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PP-I-29Table. Reaction temperature influence on the composition (wt %) and yields (wt %) of liquidproducts of directly distilled oil fraction transformations on zeolites with different silicamoduliProductn-AlkanesAlkenesIsoalkanes C 5+Cycloalkanes C 5+ArenesOctane numberYieldn-AlkanesAlkenesIsoalkanes C 5+Cycloalkanes C 5+ArenesOctane numberYieldn-AlkanesAlkenesIsoalkanes C 5+Cycloalkanes C 5+ArenesOctane numberYieldTemperature, °C300 340 380 42010.84.229.75.949.4918011.64.230.54.449.3918012.04.936.26.640.384857.73.322.05.661.496659.63.128.64.254.5936810.53.536.15.644.38673M = 60M = 150M = 2204.82.018.54.670.1100548.12.523.63.762.196579.23.135.15.247.488624.31.615.94.373.9102476.52.322.32.066.998508.22.234.35.749.69157These catalysts allow the yield of the desired products to be increased with asimultaneous decrease in the concentration of aromatic hydrocarbons and especially benzene,whose content in gasoline for cars is subject to severe limitations, without additionallymodifying them. Zeolites with silica moduli of 60 and 150 were characterized by strongeracid centers and higher concentrations of such centers. Liquid products obtained on thesecatalysts therefore contained large amounts of aromatic hydrocarbons with high octanenumbers. Catalyst acidity decreases substantially as the zeolite silica modulus increases to220. Transformations of the directly distilled gasoline fraction in the presence of zeolitecatalysts resulted in the formation of gasolines with octane numbers exceeding 80 over thewhole temperature range studied.264
KINETICS OF CO OXIDATION OVER Co-ZSM-5 ANDCo-Pd-ZSM-5 CATALYSTSV.K. Yatsimirsky, L.P. Oleksenko, L.V. LutsenkoPP-I-30National Taras Shevchenko University of Kyiv, 64 Volodymyrska Str., Kiev-33, Ukraine01033; fax: +38044(2393358); e-mail: larisa_lutsenko@ukr.netMetal-containing zeolites, in particular on the base of ZSM-5, are studied as catalysts of anumber of redox procecces [1, 2], therefore a research of their mechanism is very interesting.The kinetic regularities of carbon monoxide oxidation on Co-(Pd-)containing zeolite ZSM-5are investigated in this paper. The kinetics of CO oxidation over active low-loaded metalcatalysts – 1.2%Co-ZSM-5 and 0.8%Со-0.5%Pd-ZSM-5 – is observed.The catalyst 1.2%Co-ZSM-5 is obtained via impregnation of the zeolite with Co(NO 3 ) 2solution, and 0.8%Co-0.5%Pd-ZSM-5 – with [Pd(NH 3 )]Cl 2 solution and then with Со(NO 3 ) 2 ;dried samples are treated in hydrogen at 350 °C during 1 hr. Before kinetic experiments thesamples are treated at 100 – 110 °C in reaction gaseous mixture (1%CO+10%O 2 +89%He)during 1 hr for a stationary state to be established. The kinetics of carbon monoxide oxidationis studied in a non-gradient reactor of flowing type equipped by reciprocating-engine in thetemperature interval 110 – 165 °C. Concentration of carbon monoxide is changed from 0.25to 2vol.% at constant initial concentration of oxygen 20vol.% (C O2 =8,93·10 –3 mole/l); oxygenconcentration is changed from 5 to 25vol.% at constant initial concentration of CO 1vol.%(C CO =4,46·10 –4 mole/l).r·10 8 , mole CO 2/g·s40302010a4321r·10 8 , mole CO 2/g·s302010b43210 2 4 6 8 10c CO·10 4 , mole/l00 2 4 6 8 10 12c O2·10 3 , mole/lFig. Dependences of the reaction rate a) on concentration CO and b) on concentration O 2 for the catalyst1.2%Co-ZSM-5: 1 – 110°С; 2 – 130°С; 3 – 150°С; 4 – 165°С.The investigation of the CO oxidation kinetics showes that the dependencies of thereaction rate on concentration of reagents for both the catalysts at 110, 130 and 150 °C and at165 °C for the Co-ZSM-5 have a view of curves with «saturation» which coincide with each265
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Boreskov Institute of Catalysis of
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Mikhail G. Slinko,Honour ChairmanVa
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PLENARY LECTURES
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PL-1built up from an intrinsic cont
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PL-3DEVELOPMENT OF ZEOLITE-COATED M
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PL-4processes in order to evaluate
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PL-5CATALYTIC PARTIAL OXIDATION OF
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KEY-NOTE PRESENTATIONS
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KN-2GETTING TO THE POINT: FROM MOLE
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KN-3PROBLEMS AND PROSPECTS FOR IMRO
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KN-4remain out of the sight of rese
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KN-5SSITKA allows to study not only
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KN-6individual reaction stages with
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Section 1.Kinetics of catalytic rea
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OP-I-1-specialthat Г s /f changed
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OP-I-3-specialKINETIC MODELING OF L
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OP-I-4PARTIAL OXIDATION OF TOLUENE
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OP-I-5Also, the approach to modelin
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OP-I-6starch granules, but after a
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OP-I-8KINETICS OF CARBON MONOXIDE O
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OP-I-9CHAOTIC DYNAMICS IN THE THREE
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OP-I-10ADSORPTION OF COMPLEX MOLECU
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OP-I-11KINETIC ASPECTS OF METHANE O
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OP-I-12KINETIC STUDIES IN STRUCTURE
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OP-I-13A STUDY ON THERMAL COMBUSTIO
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OP-I-14KINETICS OF THE CONVERSION O
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OP-I-15HYDROCRACKING OF LONG CHAIN
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OP-I-16KINETICS IN THE HYDROGENATIO
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OP-I-17MECHANISM OF FORMATION OF ET
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OP-I-18KINETIC STUDIES OF PROPANE D
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OP-I-19ACTIVITY AND DEACTIVATION OF
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OP-I-20GAS PHASE OXIDATION OF FORMA
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OP-I-21Where k A is the rate consta
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OP-I-22al., 2008; Monolith, 2008).
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OP-I-23Fig. 1. Scheme of the FIM ma
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OP-I-24Θ DZ centersdeactivationr D
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OP-I-25equation [2] to nitrogen iso
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OP-II-1CHEMICAL NANOREACTORS AS BAS
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OP-II-2gas model use, there is no n
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OP-II-3Taking into account these pr
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OP-II-4WATER2METH1STEAM2AOFF3AIR10O
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OP-II-5completely dry, at the same
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OP-II-6Many factors have been found
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OP-II-7mechanistic and kinetic stud
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OP-II-9MODELLING OF DIESEL PARTICUL
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Section 3.Catalytic processesí dev
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OP-III-1BIC’s catalyst for N 2 О
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OP-III-2powder sample with the same
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OP-III-3Analysis of the results sho
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OP-III-4Exhaustaftertreatmenttechno
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OP-III-6SOME PROPERTIES OF PEROVSKI
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OP-III-7with the conventional react
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OP-III-8resistance is the membrane
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OP-III-9mass dispersion and to anal
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OP-III-11PROCESS INTENSIFICATION US
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OP-III-12ETHYL ACETATE SYNTHESIS BY
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OP-III-12products are vaporized and
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OP-III-13The reforming reaction was
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OP-III-14reactivity (compared to ot
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OP-III-15Fig. 2. The spent Smopex-1
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OP-III-16Numbers of curves are acco
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OP-III-17perimeter were determined.
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OP-III-18of 2. MSR has been coupled
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OP-III-19chemisorption heat and pro
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OP-III-20In the experiments, total
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OP-III-21obtained by the new techno
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OP-III-22reactor wall from the two-
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OP-III-23and parameters of synthesi
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OP-III-24Results and discussionThe
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OP-IV-1DEEP DESULPHURIZATION OF PET
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OP-IV-2LACTIC ACID AS A BACKGROUND
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OP-IV-3CO REMOVAL FROM H 2 -rich GA
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OP-IV-4REFORMING OF ETHANOL OVER ME
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OP-IV-5MODELING OF HYDROGEN PRODUCT
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OP-IV-6PRODUCTION OF HYDROGEN FROM
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OP-IV-7SYNTHESIS GAS PRODUCTION FRO
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OP-IV-8HYDROGEN PRODUCTION FROM MET
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OP-IV-9A NEW GENERATION OF SUPER-TH
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OP-IV-10EXERGY ANALYSIS OF ENZYMATI
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OP-IV-11ADVANCEMENT OF SLURRY BUBBL
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OP-IV-12Pd-DOPED PEROVSKITE CATALYS
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OP-IV-13HYDROGEN PRODUCTION VIA MET
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Section 5.Catalytic processing of r
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OP-V-1Scheme 1. The developing path
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OP-V-2An example of the model compo
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OP-V-3catalysts were shown to be su
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OP-V-4Catalyst deactivation was mor
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OP-V-53) Study of the FFAs esterifi
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OP-V-6In the present work, a compre
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OP-V-7Ca 2 Fe 2 O 5 , MgFe 2 O 4 an
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OP-V-8cellulose components decompos
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OP-V-9sintering a couple of spirale
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OP-V-10Catalyst preparationA series
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OP-V-11Catalysts characterizationIn
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OP-V-12Kinetic ExperimentsHexadecan
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OP-V-13DESIGN OF PILOT REACTOR AND
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OP-V-14DEVELOPMENT OF A LAB SCALE C
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OP-V-15DEVELOPMENT OF TWO-STAGE PRO
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OP-V-15The data of Table 2 show, th
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OP-V-17ENERGY PRODUCTION FROM BIOMA
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OP-V-18CATALYTIC PARTIAL OXIDATION
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OP-V-19A PHOTOCATALYTIC REACTOR FOR
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OP-V-20BIOMASS GASIFICATION IN A CA
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OP-V-21ESTIMATION OF OPTIMAL REACTO
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POSTER PRESENTATIONSSection 1. Kine
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PP-I-1CONVERSION OF ETHANOL OVER CO
Page 214 and 215: PP-I-2LATERAL INTERACTIONS, FINITE
Page 216 and 217: PP-I-3UTILIZATION OF TAFT EQUATION:
Page 218 and 219: PP-I-4SELECTIVE HYDROGENATION OF CI
Page 220 and 221: PP-I-5NON OXIDATIVE REGENERATION ME
Page 222 and 223: PP-I-6Table 1. Parameters in kineti
Page 224 and 225: PP-I-7where: k nc , k 1 , k a , k b
Page 226 and 227: PP-I-8After each adsorption or deso
Page 228 and 229: PP-I-9The increase in pressure, in
Page 230 and 231: PP-I-10The analysis of the composit
Page 232 and 233: PP-I-11The network of βP oxidation
Page 234 and 235: PP-I-12order of magnitude lower. Th
Page 236 and 237: PP-I-13ab1,01,0Isotope fraction0,5[
Page 238 and 239: PP-I-14Relations ‘rate vs alcohol
Page 240 and 241: PP-I-15[EEAA] t , M[EEAA] t -1 , M
Page 242 and 243: PP-I-17NEW OSCILLATING REACTION:CAR
Page 244 and 245: PP-I-18NEW OSCILLATING REACTIONS OF
Page 246 and 247: PP-I-19KINETICS OF GAS-LIQUID PROCE
Page 248 and 249: PP-I-20COMPLETE OXIDATION OF HARMFU
Page 250 and 251: PP-I-21THEORETICAL RESEARCH OF SURF
Page 252 and 253: PP-I-22INFLUENCE OF ORGANIC HELATES
Page 254 and 255: PP-I-23The equation of the reaction
Page 256 and 257: PP-I-25SELECTIVE OXIDATION OF METHA
Page 258 and 259: PP-I-26coefficients of the equation
Page 260 and 261: PP-I-27into propionic acid. The giv
Page 262 and 263: PP-I-28In the studied range of temp
Page 266 and 267: PP-I-30other in both direction of t
Page 268 and 269: PP-I-31Reynolds number. The boundar
Page 270 and 271: PP-I-32NANOPARTICLES AND CATALYSISI
Page 272 and 273: Section 2.Physico-chemical and math
Page 274 and 275: PP-II-1For investigation, we used n
Page 276 and 277: PP-II-2criterion «Zn dissolved in
Page 278 and 279: PP-II-3exist around the steady stat
Page 280 and 281: PP-II-4in range 0-1. In our case n
Page 282 and 283: PP-II-5at comparable activity, the
Page 284 and 285: PP-II-7CFD-CALCULATION OF MALDISTRI
Page 286 and 287: PP-II-8INVESTIGATION OF NONLINEAR P
Page 288 and 289: PP-II-8reactivity. There is a small
Page 290 and 291: PP-II-10CALCULATION OF INDUSTRIAL C
Page 292 and 293: PP-II-11type of reactors a catalyst
Page 294 and 295: PP-II-13MATHEMATTICAL MODELLING OF
Page 296 and 297: PP-II-13where I Э , M 1Э , M 2Э
Page 298 and 299: PP-II-14where TOC 0 is the initial
Page 300 and 301: PP-II-16AUTOCATALYTIC REACTION FRON
Page 302 and 303: Section 3.Catalytic processesí dev
Page 304 and 305: PP-III-1for the traditional scheme
Page 306 and 307: PP-III-2Initial conditions: С i (0
Page 308 and 309: PP-III-3Afterward, a 30% aqueous hy
Page 310 and 311: PP-III-4The influence of the water
Page 312 and 313: PP-III-5Vanadium oxide was grafted
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PP-III-6(T p ) was taken as an inde
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PP-III-7dCdτLABdCNABdτdCdτdCdτd
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PP-III-8O 2 , balanced by He, at a
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PP-III-9Solution of system (3) for
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PP-III-10HDT330ºCHDT350ºCHDT370º
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PP-III-11The activity of Au/support
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PP-III-1249775 m 3 /h0,65Initial te
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PP-III-13through one layer of ACC w
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PP-III-14the runs was always higher
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PP-III-15The experimental data for
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PP-III-16Catalytic hydrogenation of
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PP-III-17The following parameters a
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PP-III-18Figure 1 - Dependence of t
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PP-III-19Our method has some advant
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PP-III-20Furthermore, Ayude et al.
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PP-III-22OPTIMIZATION OF THE METHAN
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PP-III-23EXPERIMENTAL INVESTIGATION
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PP-III-24CATALYTIC REACTORS WITH HY
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PP-III-25ACTIVITY OF Cu/ZSM-5 CATAL
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PP-III-26SIMULATION AND OPTIMISATIO
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PP-III-27model of plug flow reactor
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PP-III-28Calculations were experime
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PP-III-29continuous and pressurized
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PP-III-30adequacy of multistage mod
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PP-III-31+CH 3 OHH 2 O + HO-(CH(CH
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PP-III-32procedure presented by Mar
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PP-III-33HPA-x + 2 H + + Pd 0 ⎯
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PP-III-34of the process as well as
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PP-III-35This study was financially
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PP-III-36phase. Peroxopolyoxometall
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PP-III-37performed under atmospheri
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PP-III-38orders of magnitude larger
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PP-III-39CATALYTIC REACTORS WITH ST
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PP-III-40THE OXIDATIVE DEHYDROGENAT
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PP-III-41MODELLING AND DESIGN OF TH
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PP-III-42COMPLEX TECHNOLOGY OF TREA
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PP-III-43PHOTO ELECTROCHEMISTRY APP
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PP-III-45MODELING OF CATALYTIC α-O
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PP-III-46steady states. It was show
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PP-III-47Results and discussion:The
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PP-III-49FIBROUS PALLADIUM-SUPPORTE
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Section 4.Catalytic technologies in
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PP-IV-1method is adiabatic or autot
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PP-IV-2It had been established that
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PP-IV-4INTERACTION OF ACTIVATED ALU
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PP-IV-5ENVIRONMENTALLY FRIENDLY PRO
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PP-IV-6THE 5%Ni-2%Au/Al 3 CrO 6 SYS
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PP-IV-7MESOPOROUS ANODES BASED ON Y
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PP-IV-8ADVANCED OXIDATION PROCESS F
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PP-IV-9PROCESSING OF POLYMERIC CORD
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PP-IV-10EFFECT OF SULPHUR ON THE CA
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PP-IV-11OXIDATIVE CONVERSION OF MET
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PP-IV-13CATALYTIC FLUE GAS CONDITIO
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PP-IV-14RIBBON POROUS NICKEL BASED
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PP-IV-15ETHANOL CONVERSION TO HYDRO
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PP-IV-16A HIGH-EFFICIENT MICROREACT
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PP-IV-17DIRECT DECOMPOSITION OF NIT
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PP-IV-18NICKEL CATALYSTS BASED ON P
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PP-IV-19SELECTION OF FAVOURABLE FEE
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PP-IV-20FORMALDEHYDE FORMATION DURI
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PP-IV-21PRODUCTION OF HYDROGEN-RICH
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PP-IV-22INFLUENCE OF COMPOSITION OF
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PP-IV-24ONE-STAGE CATALYTIC CONVERS
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PP-IV-25THE STUDY OF METHANE DEHYDR
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PP-IV-26MCM-41-SUPPORTED PdNi CATAL
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PP-IV-27IMPROVING THE FLOW SHEET OF
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PP-IV-29THE PARTIAL OXIDATION OF CH
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PP-IV-30PRODUCTION OF CO-FREE HYDRO
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PP-IV-31PHOTOCATALYTICAL ACTIVITY O
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PP-IV-32NEW ELECTRODE MATERIALSFOR
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PP-IV-33THE CATALYTIC HYDROGENATION
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PP-IV-34W 0, μmol O 2/min0,25 1. 1
Page 458 and 459:
PP-V-1INFLUENCE OF ICE ON MEAs OF P
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PP-V-2DIRECT OILS HYDROGENATION TO
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PP-V-3DEVELOPMENT OF Pd/SIBUNIT CAT
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PP-V-4Pt NANOPARTICLE-HOLLOW POROUS
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PP-V-5THE PROCESS FOR PRODUCING ORG
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PP-V-6water removing. This method p
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PP-V-7ResultsThe presented technolo
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PP-V-8the most effective catalysts.
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PP-V-9Neither the low sulphur conte
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PP-V-10composition (methyl esters,
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PP-V-11reactor we can see that its
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PP-V-12Recent studies lead in this
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PP-V-13catalysts (e.g. Pt or Pd), t
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PP-V-14Alkali catalyst. For a basic
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PP-V-15obtaining the related profil
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PP-V-16reaction parameters, not rep
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PP-V-18STUDY OF THE CATALYTIC ACTIV
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PP-V-19BIOMORPHIC CATALYSTS ON THE
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PP-V-20Al,Cu-PILLARED CLAYS AS CATA
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PP-V-21KINETICS OF THE HYDROXYMATAI
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PP-V-22THE NEW METHOD OF OBTAINING
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PP-V-23containing mono- and di-subs
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AUTOCLAVE ENGINEERS COMPANYSYSTEMAT
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CATACON CATACON CATACON CATACON CAT
Page 506 and 507:
Page 508 and 509:
Page 510 and 511:
George AvgouropoulosFoundation for
Page 512 and 513:
Leonid BykovJSC «Chemphyst-Alloy L
Page 514 and 515:
Debora FinoPolitecnico di TorinoCor
Page 516 and 517:
Jenő HancsókUniversity of Pannoni
Page 518 and 519:
Andrey KhudoshinLomonosov Moscow St
Page 520 and 521:
Cristian LedesmaEnergetic Technique
Page 522 and 523:
Uri Matatov-MeytalDepartment of Che
Page 524 and 525:
Karina OjedaIndustrial University o
Page 526 and 527:
Yuri PyatnitskyPisarzhevsky Institu
Page 528 and 529:
Vera ScmachkovaBoreskov Institute o
Page 530 and 531:
Peter StrizhakPisarzhevsky Institut
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Nadezhda VernikovskayaBoreskov Inst
Page 534 and 535:
Nataliya ZubritskayaRSC «Applied C
Page 536 and 537:
ORAL PRESENTATIONS.................
Page 538 and 539:
OP-I-21Saeedizad M., Sahebdelfar S.
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OP-III-9Nekhamkina O., Sheintuch M.
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OP-IV-5Hernández L., Kafarov V.V.M
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OP-V-13Sadykov V., Mezentseva N., V
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PP-I-15PP-I-16PP-I-17PP-I-18PP-I-19
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PP-II-9 Nikiforov A., Paek U-Hyon,
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PP-III-17 Vernikovskaya N.V., Kashk
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PP-III-42 Goshu Y.W., Tsaryov Y.V.,
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PP-IV-17 Ohnishi C.H., Yoshino H.,
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PP-V-9 Hancsók J., Magyar S., Kall
Page 558:
XVIII International Conference on C
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