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aktualisiertes pdf - DPG-Tagungen

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Fachvortrag UP 3.5 Mo 17:30 HS 118<br />

NO2-Columns measured by the AMAXDOAS instrument over<br />

Europe in 2003 — •Klaus-Peter Heue 1 , Marco Bruns 2 , John<br />

P. Burrows 2 , Wei-Der Lee 1 , Ulrich Platt 1 , Irene Pundt 1 , Andreas<br />

Richter 2 , Thomas Wagner 1 , and Ping Wang 2 — 1 Institut<br />

für Umweltphysik, Universität Heidelberg, INF 229, D-69120 Heidelberg<br />

— 2 Institut für Umweltphysik, Universität Bremen, Otto-Hahn-Allee 1,<br />

D-28359 Bremen<br />

The Air borne Multi AXis DOAS (AMAXDOAS) was successfully operated<br />

during two campaigns in winter and summer 2003. During winter<br />

it was run aboard the DLR Falcon (2nd airborne campaign for SCIA-<br />

MACHY validation). The aircraft flew to the Arctic and to the Tropics<br />

at about 10 km flight altitude with a total flight track of 6400 km over<br />

Europe. In addition the OLEX (Lidar) and the ASUR (Microwave) instruments<br />

were operated onboard this aeroplane.<br />

During summer (EU-FORMAT II campaign), the AMAXDOAS was<br />

mounted on a small Partenavia 68, which is perfectly suited for flying<br />

slowly just above the boundary layer. Here, nine flight tracks (4000 km)<br />

were flown in the Po-Valley, in particular around Milano.<br />

With different viewing angles, looking above and below the aircrafts,<br />

AMAXDOAS provides profile information of many trace gases e.g.: NO2,<br />

BrO, H2O, HCHO, O3, OClO, SO2.<br />

Here results of both campaigns will be presented.<br />

Fachvortrag UP 3.6 Mo 17:45 HS 118<br />

Disjunct Eddy Covariant flux measurements with PTR-<br />

MS during BEWA 2002 — •Wolfgang Grabmer 1 , Martin<br />

Graus 1 , Christian Lindinger 1 , Armin Wisthaler 1 , Armin<br />

Hansel 1 , Bernhard Rappenglueck 2 , Dominik Steigner 2 ,<br />

Roos Zuurbier 2 , and Rainer Steinbrecher 2 — 1 Institut fuer<br />

Ionenphysik, Universitaet Innsbruck — 2 Institut fuer Meteorologie und<br />

Klimaforschung, Atmosphaerische Umweltforschung, FZ Karlsruhe,<br />

Garmisch-Partenkirchen<br />

A disjunct eddy covariance (DEC) measurement system, which determines<br />

the fluxes of biogenic volatile organic compounds (BVOCs) out<br />

of vegetation, has been tested in the field. In disjunct sampling, short<br />

separate samples are taken instead of continuously sampling the air as in<br />

traditional relaxed eddy accumulation (REA) and true eddy covariance<br />

systems. This method reduces the number of samples but allows more<br />

time to analyse them in order to gain higher measurement precision and<br />

accuracy. The disjunct eddy covariance system combined with PTR-MS<br />

analysis (proton transfer reaction mass spectrometry) was successfully<br />

deployed to measure monoterpene fluxes during the BEWA field campaign<br />

2002 at the Waldstein tower in the Bavarian Fichtelgebirge. The<br />

ability of the system to measure monoterpene fluxes above a Norway<br />

Spruce (Picea abies) forest was demonstrated by comparing successfully<br />

flux results obtained with the REA and enclosure approach at the same<br />

location.<br />

Fachvortrag UP 3.7 Mo 18:00 HS 118<br />

Lidar systems for 4-dimensional observations of atmospheric<br />

key parameters in development at University of Hohenheim —<br />

•Andreas Behrendt, Anna Petrova, Thorsten Schaberl, Max<br />

Shiler, Gerd Wagner, and Volker Wulfmeyer — Institut fuer<br />

Physik und Meteorologie, Universitaet Hohenheim<br />

The lidar activities at University of Hohenheim are based on a new<br />

Nd:YAG laser which emits a nearly Gaussian-shaped beam (M 2 ¡ 1.5) of<br />

100 W at 1064 nm with a repetition rate of 250 Hz. Frequency-doubling<br />

yields 50 W output power at 532 nm. We employ the 532-nm radiation for<br />

UP 4 Satelliten und Anwendungen I<br />

pumping a Ti:sapphire ring-resonator which will be used for water vapor<br />

measurements with the differential absorption lidar (DIAL) technique.<br />

In a second branch a Cr4+:YAG crystal is pumped with the 1064-nm<br />

radiation. Its eye-safe output of 1400 to 1500 nm will be used for monitoring<br />

aerosols and clouds; in a second step, we will explore the feasibility<br />

of water vapor DIAL measurements at 1480 nm. The 532 and 1064<br />

nm radiation is also used for lidar observations and, in the near future,<br />

frequency tripling will yield 355-nm radiation for simultaneous measurements<br />

of temperature, particle extinction, and particle backscattering<br />

with the rotational Raman technique. The high power of this combined<br />

transmitter and effective use of the received signals will allow scanning<br />

operation. As a result, it will be possible to observe the spatial structure<br />

of a highly interesting set of atmospheric key parameters with unprecedented<br />

spatial and temporal resolution.<br />

Fachvortrag UP 3.8 Mo 18:15 HS 118<br />

Carbon Monoxide Variability in the Northern and Southern<br />

Hemisphere Measured by High-Resolution Solar Absorption<br />

Spectroscopy — •Voltaire Velazco 1 , Justus Notholt 1 ,<br />

Thorsten Warneke 1 , Astrid Schultz 2 , and Otto Schrems 3 —<br />

1 Univesity of Bremen, Otto Hahn Allee 1, 28359 Bremen, Germany —<br />

2 Alfred Wegener Institute for Polar and Marine Research, Telegrafenberg<br />

A43 D14473 Potsdam, Germany — 3 Alfred Wegener Institute for Polar<br />

and Marine Research, Am Handelshafen 12, Bremerhaven, Germany<br />

Vertical profiles of atmospheric Carbon Monoxide (CO) have been retrieved<br />

from solar absorption FT-IR spectra measured at the NDSC station<br />

in Ny-Alesund, Spitsbergen (79N, 12E) and on board the German<br />

research vessel Polarstern. Results are presented from seven years of FT-<br />

IR measurements in Spitsbergen and from 5 different ship cruises in the<br />

Atlantic between 50N and 40S. CO enhancements due to biomass burning<br />

have been detected in the equatorial regions as well as in the Arctic.<br />

Other trace gases related to biomass burning have also been studied. The<br />

characterization of the profiles has been established by an information<br />

content analysis and an estimation of the error budgets.<br />

Fachvortrag UP 3.9 Mo 18:30 HS 118<br />

Dekadische Ozonänderungen über der Nordatlantik-<br />

Europaregion — •Peters Dieter, Günter Entzian, and<br />

Gerhard Schmitz — Leibniz-Institut für Atmosphärenphysik,<br />

Kühlungsborn, Mecklenburg<br />

In this study we extend our ozone investigation from the 1980s to the<br />

period from 1959 up to 2001. The results represent a first approximation<br />

of the decadal change of longitude-dependent ozone distribution which<br />

is unknown for the decades before the FGGE experiment was started<br />

in 1978-79. This was possible because the NCEP re-analyses data set<br />

(Kalnay et al., 1996, upgrades) cover this period. With the help of a linear<br />

transport model for large-scale waves of ozone (Peters et al., 1996) we<br />

were able to calculate the decadal ozone changes for all 4 decades. The<br />

zonal mean ozone distribution was fixed to January 1979 after McPeters<br />

et al. (1989) to study only the result of wave structure changes. We estimated<br />

a 3-dimensional distribution of ozone change up to 10hPa (about<br />

30km) but here we focus only on total ozone changes.<br />

Zeit: Montag 14:15–16:00 Raum: HS 225<br />

Fachvortrag UP 4.1 Mo 14:15 HS 225<br />

Abschätzung anthropogener NOx–Emissionen mit Hilfe von Satellitendaten<br />

— •Nicola Toenges-Schuller, Olaf Stein und<br />

Franz Rohrer — ICG-II, Forschungszentrum Jülich, 52425 Jülich<br />

Stickoxide (NOx) spielen eine wichtige Rolle in der Chemie der<br />

Atmosphäre. Ihre globale Verteilung wird mit Hilfe von Chemie–<br />

Transport–Modellen untersucht, die auf sogenannte Emissionskataster<br />

zurückgreifen. Weit verbreitet ist die EDGAR–Datenbank, deren<br />

Abschätzung für anthropogene Quellen auf Wirtschaftsdaten der<br />

153<br />

einzelnen Länder basiert.<br />

Wir schätzen mit Hilfe von Satellitendaten unabhängig von EDGAR<br />

verschiedene NOx–Quellen hinsichtlich ihres relativen Beitrags und ihrer<br />

geographischen Verteilung ab und vergleichen sie mit Messungen<br />

troposphärischer NO2–Säulendichten des GOME-Satelliteninstruments<br />

(Leue et al., IUP Heidelberg, Richter et al., IUP Bremen). Als Proxy für<br />

die anthropogenen Emissionen dienen uns kalibrierte Satellitenaufnahmen<br />

der Lichter der Welt bei Nacht (C. Elvidge, OLS, DMSP).<br />

Die aus den Lichtern gewonnene NOx–Quellverteilung korreliert<br />

räumlich mit den GOME–Säulendichten ebensogut wie die der EDGAR–

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