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aktualisiertes pdf - DPG-Tagungen

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UP 12.7 Di 14:00 Schellingstr. 3<br />

Water Vapour Column Retrieval from SCIAMACHY —<br />

•Stefan Noël, Michael Buchwitz, John P. Burrows, and<br />

Kai-Uwe Eichmann — Institute of Environmental Physics/Remote<br />

Sensing, University of Bremen, Germany<br />

Global water vapour column amounts have been derived from measurements<br />

of the SCanning Imaging Absorption spectroMeter for Atmospheric<br />

CHartographY (SCIAMACHY) on the European environmental<br />

satellite ENVISAT. For this purpose, the Air Mass Corrected Differential<br />

Absorption Spectroscopy (AMC-DOAS) approach, which was originally<br />

designed for GOME, has been applied to SCIAMACHY’s nadir measurements<br />

in the near-visible spectral region around 700 nm. The resulting<br />

SCIAMACHY total water vapour columns are compared with corresponding<br />

SSM/I and ECMWF water vapour data. Taking into account<br />

a systematic offset of about 10%, which may be related to the presence<br />

of clouds, the SCIAMACHY water vapour results agree well with these<br />

correlative data not only over ocean but also over land, thus showing the<br />

capability of SCIAMACHY to derive water vapour concentrations on the<br />

global scale.<br />

UP 12.8 Di 14:00 Schellingstr. 3<br />

First near global measurements of stratospheric BrO and<br />

comparison with model results — •NINAD SHEODE 1 ,<br />

BJOERN-MARTIN SINNHUBER 2 , ALEXEJ ROZANOV 3 ,<br />

and JOHN BURROWS 4 — 1 nsheode@iup.physik.uni-bremen.de —<br />

2 bms@iup.physik.uni-bremen.de — 3 alexej@iup.physik.uni-bremen.de<br />

— 4 burrows@iup.physik.uni-bremen.de<br />

Bromine species play an important role in the stratospheric ozone depletion,<br />

both at high latitudes and at mid-latitudes. However, inspite<br />

of its importance, there exist only very few measurements of bromine<br />

species in the stratosphere so far. Here we present the first near-global<br />

measurements of stratospheric bromine monoxide (BrO) from the SCIA-<br />

MACHY instrument on board the ENVISAT satellite. The measurements<br />

are compared with calculations from a chemical model in order to test<br />

our current understanding of the stratospheric bromine chemistry.<br />

UP 12.9 Di 14:00 Schellingstr. 3<br />

Occultation Measurements with SCIAMACHY: First Results<br />

and Validation — •Leonard Amekudzi, Bettina Hoffmann, Jerome<br />

Meyer, Alexei Rozanov, Heinrich Bovensmann und John<br />

P. Burrows — Institut für Umweltphysik - Universität Bremen<br />

UP 13 Poster: Aerosol und Mensch<br />

SCIAMACHY (SCanning Imaging Absorption spectroMeter for Atmospheric<br />

CHartographY) has successfully been launched onboard ENVI-<br />

SAT (ENVIronmental SATellite) in March 2002. It measures scattered,<br />

reflected, and direct radiation in the UV-Vis-IR range in three different<br />

viewing geometries (nadir, limb, and solar/lunar occultation). The focus<br />

of this presentation is on first solar and lunar occultation results.<br />

Height resolved concentration profiles of O3 and NO2 are derived from<br />

the occultation data as a standard product. First validations for these<br />

species have been carried out successfully. Furthermore, first vertical<br />

concentration profiles of NO3 have been retrieved from lunar occultation<br />

measurements and will be presented. The retrieval algorithm is based on<br />

the optimal estimation method. It is specialised on the spectral fitting of<br />

differential structures of radiation transmitted through the atmosphere.<br />

UP 12.10 Di 14:00 Schellingstr. 3<br />

Cloud effects in SCIAMACHY tropospheric NO2 — •Andreas<br />

Richter, Hendrik Nüß, Bernd Sierk, and John P. Burrows<br />

— Institut für Umweltphysik, Universität Bremen, Otto-Hahn-Allee, D-<br />

28359 Bremen<br />

The SCIAMACHY instrument on ENVISAT provides amongst other<br />

quantities accurate nadir measurements of the UV/visible radiances scattered<br />

back from the atmosphere. From these measurements, tropospheric<br />

columns of NO2 can be retrieved using the well known DOAS method<br />

and some assumptions on the stratospheric NO2 fields.<br />

Most of the tropospheric NO2 is located close to the surface as - with<br />

the exception of lightning - the sources are at the ground and the lifetime<br />

of NO2 is short. Thus, one would expect to see a clear reduction in tropospheric<br />

NO2 signal in the presence of clouds, and in fact this is observed<br />

in many cases. However, there are also numerous situations where large<br />

signals are observed over cloud covered pixels, often linked to weather<br />

fronts and transport events.<br />

In this study, the effects of clouds on tropospheric NO2 columns derived<br />

from SCIAMACHY measurements are evaluated and possible explanations<br />

discussed. In addition, measurements form the GOME instrument<br />

on ERS-2 are used to check if the findings are consistent with those from<br />

the long GOME time series available, and in howfar they depend on the<br />

size of the ground-pixels of the measurements.<br />

Zeit: Dienstag 14:00–16:00 Raum: Schellingstr. 3<br />

UP 13.1 Di 14:00 Schellingstr. 3<br />

Mass Spectrometric Aerosol Composition Measurements in<br />

the Free Troposphere — •Johannes Schneider 1 , Joachim Curtius<br />

2 , Frank Drewnick 1 , Silke Henseler 1 , Nele Hock 1 , Silke<br />

Weimer 1 , and Stephan Borrmann 1,2 — 1 Abt. Wolkenphysik und -<br />

chemie, Max-Planck-Institut für Chemie, Mainz — 2 Institut für Physik<br />

der Atmosphäre, Johannes Gutenberg-Universität Mainz<br />

Aircraft based measurements of the chemical composition of aerosol<br />

particles in the mid-latitude tropopause region have been performed using<br />

the Aerodyne Aerosol Mass Spectrometer (AMS). The AMS detects<br />

particles in the size range between 50 and 1500 nm and measures quantitatively<br />

the mass concentrations and size distributions of ammonium,<br />

nitrate, sulfate, and organics. The aircraft measurements were part of<br />

the research project PAZI (Particles From Aircraft: Impact on Cirrus<br />

Clouds and Climate), which is funded by the German HGF (Hermann<br />

von Helmholtz-Gemeinschaft Deutscher Forschungszentren) research organization.<br />

The main objective of this project is to investigate the relationship<br />

between aircraft exhaust particles and the formation of cirrus<br />

clouds. The measurements took place in Southern Germany using the<br />

twin-jet research aircraft ”Falcon” of the DLR (Deutsches Zentrum fuer<br />

Luft- und Raumfahrt). The measurement flights included sampling in<br />

aged aircraft exhaust as well as background flights in regions with little<br />

air traffic, at altitudes between 8000 and 12000 m, representing the<br />

mid-latitude upper troposphere. Here we present first results like size<br />

distributions and vertical profiles.<br />

161<br />

UP 13.2 Di 14:00 Schellingstr. 3<br />

Sedimentationsgeschwindigkeit realer Staubpartikel —<br />

•Gregor Schmitt 1,2 , Oliver Wallenfang 2 , Bernd Diekmann 1<br />

und Wolfgang Büscher 2 — 1 Universität Bonn, Physikalisches<br />

Institut, Nußallee 12, 53115 Bonn — 2 Universität Bonn, Institut für<br />

Landtechnik, Nußallee 5, 53115 Bonn<br />

In der Tierhaltung treten nicht zu unterschätzende Bioaerosolkonzentrationen<br />

(Staub und Mikroorganismen) auf, deren Auswirkungen auf<br />

Mensch und Tier bislang nur in Ansätzen untersucht worden sind. Daher<br />

stellen sich vermehrt Fragen bezüglich der Ausbreitung von Bioaerosolen.<br />

Am Institut für Landtechnik der Universität Bonn wird ein computergestütztes<br />

Modell zur Ausbreitungsberechnung von Partikeln erstellt.<br />

Staubspezifische Eigenschaften wie z.B. die Sedimentationsgeschwindigkeit<br />

werden in der Regel in Modellen auf Partikel einer definierten Dichte<br />

eingegrenzt. Untersuchungen am Institut für Landtechnik haben gezeigt,<br />

dass die Staubzusammensetzung bei einer Tierart in verschiedenen Haltungsformen<br />

bereits so stark differiert, dass eine Einteilung der Partikel<br />

in verschiedene Größenfraktionen notwendig ist, um eine korrekte Modellierung<br />

der Staubausbreitung vornehmen zu können. In dieser Posterpräsentation<br />

wird eine Methode zur empirischen Bestimmung der Sedimentationsgeschwindigkeit<br />

sowie die Berechnung der Dichte und Masse<br />

von Partikeln vorgestellt und diskutiert. Das Poster ergänzt den Hauptvortrag<br />

”Modellierung und Detektion von Geruch und Staub” von O.<br />

Wallenfang.

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