ÏÎËÓ×ÅÍÈÅ ÆÈÄÊÈÕ Ó
Page 60 and 61: ÈÇÎÌÅÐÈÇÀÖÈß ÓÃËÅÂ
Page 62 and 63: ÊÀÒÀËÈÒÈ×ÅÑÊÈÅ ÏÐÅ
Page 64 and 65: îáðàçîâàíèÿ öèêëîï
Page 66 and 67: ïðåèìóùåñòâåííîå ï
Page 68 and 69: ÈÍÒÅÐÊÀËÈÐÎÂÀÍÍÛÅ
Page 70 and 71: ÊÐÅÊÈÍÃ Ñ 10 -Ñ 15 - ÀË
Page 72 and 73: Â ÈÊ- ñïåêòðàõ àäñî
Page 74 and 75: Ïî âëèÿíèþ íà êàòàë
Page 78 and 79: ÃÈÄÐÎÏÅÐÅÐÀÁÎÒÊÀ Í
Page 80 and 81: Ïîñëå ãèäðîïåðåðàá
Page 82 and 83: óñëîâèé ïðîöåññà î
Page 84 and 85: åå ðåàêöèè. Èìåííî
Page 86 and 87: í-C 4 H 8 + Pd II + Í 2 Î ⎯⎯
Page 88 and 89: ïðîäóêòîâ. Íàïðèìå
Page 90 and 91: ×ÈÑËÎ È ÐÅÀÊÖÈÎÍÍÀ
Page 92 and 93: Äëÿ âñåõ ñèñòåì îïð
Page 94 and 95: ñèíäèîòàêòè÷åñêèé
Page 96 and 97: ñâÿçåé è ýêâèâàëåí
Page 98 and 99: ÝËÅÊÒÐÎÕÈÌÈ×ÅÑÊÈÉ
Page 100 and 101: ÑÒÅÍÄÎÂÛÅ ÄÎÊËÀÄÛ
Page 102 and 103: ÈÇÓ×ÅÍÈÅ ÌÅÕÀÍÈÇÌÀ
Page 104 and 105: Ðèñóíîê 2. Äèôôåðåí
Page 106 and 107: âòîðîé ïî èíòåíñèâ
Page 108 and 109: êîëåáàíèÿ â ìîñòèê
Page 110 and 111: ÑÒÐÓÊÒÓÐÍÎ-ÎÐÃÀÍÈÇ
Page 112 and 113: Òàáëèöà 2. Ðàñïðåäå
Page 114 and 115: 50 Rate/10 -8 mol g -1 s -1 40 30 2
Page 116 and 117: ÐÀÇÐÀÁÎÒÊÀ È ÈÑÑËÅ
Page 118 and 119: êèñëîðîäó øïèíåëè C
Page 120 and 121: èçîìåðèçàöèè í-ãåê
Page 122 and 123: ÃÅÍÅÇÈÑ ÔÀÇÎÂÎÃÎ Ñ
Page 124 and 125: óïëîòíåíèÿ çàïîëíÿ
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Ïðèðîäà èñõîäíûõ ñ
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ÏÎËÈÌÅÐÍÛÅ ÐÎÄÈÉÑÎ
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ïðîìîòîðîâ. Â ðàáîò
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ôîðìàëüäåãèä, äè- è
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Äàëüíåéøàÿ äåãèäðî
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ÌÅÒÎÄÛ ÐÅÃÓËÈÐÎÂÀÍ
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ÑÈÍÒÅÇ È ÈÑÑËÅÄÎÂÀ
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ÂËÈßÍÈÅ ÎÁÐÀÁÎÒÎÊ
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Íàðÿäó ñ óâåëè÷åíè
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îáîðîòîâ êàòàëèçàò
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Íàìè ðàçðàáîòàí ïð
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äî 0,5 ÌÏà. Ôîðìû çàâ
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Î ÏÐÎÖÅÑÑÀÕ ÏÐÅÄÎÒ
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ÐÀÇÐÀÁÎÒÊÀ ÊÀÒÀËÈÒ
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ÏÐÅÂÐÀÙÅÍÈß ÑÒÈÐÎË
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ÆÈÄÊÎÔÀÇÍÀß ÈÇÎÌÅÐ
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ÍÅÏÎËÍÎÅ ÎÊÈÑËÅÍÈÅ
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ÍÀÍÎÑÒÐÓÊÒÓÐÍÛÅ ÊÀ
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ÃÈÄÐÎÊÎÍÂÅÐÑÈß Í-Ã
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ðàñòåò ñ ïîâûøåíèå
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Èíäèâèäóàëüíàÿ àäñ
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â ÑÍÃ ñíèæàåò òåìïå
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Ïðîöåññ áèôîðìèíãà
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ÈÑÏÎËÜÇÎÂÀÍÈÅ ÊÀÒÀ
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Ïîâûøåíèå äàâëåíèÿ
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Èç ïðèðîäíîãî öåîë
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ÄÅÃÈÄÐÈÐÎÂÀÍÈÅ ËÅÃ
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ðîäèåâûå è ðóòåíèå
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Òàáëèöà 1. Âëèÿíèå ï
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ÈÑÑËÅÄÎÂÀÍÈÅ ÏÐÎÖÅ
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ÏÅÐÅÐÀÁÎÒÊÀ ÄÈÑÒÈË
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ÃÈÄÐÎÏÅÐÅÐÀÁÎÒÊÀ í
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ÊÐÅÊÈÍÃ ÒßÆÅËÎÃÎ Í
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óãëåðîäà â äèîêñèä
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ïîäà÷è ñûðüÿ 1,0-1,5 ÷
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ëîêàëèçîâàííûå íà
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CÓËÜÔÎÊÀÒÈÎÍÈÒÛ ÍÀ
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Ïðè íàëè÷èè â ñèñòå
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ãåêñàäåêàíîë-2 (ïðè
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óñëîâèÿ îêèñëåíèÿ
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ãàçîâ òåðìîäåñîðáö
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ïîëèìåðèçàöèè ýòèë
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ÊÀÒÀËÈÇÈÐÓÅÌÎÅ ÏÀË
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ÈÑÑËÅÄÎÂÀÍÈÅ ÂËÈßÍ
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ÄÈÌÅÐÈÇÀÖÈß ÝÒÈËÅÍ
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ÈÇÓ×ÅÍÈÅ ÏÐÎÖÅÑÑÎÂ
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ÐÀÑÏÐÅÄÅËÅÍÈÅ ÂÍÓÒ
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ÃÎÌÎ - È ÑÎÏÎËÈÌÅÐÈ
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ÏÎËÈÌÅÐÈÇÀÖÈß ÝÒÈË
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Ñ ïðèìåíåíèåì ìåòî
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àìîðôíûìè è êðèñòà
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ÑÏÈÑÎÊ ÀÄÐÅÑÎÂ Ó×À
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ÃÐÈÃÎÐÜÅÂÀ Íåëëè Ã
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ÊÀÐÛÌÎÂÀ Ðàøèäà Õà
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ÌÓÍØÈÅÂÀ Ìèíà Êåðè
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ÓÑÌÀÍÎÂÀ Ìàíçóðà Ì
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ÑÎÄÅÐÆÀÍÈÅ ÊËÞ×ÅÂÛ
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Ñåêöèÿ II Êàòàëèç â
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CÄ-I-3 CÄ-I-4 CÄ-I-5 CÄ-I-6 CÄ
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CÄ-II-10 Çàêèðîâà À.Ã.,
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CÄ-III-4 Ìèêåíàñ T.Á., Å
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