aktualisiertes pdf - DPG-Tagungen
aktualisiertes pdf - DPG-Tagungen
aktualisiertes pdf - DPG-Tagungen
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UP 17.3 Di 14:00 Schellingstr. 3<br />
On-line monitoring of VOCs at a high mountain site in the German<br />
Alps (Schneefernerhaus, Zugspitze) — •Gregor Simmer 1 ,<br />
Wolfgang Gramber 1 , Armin Wisthaler 1 , Martin Graus 1 , Ulrich<br />
Poeschl 2 , and Armin Hansel 1 — 1 Institute of Ion Physics,<br />
University of Innsbruck, Technikerstr. 25, A-6020 Innsbruck, Austria —<br />
2 Institute of Hydrochemistry, Technical University of Munich, Marchioninstr.<br />
17, D-81377 Munich, Germany<br />
In the frame of the Schneefernerhaus Aerosol and Reactive Nitrogen<br />
Experiment (SCAVEX) a Proton-Transfer-Reaction Mass Spectrometer<br />
was installed on the Environmental Research Station Schneefernerhaus<br />
(2650 m a.s.l.). The Schneefernerhaus is situated about 300 m below<br />
the peak of the Zugspitze in the German Alps. From 28th October 2002<br />
till 12th March 2003 the remotely operated PTR-MS instrument measured<br />
a series of volatile organic compounds (VOCs) including oxygenates<br />
(methanol, acetaldehyde, acetone, methyl ethyl ketone), aromatics (benzene,<br />
toluene, alkyl substituted benzenes) and the biomass burning tracer<br />
acetonitrile. PTR-MS measurements on high mountain sites can be used<br />
to identify air masses with very different chemical characteristics, which<br />
have originated in the planetary boundary layer or have undergone longrange<br />
transport in the free troposphere. First results will be presented.<br />
UP 17.4 Di 14:00 Schellingstr. 3<br />
AMAXDOAS TROPOSPHERIC NO2 MEASUREMENT ON<br />
FALCON — •Ping Wang 1 , Marco Bruns 1 , Andreas Richter 1 ,<br />
John P. Burrows 1 , Klaus-Peter Heue 2 , Irene Pundt 2 ,<br />
Thomas Wagner 2 , and Ulrich Platt 2 — 1 Institute of Environmental<br />
Physics, University of Bremen, Otto-Hahn-Allee 1, D-28359 Bremen,<br />
Germany — 2 Institute of Environmental Physics, University of Heidelberg,<br />
In Neuenheimer Feld 229, 69120 Heidelberg, Germany<br />
The AMAXDOAS instrument on the DLR Falcon participated in the<br />
SCIAVAL campaign in September 2002 and February, March 2003. The<br />
AMAXDOAS instrument is a UV/visible spectrometer observing scattered<br />
light in four different directions: zenith, nadir, zenith off-axis and<br />
nadir off-axis. From the spectra, columns can be retrieved for several trace<br />
gases including BrO, OClO, NO2, and O3 using the well known DOAS<br />
(Differential Optical Absorption Spectroscopy) method. Large NO2 column<br />
enhancements are measured in nadir direction over Europe during<br />
some flights in 2002 and 2003. In this presentation we will describe the<br />
instrument and data analysis briefly. The NO2 slant columns are interpreted<br />
using fitting windows at different wavelengths and different viewing<br />
directions. Tropospheric NO2 AMFs are calculated with the radiative<br />
transport model SCIATRAN. Tropospheric NO2 vertical columns<br />
derived from the difference of zenith and nadir measurements will be<br />
presented and compared to measurements from the GOME and SCIA-<br />
MACHY satellite instruments.<br />
UP 17.5 Di 14:00 Schellingstr. 3<br />
Formaldehyde and other trace gases retrieved by MAX-DOAS<br />
— •Tiberiu Tarsu, Andreas Heckel, Andreas Richter,<br />
Folkard Wittrock, and John Burrows — Otto-Hahn-Allee 1,<br />
Universitaet Bremen, D-28359 Bremen<br />
The FORMAT (Formaldehyde as a tracer of oxidation in the troposphere)<br />
project represented an opportunity for the newly-developed concept<br />
of Multi Axis DOAS (MAX-DOAS) to determine volume mixing<br />
ratios in the lower troposphere. Tropospheric levels of several trace gases<br />
(HCHO, NO2 and O4) were investigated in the near-UV spectral region,<br />
employing zenith observations and four off-axis elevation angles close to<br />
the horizon. Atmospheric measurements were performed during two campaigns<br />
(summer 2002 and fall 2003) in the Po Valley (Northern Italy),<br />
a highly polluted, densely populated region, typical for midlatitudes ur-<br />
UP 18 Poster: Aerosol und Messtechnik<br />
ban areas. The results show that significant levels of HCHO and NO2<br />
were present during the campaigns despite unusual weather conditions:<br />
holiday time (in 2002) and showers which prevented the accumulation of<br />
high atmospheric concentrations during both periods. For the days with<br />
clear sky conditions, slant columns of good quality can be retrieved. In<br />
order to calculate vertical columns realistic air mass factors have to be<br />
computed. Their quality is verified by comparing O4 columns for different<br />
elevation angles. Results indicate the presence of HCHO in the whole<br />
area, providing a picture of the horizontal and temporal distribution.<br />
UP 17.6 Di 14:00 Schellingstr. 3<br />
Simulation of a Direct Detection Doppler Wind LIDAR for the<br />
ADM — •Ulrike Paffrath 1 , Ines Leike 2 , Oliver Reitebuch 1<br />
und Juergen Streicher 1 — 1 DLR 82230 Wessling — 2 Physiks Solutions<br />
Woertherstr. 2a 85457 Woerth<br />
The ” Atmospheric Dynamic Mission” ADM by ESA (European Space<br />
Agency) is the first mission worldwide to provide global atmospheric wind<br />
profiles by applying a Doppler wind LIDAR (Light Detection And Ranging)<br />
at a wavelength of 355 nm. This unit will be evaluated as an airborne<br />
system by DLR and it is essential to validate the complete system<br />
beforehand by a simulator.<br />
The transmitter is a pulsed, tripled Nd:YAG laser with a pulse repetition<br />
rate of 100 Hz. The receiver unit includes a detector for the Mie<br />
aerosol backscatter with a multi channel Fizeau interferometer and one<br />
for the Rayleigh molecular backscatter with a double edge Fabry Perot<br />
interferometer.<br />
Simulations of Doppler wind LIDAR will address the assessment of<br />
different instrument parameters, the impact of wind and atmospheric<br />
structures, the improvement of the data processing algorithms, the correlations<br />
between aerosol respectively molecular backscatter and atmospheric<br />
dynamics, cloud properties and calibration and monitoring using<br />
natural targets. All of these factors must be taken into account when<br />
predicting the performance of a Doppler wind LIDAR using a simulator<br />
and ultimately the impact of the measurements on climate studies and<br />
numerical weather prediction<br />
UP 17.7 Di 14:00 Schellingstr. 3<br />
Airborne microwave observations of stratospheric trace gases<br />
during SCIAMACHY validation campaigns — •Jayanarayanan<br />
Kuttippurath, Holger Bremer, Armin Kleinboehl, Harry<br />
Kuellmann, and Klaus Kuenzi — Institute of Environmental<br />
Physics, University of Bremen<br />
The Airborne Submillimeter Radiometer is a heterodyne sensor. It operates<br />
in a tuning frequency range of 604 GHz to 662 GHz and is equipped<br />
with two spectrometers namely, AOS and CTS. The AOS has a total<br />
bandwidth of 1.5 GHz, a resolution of 1.5 MHz and is used for probing<br />
stratospheric constituents. The sensor is operated onboard a high altitude<br />
research aircraft at an altitude of about 10-13 km in order to avoid<br />
signal absorption due to tropospheric water vapour. The sensor looks<br />
upward at a zenith angle of 78 deg., detects the thermal emissions from<br />
the rotational lines of various molecules. From the pressure broadening<br />
of the detected thermal lines, vertical profiles of volume mixing ratio are<br />
retrieved employing the Optimal Estimation Method. ASUR measures a<br />
range of stratospheric molecules like, Ozone, ClO, HCl, HNO3, N2O, etc.<br />
SCIA-VALUE 2002-03 is the validation campaigns performed onboard<br />
the DLR Falcon to validate SCIAMACHY data, which is a sensor onboard<br />
ESA’s ENVISAT satellite. A latitude band spanned from the Arctic<br />
to tropics was covered during the campaign in two different seasons.<br />
In this presentation, an overview of the ASUR sensor, the campaign,<br />
the data set gathered and the first attempts for the validation of SCIA-<br />
MACHY data will be presented.<br />
Zeit: Dienstag 14:00–16:00 Raum: Schellingstr. 3<br />
UP 18.1 Di 14:00 Schellingstr. 3<br />
Ice–supersaturated regions — •Peter Spichtinger and Klaus<br />
Gierens — Deutsches Zentrum für Luft- und Raumfahrt, Institut für<br />
Physik der Atmosphäre, Oberpfaffenhofen, Germany<br />
Cirrus clouds, including sub–species as condensation trails and subvisible<br />
cirrus, constitute now a well established research topic within the<br />
atmospheric sciences. But their formation regions, i.e. ice–supersaturated<br />
164<br />
air masses, are still not very well characterised. There is now direct evidence,<br />
that ice–supersaturation is frequent in upper tropospheric clear air<br />
and that it does even occur in the lowermost stratosphere. Such regions<br />
have been termed ice–supersaturated regions (ISSRs,<br />
[1] Gierens et al., Ann. Geophys. 17, 1218–1226, 1999<br />
). In the last three years we have evaluated various data sets (aircraft –<br />
MOZAIC, satellite – MLS, radiosondes) and could answer some questions