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PP-III-7dCdτLABdCNABdτdCdτdCdτdCdτolefinesi-olefinesdiolefines= k C − k C ( C + C )1 olefines 3 LAB olefines i-olefines= k C − k C ( C + C )2 i-olefines 3 NAB olefines i-olefines=−k C − k C ( C + C ) − k C ( C + C1 olefines 3 olefines LAB NAB 5 olefines aromatics DAB=−k C − k C ( C + C ) −k C ( C=−kC2 i-olefines 3 i-olefines LAB NAB 5 i-olefines aromaticsC24 diolefines benzenedCbenzene=−2kC C −kC −kCdτdCDPA2= kC4 diolefinesCbenzenedτdCPAB= k5( Colefines + Ci-olefines )( Caromatics + CDAB)dτdCDABdττ = 0 C (0) = C24 diolefines benzene 1 olefines 2 i-olefines= k3( Colefines + Ci-olefines )( CLAB + CNAB) − k5(Colefines+ C i-olefines) C DABi i, 0Where τ – contact time, sec; C – concentration of i-component, mol·m –3 i.Estimation of rate constants for these reactions ( k 1− k 5) was carried out based onavailable information from different sources [1, 2, 3] and experimental data from realindustrial unit at Kirishi LAS-production plant.)+ CAnother input data were processed with the use of mathematical model and the calculatedoutput data (yield and biodegradability factor of the target product) were compared to theexperimental ones.As the results of product yield and quality calculation conform to similar experimentalfigures, the model can be used for estimation of alkylation process efficiency under differenttechnological conditions.References1. Zhigang Lei, Chengyue Li, Biaohua Chen, Wang Erqiang and Jinchang Zhang. Study on the alkylation ofbenzene and 1-dodecene. Chemical Engineering Journal. Volume 93, Issue 3 (2003), pp. 191-200.2. Jinchang Zhang, Biaohua Chen, Chengyue Li, Zuogang Zhu, Langyou Wen and Enze Min. Kinetics ofbenzene alkylation with 1-dodecene over a supported tungstophosphoric acid catalyst. Applied Catalysis A:General. Volume 249, Issue 1 (2003), pp. 27-34.3. G.D. Yadav, N.S. Doshi. Synthesis of Linear Phenyldodecanes by the Alkylation of Benzene with1-Dodecene over Non-Zeolitic Catalysts. Org. Proc. Res. Dev., 6 (3) (2003), pp. 263 -272.DAB)316
PEROVSKITE CATALYSTS FOR NO REDUCTION WITH H 2S. Furfori, N. Russo, D. Fino, G. Saracco, V. SpecchiaDepartment of Material Science and Chemical Engineering, Politecnico di Torino,Corso Duca degli Abruzzi, 24 10129, TorinoTel./Fax: 011.564.4710/4699; corresponding author: debora.fino@polito.itPP-III-8IntroductionRoad transport is a major contributor of hydrocarbons (HC), nitrogen oxides (NO x ) andparticulate matter (PM). The prevalent technology available to control NO x emission is indeedthe selective catalytic reduction (SCR) by NH 3 . In the last years, the use of hydrocarbons, coexistingin the vehicle exhaust, as reducing agents has been extensively studied [1]. Hydrogencould be the most likely candidate as a reducing agent in the SCR reaction to abate NO xemissions in an excess oxygen environment, such as diesel engine exhaust; this possibility hasbeen reported by several researchers [2]. The high performance of H 2 -SCR reaction canjustify the employment of a reformer for H 2 generation from diesel fuel.In the present paper, the activity of perovskite catalysts belonging to the LaFeO 3 familywas investigated for the H 2 -SCR technology. On the basis of the obtained results, thesuitability of the mentioned catalysts for application in the treatment of the diesel exhaustswill be finally discussed.Experimental Campaign & ResultsA series of perovskite catalysts(La 0.8 Sr 0.2 FeO 3 , La 0.8 Sr 0.2 Fe 0.9 Pd 0.1 O 3 ,La 0.7 Sr 0.2 Ce 0.1 FeO 3 , Pd/La 0.7 Sr 0.2 Ce 0.1 FeO 3 ) havebeen prepared by Solution Combustion Synthesis(SCS) from an aqueous solution of metal nitratesprecursors and urea (acting as a sacrificial fuel).According to this method an easily-crumblingfoam of nano-sized particles (see Fig. 1) with high Fig. 1. FESEM picture of La 0.7 Sr 0.2 Ce 0.1 FeO 3 .specific surface area was obtained. Pd was then deposited via IWP [3] employing an aqueoussolution of Palladium nitrate. The prepared powder was dried in oven at 120°C for 12 hours,then calcined in air at 500°C for 5 hours in order to decompose the nitrate and obtain smalland well dispersed Palladium clusters on the perovskite surface.The catalysts were characterized (XRD, FESEM, BET) and tested in a fixed-bed quartzmicroreactor under an atmosphere of 1000 ppmv NO, 4000 ppmv H 2 , with 10% or without317
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Boreskov Institute of Catalysis of
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Mikhail G. Slinko,Honour ChairmanVa
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PLENARY LECTURES
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PL-1built up from an intrinsic cont
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PL-3DEVELOPMENT OF ZEOLITE-COATED M
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PL-4processes in order to evaluate
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PL-5CATALYTIC PARTIAL OXIDATION OF
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KEY-NOTE PRESENTATIONS
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KN-2GETTING TO THE POINT: FROM MOLE
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KN-3PROBLEMS AND PROSPECTS FOR IMRO
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KN-4remain out of the sight of rese
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KN-5SSITKA allows to study not only
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KN-6individual reaction stages with
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Section 1.Kinetics of catalytic rea
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OP-I-1-specialthat Г s /f changed
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OP-I-3-specialKINETIC MODELING OF L
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OP-I-4PARTIAL OXIDATION OF TOLUENE
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OP-I-5Also, the approach to modelin
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OP-I-6starch granules, but after a
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OP-I-8KINETICS OF CARBON MONOXIDE O
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OP-I-9CHAOTIC DYNAMICS IN THE THREE
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OP-I-10ADSORPTION OF COMPLEX MOLECU
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OP-I-11KINETIC ASPECTS OF METHANE O
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OP-I-12KINETIC STUDIES IN STRUCTURE
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OP-I-13A STUDY ON THERMAL COMBUSTIO
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OP-I-14KINETICS OF THE CONVERSION O
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OP-I-15HYDROCRACKING OF LONG CHAIN
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OP-I-16KINETICS IN THE HYDROGENATIO
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OP-I-17MECHANISM OF FORMATION OF ET
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OP-I-18KINETIC STUDIES OF PROPANE D
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OP-I-19ACTIVITY AND DEACTIVATION OF
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OP-I-20GAS PHASE OXIDATION OF FORMA
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OP-I-21Where k A is the rate consta
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OP-I-22al., 2008; Monolith, 2008).
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OP-I-23Fig. 1. Scheme of the FIM ma
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OP-I-24Θ DZ centersdeactivationr D
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OP-I-25equation [2] to nitrogen iso
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OP-II-1CHEMICAL NANOREACTORS AS BAS
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OP-II-2gas model use, there is no n
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OP-II-3Taking into account these pr
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OP-II-4WATER2METH1STEAM2AOFF3AIR10O
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OP-II-5completely dry, at the same
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OP-II-6Many factors have been found
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OP-II-7mechanistic and kinetic stud
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OP-II-9MODELLING OF DIESEL PARTICUL
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Section 3.Catalytic processesí dev
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OP-III-1BIC’s catalyst for N 2 О
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OP-III-2powder sample with the same
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OP-III-3Analysis of the results sho
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OP-III-4Exhaustaftertreatmenttechno
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OP-III-6SOME PROPERTIES OF PEROVSKI
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OP-III-7with the conventional react
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OP-III-8resistance is the membrane
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OP-III-9mass dispersion and to anal
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OP-III-11PROCESS INTENSIFICATION US
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OP-III-12ETHYL ACETATE SYNTHESIS BY
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OP-III-12products are vaporized and
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OP-III-13The reforming reaction was
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OP-III-14reactivity (compared to ot
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OP-III-15Fig. 2. The spent Smopex-1
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OP-III-16Numbers of curves are acco
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OP-III-17perimeter were determined.
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OP-III-18of 2. MSR has been coupled
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OP-III-19chemisorption heat and pro
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OP-III-20In the experiments, total
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OP-III-21obtained by the new techno
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OP-III-22reactor wall from the two-
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OP-III-23and parameters of synthesi
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OP-III-24Results and discussionThe
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OP-IV-1DEEP DESULPHURIZATION OF PET
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OP-IV-2LACTIC ACID AS A BACKGROUND
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OP-IV-3CO REMOVAL FROM H 2 -rich GA
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OP-IV-4REFORMING OF ETHANOL OVER ME
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OP-IV-5MODELING OF HYDROGEN PRODUCT
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OP-IV-6PRODUCTION OF HYDROGEN FROM
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OP-IV-7SYNTHESIS GAS PRODUCTION FRO
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OP-IV-8HYDROGEN PRODUCTION FROM MET
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OP-IV-9A NEW GENERATION OF SUPER-TH
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OP-IV-10EXERGY ANALYSIS OF ENZYMATI
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OP-IV-11ADVANCEMENT OF SLURRY BUBBL
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OP-IV-12Pd-DOPED PEROVSKITE CATALYS
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OP-IV-13HYDROGEN PRODUCTION VIA MET
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Section 5.Catalytic processing of r
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OP-V-1Scheme 1. The developing path
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OP-V-2An example of the model compo
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OP-V-3catalysts were shown to be su
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OP-V-4Catalyst deactivation was mor
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OP-V-53) Study of the FFAs esterifi
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OP-V-6In the present work, a compre
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OP-V-7Ca 2 Fe 2 O 5 , MgFe 2 O 4 an
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OP-V-8cellulose components decompos
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OP-V-9sintering a couple of spirale
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OP-V-10Catalyst preparationA series
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OP-V-11Catalysts characterizationIn
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OP-V-12Kinetic ExperimentsHexadecan
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OP-V-13DESIGN OF PILOT REACTOR AND
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OP-V-14DEVELOPMENT OF A LAB SCALE C
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OP-V-15DEVELOPMENT OF TWO-STAGE PRO
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OP-V-15The data of Table 2 show, th
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OP-V-17ENERGY PRODUCTION FROM BIOMA
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OP-V-18CATALYTIC PARTIAL OXIDATION
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OP-V-19A PHOTOCATALYTIC REACTOR FOR
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OP-V-20BIOMASS GASIFICATION IN A CA
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OP-V-21ESTIMATION OF OPTIMAL REACTO
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POSTER PRESENTATIONSSection 1. Kine
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PP-I-1CONVERSION OF ETHANOL OVER CO
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PP-I-2LATERAL INTERACTIONS, FINITE
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PP-I-3UTILIZATION OF TAFT EQUATION:
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PP-I-4SELECTIVE HYDROGENATION OF CI
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PP-I-5NON OXIDATIVE REGENERATION ME
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PP-I-6Table 1. Parameters in kineti
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PP-I-7where: k nc , k 1 , k a , k b
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PP-I-8After each adsorption or deso
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PP-I-9The increase in pressure, in
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PP-I-10The analysis of the composit
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PP-I-11The network of βP oxidation
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PP-I-12order of magnitude lower. Th
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PP-I-13ab1,01,0Isotope fraction0,5[
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PP-I-14Relations ‘rate vs alcohol
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PP-I-15[EEAA] t , M[EEAA] t -1 , M
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PP-I-17NEW OSCILLATING REACTION:CAR
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PP-I-18NEW OSCILLATING REACTIONS OF
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PP-I-19KINETICS OF GAS-LIQUID PROCE
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PP-I-20COMPLETE OXIDATION OF HARMFU
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PP-I-21THEORETICAL RESEARCH OF SURF
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PP-I-22INFLUENCE OF ORGANIC HELATES
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PP-I-23The equation of the reaction
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PP-I-25SELECTIVE OXIDATION OF METHA
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PP-I-26coefficients of the equation
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PP-I-27into propionic acid. The giv
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PP-I-28In the studied range of temp
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PP-I-29Table. Reaction temperature
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Page 268 and 269: PP-I-31Reynolds number. The boundar
Page 270 and 271: PP-I-32NANOPARTICLES AND CATALYSISI
Page 272 and 273: Section 2.Physico-chemical and math
Page 274 and 275: PP-II-1For investigation, we used n
Page 276 and 277: PP-II-2criterion «Zn dissolved in
Page 278 and 279: PP-II-3exist around the steady stat
Page 280 and 281: PP-II-4in range 0-1. In our case n
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Page 284 and 285: PP-II-7CFD-CALCULATION OF MALDISTRI
Page 286 and 287: PP-II-8INVESTIGATION OF NONLINEAR P
Page 288 and 289: PP-II-8reactivity. There is a small
Page 290 and 291: PP-II-10CALCULATION OF INDUSTRIAL C
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Page 294 and 295: PP-II-13MATHEMATTICAL MODELLING OF
Page 296 and 297: PP-II-13where I Э , M 1Э , M 2Э
Page 298 and 299: PP-II-14where TOC 0 is the initial
Page 300 and 301: PP-II-16AUTOCATALYTIC REACTION FRON
Page 302 and 303: Section 3.Catalytic processesí dev
Page 304 and 305: PP-III-1for the traditional scheme
Page 306 and 307: PP-III-2Initial conditions: С i (0
Page 308 and 309: PP-III-3Afterward, a 30% aqueous hy
Page 310 and 311: PP-III-4The influence of the water
Page 312 and 313: PP-III-5Vanadium oxide was grafted
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Page 320 and 321: PP-III-9Solution of system (3) for
Page 322 and 323: PP-III-10HDT330ºCHDT350ºCHDT370º
Page 324 and 325: PP-III-11The activity of Au/support
Page 326 and 327: PP-III-1249775 m 3 /h0,65Initial te
Page 328 and 329: PP-III-13through one layer of ACC w
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Page 332 and 333: PP-III-15The experimental data for
Page 334 and 335: PP-III-16Catalytic hydrogenation of
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Page 338 and 339: PP-III-18Figure 1 - Dependence of t
Page 340 and 341: PP-III-19Our method has some advant
Page 342 and 343: PP-III-20Furthermore, Ayude et al.
Page 344 and 345: PP-III-22OPTIMIZATION OF THE METHAN
Page 346 and 347: PP-III-23EXPERIMENTAL INVESTIGATION
Page 348 and 349: PP-III-24CATALYTIC REACTORS WITH HY
Page 350 and 351: PP-III-25ACTIVITY OF Cu/ZSM-5 CATAL
Page 352 and 353: PP-III-26SIMULATION AND OPTIMISATIO
Page 354 and 355: PP-III-27model of plug flow reactor
Page 356 and 357: PP-III-28Calculations were experime
Page 358 and 359: PP-III-29continuous and pressurized
Page 360 and 361: PP-III-30adequacy of multistage mod
Page 362 and 363: PP-III-31+CH 3 OHH 2 O + HO-(CH(CH
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PP-III-33HPA-x + 2 H + + Pd 0 ⎯
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PP-III-34of the process as well as
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PP-III-35This study was financially
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PP-III-36phase. Peroxopolyoxometall
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PP-III-37performed under atmospheri
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PP-III-38orders of magnitude larger
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PP-III-39CATALYTIC REACTORS WITH ST
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PP-III-40THE OXIDATIVE DEHYDROGENAT
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PP-III-41MODELLING AND DESIGN OF TH
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PP-III-42COMPLEX TECHNOLOGY OF TREA
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PP-III-43PHOTO ELECTROCHEMISTRY APP
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PP-III-45MODELING OF CATALYTIC α-O
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PP-III-46steady states. It was show
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PP-III-47Results and discussion:The
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PP-III-49FIBROUS PALLADIUM-SUPPORTE
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Section 4.Catalytic technologies in
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PP-IV-1method is adiabatic or autot
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PP-IV-2It had been established that
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PP-IV-4INTERACTION OF ACTIVATED ALU
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PP-IV-5ENVIRONMENTALLY FRIENDLY PRO
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PP-IV-6THE 5%Ni-2%Au/Al 3 CrO 6 SYS
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PP-IV-7MESOPOROUS ANODES BASED ON Y
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PP-IV-8ADVANCED OXIDATION PROCESS F
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PP-IV-9PROCESSING OF POLYMERIC CORD
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PP-IV-10EFFECT OF SULPHUR ON THE CA
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PP-IV-11OXIDATIVE CONVERSION OF MET
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PP-IV-13CATALYTIC FLUE GAS CONDITIO
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PP-IV-14RIBBON POROUS NICKEL BASED
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PP-IV-15ETHANOL CONVERSION TO HYDRO
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PP-IV-16A HIGH-EFFICIENT MICROREACT
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PP-IV-17DIRECT DECOMPOSITION OF NIT
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PP-IV-18NICKEL CATALYSTS BASED ON P
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PP-IV-19SELECTION OF FAVOURABLE FEE
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PP-IV-20FORMALDEHYDE FORMATION DURI
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PP-IV-21PRODUCTION OF HYDROGEN-RICH
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PP-IV-22INFLUENCE OF COMPOSITION OF
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PP-IV-24ONE-STAGE CATALYTIC CONVERS
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PP-IV-25THE STUDY OF METHANE DEHYDR
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PP-IV-26MCM-41-SUPPORTED PdNi CATAL
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PP-IV-27IMPROVING THE FLOW SHEET OF
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PP-IV-29THE PARTIAL OXIDATION OF CH
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PP-IV-30PRODUCTION OF CO-FREE HYDRO
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PP-IV-31PHOTOCATALYTICAL ACTIVITY O
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PP-IV-32NEW ELECTRODE MATERIALSFOR
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PP-IV-33THE CATALYTIC HYDROGENATION
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PP-IV-34W 0, μmol O 2/min0,25 1. 1
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PP-V-1INFLUENCE OF ICE ON MEAs OF P
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PP-V-2DIRECT OILS HYDROGENATION TO
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PP-V-3DEVELOPMENT OF Pd/SIBUNIT CAT
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PP-V-4Pt NANOPARTICLE-HOLLOW POROUS
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PP-V-5THE PROCESS FOR PRODUCING ORG
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PP-V-6water removing. This method p
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PP-V-7ResultsThe presented technolo
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PP-V-8the most effective catalysts.
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PP-V-9Neither the low sulphur conte
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PP-V-10composition (methyl esters,
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PP-V-11reactor we can see that its
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PP-V-12Recent studies lead in this
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PP-V-13catalysts (e.g. Pt or Pd), t
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PP-V-14Alkali catalyst. For a basic
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PP-V-15obtaining the related profil
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PP-V-16reaction parameters, not rep
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PP-V-18STUDY OF THE CATALYTIC ACTIV
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PP-V-19BIOMORPHIC CATALYSTS ON THE
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PP-V-20Al,Cu-PILLARED CLAYS AS CATA
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PP-V-21KINETICS OF THE HYDROXYMATAI
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PP-V-22THE NEW METHOD OF OBTAINING
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PP-V-23containing mono- and di-subs
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AUTOCLAVE ENGINEERS COMPANYSYSTEMAT
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CATACON CATACON CATACON CATACON CAT
Page 506 and 507:
Page 508 and 509:
Page 510 and 511:
George AvgouropoulosFoundation for
Page 512 and 513:
Leonid BykovJSC «Chemphyst-Alloy L
Page 514 and 515:
Debora FinoPolitecnico di TorinoCor
Page 516 and 517:
Jenő HancsókUniversity of Pannoni
Page 518 and 519:
Andrey KhudoshinLomonosov Moscow St
Page 520 and 521:
Cristian LedesmaEnergetic Technique
Page 522 and 523:
Uri Matatov-MeytalDepartment of Che
Page 524 and 525:
Karina OjedaIndustrial University o
Page 526 and 527:
Yuri PyatnitskyPisarzhevsky Institu
Page 528 and 529:
Vera ScmachkovaBoreskov Institute o
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Peter StrizhakPisarzhevsky Institut
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Nadezhda VernikovskayaBoreskov Inst
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Nataliya ZubritskayaRSC «Applied C
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ORAL PRESENTATIONS.................
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OP-I-21Saeedizad M., Sahebdelfar S.
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OP-III-9Nekhamkina O., Sheintuch M.
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OP-IV-5Hernández L., Kafarov V.V.M
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OP-V-13Sadykov V., Mezentseva N., V
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PP-I-15PP-I-16PP-I-17PP-I-18PP-I-19
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PP-II-9 Nikiforov A., Paek U-Hyon,
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PP-III-17 Vernikovskaya N.V., Kashk
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PP-III-42 Goshu Y.W., Tsaryov Y.V.,
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PP-IV-17 Ohnishi C.H., Yoshino H.,
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PP-V-9 Hancsók J., Magyar S., Kall
Page 558:
XVIII International Conference on C
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