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Plenarvorträge - DPG-Tagungen

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Magnetismus Mittwoch<br />

MA 15.5 Mi 16:15 H10<br />

Thickness and temperature driven Spin Reorientation Transition<br />

in ultrathin Co films on Pd(110) — •L. Yan, Y. Lu,<br />

H. Meyerheim, M. Przybylski, W. Wang, J. Barthel, and J.<br />

Kirschner — Max-Planck-Institut für Mikrostrukturphysik, Weinberg<br />

2, 06120 Halle<br />

Morphology, structure and magnetism of ultrathin Co films (0.1 to<br />

3ML) grown epitaxially on Pd(110) at room temperature (RT) were studied.<br />

The elongated Co stripes resulting from the anisotropy of Pd(110)<br />

surface are observed by STM. These Co stripes become ferromagnetic<br />

above 0.2ML at low temperature (LT=80K), and are magnetized outof-plane.<br />

Between 0.5ML and 1.1ML, the polar MOKE signal (measured<br />

in remanence) decreases with increasing Co coverage. The magnetization<br />

rotates towards the film plane showing an increasing longitudinal<br />

component to the total Kerr signal. With further increasing coverage,<br />

another spin reorientation transition occurs. At the thickness of about<br />

2ML the film magnetization is again oriented out-of-plane at LT. However,<br />

with increasing temperature the magnetization rotates towards the<br />

film plane and no polar MOKE signal is detected at RT. The films are<br />

magnetized in-plane independently of the temperature above a thickness<br />

of about 2.7ML. We suggest that such magnetic behaviors are attributed<br />

to the morphology and structural reconstruction which the film experiences<br />

with increasing thickness.<br />

MA 15.6 Mi 16:30 H10<br />

Prinzipielle Unterschiede bei Ni/Pd-Grenzflächen — •Y.<br />

Manzhur 1 , K. Potzger 1 , M. J. Prandolini 1 , H. H. Bertschat<br />

1 und Mark Dietrich 2 — 1 Hahn-Meitner-Institut, Bereich<br />

Festkörperphysik, Glienicker Strasse 100, 14109 Berlin — 2 Mark<br />

Dietrich, ISOLDE-Collaboration, EP Division, CERN, CH 1211 Genf<br />

Ni/Pd-Grenzflächen können u. a. durch Aufdampfen von Pd auf Ni-<br />

Einkristallen erzeugt werden oder durch Aufdampfen von Ni auf Pd-<br />

Einkristallen. Pd auf Ni ist ein häufiger studiertes System und wurde<br />

auch von uns mit der PAC-Spektroskopie unter Verwendung von radioaktiven<br />

Proben untersucht [1]. Das mehrfach bestätigte Ergebnis ist, dass<br />

wenige Monolagen Pd auf Ni eine ferromagnetische Ordnung annehmen.<br />

Dagegen gibt es neben der PAC so gut wie keine Experimentiermethode,<br />

um das magnetische Verhalten von Ni bedecktem Pd zu erforschen. In<br />

einen früheren Experiment [2] fanden wir, dass in Pd einige Atomlagen<br />

von der Grenzfläche entfernt induzierte magnetische Wechselwirkungen<br />

nachzuweisen sind, Pd aber paramagnetisch bleibt. Nun konnten wir zeigen,<br />

dass auch die oberste Pd-Atomlage des Einkristalls, die sich in direktem<br />

Kontakt zu Ni befindet, keine ferromagnetische Ordnung annimmt,<br />

im Kontrast zu dünnem Pd auf Ni.<br />

Die Messungen wurden am Massenseparator ISOLDE / CERN durchgeführt.<br />

[1] Phys. Rev. Lett. 80, 2721 (1998).<br />

[2] Phys. Rev. Lett. 78, 342 (1997).<br />

MA 15.7 Mi 16:45 H10<br />

Spin-Polarisation von EuS oberhalb 77 K: Temperaturabhängige<br />

MOKE- und XMCD-Messungen an dünnen<br />

Co/EuS-Vielfachlagen-Filmen — •C. Müller, H. Lippitz, J.J.<br />

Paggel und P. Fumagalli — Institut für Experimentalphysik, Freie<br />

Universität Berlin, Arnimallee 14, 14195 Berlin<br />

Sein großes Spin-Moment (mS = 7/2) macht den Halbleiter EuS interessant<br />

für Spintronics-Anwendungen. Demgegenüber steht die niedrige<br />

Curie-Temperatur (TC=16.5 K), die eine kommerzielle Nutzung<br />

ausschließt. Messungen des magnetischen Röntgen-Circulardichroismus<br />

(X-MCD) an Vielfachlagen von Co und EuS zeigen eine Spin-Polarisation<br />

von EuS bei einer Temperatur größer als 77 K. Als Ursache wird eine<br />

antiferromagnetische Kopplung zwischen Co und EuS festgestellt, d.h.<br />

die Polarisation des EuS wird durch das Co induziert. Tieftemperatur-<br />

Messungen (10 K) des magnetooptischen Kerr-Effektes (MOKE) können<br />

dies bestätigen: Nichtlinearitäten in Hysterese-Kurven werden durch<br />

einen solchen Kopplungs-Effekt erklärt. Bei Raumtemperatur liefern<br />

MOKE-Messungen keinen eindeutigen Nachweis für die Existenz einer<br />

antiferromagnetischen Kopplung.<br />

Diese Arbeit wurde unterstützt durch die Deutsche Forschungsgemeinschaft<br />

im Rahmen des SFB 290.<br />

MA 15.8 Mi 17:00 H10<br />

Pulsed Laser Deposition of Epitaxial SmCo Thin films — •A.<br />

Singh 1 , R. Tamm 2 , V. Neu 1 , S. Leinert 1 , S. Fähler 1 , C.-G. Oertel<br />

2 , W. Skrotzki 2 , L. Schultz 1 , and B. Holzapfel 1 — 1 IFW<br />

Dresden, Helmholtzstr. 20, 01069 Dresden — 2 Inst. f. Strukturphysik,<br />

TU Dresden, 01062 Dresden<br />

To explore the potential of a permanent magnetic material with uniaxial<br />

anisotropy, a well aligned easy magnetisation axis is required. One way<br />

to achieve this is by growing epitaxial films on single crystal substrates.<br />

With the same aim and motivation of achieving high coercivity and remanance<br />

along a crystallographic direction, epitaxial SmCo on Cr buffered<br />

(100) and (110) MgO single crystal substrates was deposited. These films<br />

were prepared using PLD from elemental targets, and showed the epitaxial<br />

relation: MgO(001)[100]-Cr(001)[110]-SmCo(110)[001], which indicates<br />

an in plane direction of the easy axis. But besides this the easy axis<br />

also shows a 60 ◦ out of plane component coming from a (1 1 16) texture.<br />

These results have been reached at by careful analysis of several pole figures<br />

measured in the texture goniometer and magnetic measurements in<br />

the SQUID. The volume fractions of these two texture components show<br />

a strong dependence on the deposition temperature. The exact contributions<br />

of these two components will be discussed in relation to the results<br />

from magnetic properties.<br />

MA 15.9 Mi 17:15 H10<br />

Magnetic microstructure of granular epitaxial NdFeB films —<br />

•V. Neu, S. Melcher, U. Hannemann, and S. Fähler — IFW<br />

Dresden, Helmholtzstr. 20, 01069 Dresden<br />

Epitaxial NdFeB films combine a perfect alignment of the easy magnetic<br />

axis perpendicular to the substrate with a high coercivity up to 2<br />

T [1]. They possess high nucleation fields and the coercivity is mainly<br />

limited by local stray fields. Furthermore they grow in isolated, rectangular<br />

grains, which makes these films an ideal system to locally study<br />

the magnetic domains of a self-organized microstructure.<br />

In this paper we used Magnetic Force Microscopy (MFM) and global<br />

magnetization measurements to examine a series of Nd-rich NdFeB films<br />

deposited at different temperatures. At deposition temperatures around<br />

545 ◦ C the films neither have a perfect degree of texture nor do they switch<br />

homogeneously. The microstructure consists of a small grained film of Nd-<br />

FeB with the Nd-rich phase segregated as large spherical grains. At the<br />

optimum temperature of 630 ◦ C uniform switching occurs and a coercivity<br />

of 2 T is obtained. These films consist of rectangular, µm-sized NdFeB<br />

grains, which show typical stripe domains with an average width of 150<br />

nm. At higher temperatures (670 ◦ C) the grain size distribution broadens<br />

significantly. This is reflected in a less uniform switching behavior, which<br />

is observed with global and local measurement techniques.<br />

[1] U. Hannemann, S. Fähler, V. Neu, B. Holzapfel, L. Schultz, Appl.<br />

Phys. Lett. 82, 3710 (2003)<br />

MA 15.10 Mi 17:30 H10<br />

Highly coercive and highly remanent Nd-Fe-B films —<br />

•Sebastian Fähler, Jörg Buschbeck, Ah-Ram Kwon, Ullrich<br />

Hannemann, Volker Neu, Bernhard Holzapfel, and Ludwig<br />

Schultz — IFW Dresden, Helmholtzstr. 20, 01069 Dresden and SFB<br />

463<br />

Miniaturised magnets with high remanences are needed for microelectromechanical<br />

systems (MEMS). A possible solution is epitaxially<br />

grown Nd2Fe14B films which exhibit due to the perfect alignment of the<br />

c-axis (easy magnetisation direction) very high remanence to saturation<br />

magnetisation ratios close to unity. Furthermore these films reach coercivities<br />

up to 2 T [1]. Films, which were deposited at lower temperatures<br />

and subsequently annealed at higher temperatures, show similar results<br />

despite the different temperature treatment [2]. One result of the different<br />

temperature treatment is a change in the morphology of the films,<br />

which consists of isolated grains for the epitaxial films or appears continuous<br />

for the post-deposition annealed films. We present a study of the<br />

effect of the 2 different deposition conditions on the microstructure and<br />

consequently on the magnetic properties of the films.<br />

[1] U.Hannemann, S. Fähler, V. Neu, B. Holzapfel, L.Schultz, Appl.<br />

Phys. Lett. 82 (2003) 3710<br />

[2] L.K.E.B Serrona, A. Sugimura, N. Adachi et al., Appl. Phys. Lett.<br />

82 (2003) 1751

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