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Tiefe Temperaturen Dienstag TT 13.10 Di 18:30 H20 Measurements of coherent transition radiation by Hilberttransform spectroscopy with Josephson junctions — •Andre Kaestner 1 , Frank Ludwig 2 , Frank Ludwig 1 , and Meinhard Schilling 1 — 1 Institut für elektrische Messtechnik und Grundlagen der Elektrotechnik, TU Braunschweig, Hans-Sommer-Straße 66, D-38106 Braunschweig — 2 Deutsches-Elektronen-Synchrotron DESY, Notkestraße 85, D-22603 Hamburg We present measurements of coherent transition radiation from 50 to 500 GHz using the method of Hilbert-transform spectroscopy. The Josephson junctions out of YBa2Cu3O7 (YBCO) used for Hilberttransform spectroscopy are prepared on symmetric 24 o LaAlO3 bicrystal substrates. For better coupling of high frequency radiation they are equiped with integrated wideband antennas out of YBCO. We obtain for a 6 micrometer wide junction an ICRN-product of 170 microvolt at 77 K and 2.0 millivolt at 10 K. The set-up is optimized for low insertion loss over a wide frequency range from 50 GHz to 2 THz. The measurements of coherent transition radiation are compared with similar measurements done at the Tesla Test Facility for the same set-up. TT 14 FV-internes Symposium ”Orbital Physics” Zeit: Dienstag 14:30–18:55 Raum: H18 Hauptvortrag TT 14.1 Di 14:30 H18 Lattice instability of frustrated orbital and spin systems — •Maxim Mostovoy — Materials Science Center, University of Groningen, The Netherlands In materials with strong exchange interactions between electrons occupying degenerate orbitals the cooperative Jahn-Teller effect may be suppressed, as it is often impossible to order orbitals on all pairs of neighboring transition metal ions in a unique optimal way. This frustration may be relieved by several competing mechanisms, e.g., quantum orbital fluctuations or ‘Peierls-like’ lattice distortions. I will discuss similarities and differences between frustrated Jahn-Teller materials and frustrated spin systems, such as antiferromagnets with a pyrocholore and triangular lattice. Fachvortrag TT 14.2 Di 15:00 H18 Magnetism, Charge Order and Giant Magnetoresistance in SrFeO3−δ — •C. Ulrich 1 , A. Lebon 1 , P. Adler 2 , C. Bernhard 1 , A. Boris 1 , A. Pimenov 1 , A. Maljuk 1 , C.T. Lin 1 , and B. Keimer 1 — 1 Max-Planck-Institut FKF, Stuttgart — 2 Institut für Anorganische Chemie, Universität Karlsruhe The relationship between spin ordering, charge ordering, and magneto– transport effects has recently received much attention in the context of the colossal magnetoresistance (CMR) phenomenon in manganites. In the 3D perovskite SrFeO3, Fe 4+ is isoelectric to the Jahn–Teller ion Mn 3+ in the manganite system. However, while the parent compound of the CMR manganites, LaMnO3, is insulating and shows a cooperative Jahn–Teller effect, its analogue SrFeO3 remains metallic at all temperatures and exhibits a helical antiferromagnetic spin structure below 130 K. Therefore, SrFeO3 is right at the borderline between an itinerant and a strongly localized electron system. We have studies three single crystals of SrFeO3−δ with different oxygen content. Cubic SrFeO3.00 is metallic in the entire temperature range and shows a large negative magnetoresistance effect at 55 K. Tetragonal SrFeO2.87 shows semiconducting behavior below a second magnetic phase transition at 75 K. Our Mössbauer studies reveal that this phase transition is accompanied by a charge ordering of Fe 3.5+ into Fe 3+ and Fe 4+ . An orthorhombic sample SrFeO2.81 on the other side showed semiconducting behavior and a pronounced positive MR effect at 70 K. TT 14.3 Di 15:20 H18 Frustrated orbital ground state in thiospinels — •J. Hemberger, H.-A. Krug von Nidda, V. Fritsch, N. Büttgen, E.-W. Scheidt, P. Lunkenheimer, R. Fichtl, V. Tsurkan, and A. Loidl — Center for Electronic Correlations and Magnetism, Institute of Physics, University of Augsburg We studied the ground state properties of the normal cubic spinel compounds AB2S4 (A = Fe, Mn and B = Sc, Cr) by means of specific heat, magnetization and susceptibility measurements, as well as dielectric and optical spectroscopy. In all compounds frustration strongly influences the interplay of orbital and magnetic degrees of freedom and corresponding order phenomena. Our results indicate the existence of distinguished spinorbital scenarios: In the case of nonmagnetic B-sites (Sc) we find strong magnetic coupling (Curie-Weiss temperature θCW = −45 K for A = Fe) without any indications of order down to 50 mK. The ground states of these compounds have to be characterized as a spin liquid in MnSc2S4 and a spin-orbital liquid in FeSc2S4, where Fe 2+ is Jahn-Teller active but orbitally frustrated. In the case of magnetic B-sites (Cr) spin-order is induced and the low-temperature states have to be described as orbital liquid, orbital glass, or finally orbital order. TT 14.4 Di 15:35 H18 Isotropic spin waves in the paramagnetic spin liquid state of FeSc2S4 — •Alexander Krimmel 1 , Vladimir Tsurkan 1 , Alois Loidl 1 , Michael Mücksch 1,2 , and Marek Koza 2 — 1 Institut für Physik, Univ. Augsburg, D-86159 Augsburg, Germany — 2 Institut Laue Langevin, BP156, 38042 Grenoble Cedex 9, France FeSc2S4 crystallizes in the normal cubic spinel structure with magnetic Fe 2+ ions (3d 6 , high spin configuration, µeff = 5.12µB) on the A-site. The Jahn-Teller ions Fe 2+ are orbitally frustrated. Specific heat and magnetic measurements showed no signs of long range magnetic order down to 50 mK. The ground state properties of FeSc2S4 can be described by a spinorbit liquid. Here we report on inelastic neutron scattering experiments on polycrystalline FeSc2S4. Even at 80 K, the paramagnetic spectral response is centered around 0.6 ˚A −1 corresponding to the antiferromagnetic Bragg position. On cooling, a well defined isotropic magnon dispersion evolves but the system remains in a cooperative paramagnetic state without magnetic Bragg peaks. These results are discussed within a scenario of collective magnetic excitations in an orbital liquid state. TT 14.5 Di 15:50 H18 Orbital degree of freedom in manganites determined by O1s and Mn2p NEXAFS: crystal field versus orbital coupling in single-layered La1−xSr1+xMnO4 — •Michael Merz 1 , P. Reutler 2 , B. Büchner 2 , Y. U. Idzerda 3 , S. Tokumitsu 4 , N. Nücker 4 , and S. Schuppler 4 — 1 Institut für Kristallographie, RWTH Aachen — 2 Institut für Festkörper- und Werkstoffforschung, Dresden — 3 Naval Research Laboratory, Washington — 4 Forschungszentrum Karlsruhe, Institut für Festkörperphysik Manganites exhibit a manifold of highly interesting magnetic and electronic phases, with charge- and orbital-ordered states being at the center of interest. Especially single-layered La1−xSr1+xMnO4 is a prototypical example for such ordering effects. For this compound a ferro-orbital ordering of |3z2 − r2 > states is expected from the strong crystal field, yet anti-ferro type orbital coupling might lead to an admixture of |x2 −y2 > states. Using polarization-dependent O1s and Mn2p near-edge x-ray absorption spectroscopy on untwinned La1−xSr1+xMnO4 single crystals (0 ≤ x ≤ 0.5), the doping- and temperature-dependent occupancies of the O2p and Mn3d orbitals were studied. According to the spectra, Sr doping not only provides holes to the system but also induces a continuous transfer of electrons from out-of-plane |3z2−r2 > to in-plane |3x2−r2 > and |3y2 − r2 > states. The data clearly demonstrate that electrons reside for all doping levels on mixed α|3z2 − r2 > +β|x2 − y2 > states, i. e., antiferro-coupled canted orbitals where α and β strongly depend on the Sr content. TT 14.6 Di 16:05 H18 Magnetische Polaronen: Magnetismus der dotierten Schichtmanganate La1−xSr1+xMnO4 (x=1/8) — Davide Cattani 1 , Christoph Baumann 2,1 , Pascal Reutler 2 , •Rüdiger Klingeler 2 , Alexandre Revcolevschi 3 und Bernd Büchner 2 — 1 Università di Parma, I-43100 Parma — 2 Leibniz-Institut für Festkörperund Werkstoffforschung Dresden, PF 270116, D-01171 Dresden — 3 Laboratoire de Chimie des Solides, Université Paris-Sud, F-91405 Orsay Cedex In den einfach geschichteten Manganaten La1−xSr1+xMnO4 zeigen Messungen der thermischen Ausdehnung im Fall lochfreier (x=0) oder gering dotierter Systeme (x=1/8) eine grosse, stark anisotrope magnetoelastische Kopplung beim Einsetzen der langreichweitig antiferromagne-
Tiefe Temperaturen Dienstag tisch geordneten Tieftemperaturphase. Darüber hinaus ergeben sich Belege für eine temperaturabhängige Umbesetzung der Orbitale. Eine geringe Dotierung (x=1/8) mit Löchern, d.h. das Einschalten von konkurrierenden ferromagnetischen Doppelaustauschwechselwirkungen, verringert die Stabilität der antiferromagnetischen Tieftemperaturphase. Dabei zeigen Messungen der Magnetisierung das Auftreten zusätzlicher xy-artiger magnetischer Momente in der geordneten Phase, die als stark anisotrope magnetische Polaronen verstanden werden können. TT 14.7 Di 16:20 H18 Bond centered vs. site-centered charge ordering and ferroelectricity in oxides. — •Dmitry Efremov 1 , Jeroen van den Brink 2 , and Daniel Khomskii 3 — 1 Technische Universität Dresden, Institut für Theoretische Physik, 01062 Dresden — 2 Institut-Lorentz for Theoretical Physics, Universiteit Leiden, 2300 RA Leiden, The Netherlands — 3 Universität zu Köln, 50937 Köln Many transition metal oxides show charge ordering, which up to now was always treated as alternation of valency of transition metal ions. We show that besides this site-centered charge ordering there may exist another type of charge and orbital ordering, namely bond-centered ordering. We demonstrate that such type of ordering should exist in manganites close to half-filling. Moreover we show that these two types of ordering may coexist making the system ferroelectric. 16:35 Pause Hauptvortrag TT 14.8 Di 16:50 H18 Resonant Soft Energy X-ray Diffraction of Charge, Spin and Orbital Ordering — •Peter Hatton — Dept. of Physics, University of Durham, UK Soft x-ray resonant diffraction is a new technique pioneered by our group. We have published examples of the huge resonant enhancements of charge and magnetic scattering that can be obtained at the L-edges of 3d transition metal oxides as well as the first direct observation of orbital ordering. In this talk we will review the technique of soft x-ray diffraction as well as giving recent examples of results In particular we will report the first resonant soft x-ray scattering observations of orbital ordering from a bulk single crystal. We have studied the low temperature phase of La1.5Sr0.5MnO4 that displays charge, spin and orbital ordering. Previous claims of orbital ordering in such materials have relied on observations at the K edge. These claims have attracted a barrage of controversy from theoretical studies. Instead we have employed resonant soft x-ray scattering at the manganese LIII and LII edges which provides a direct measurement of the orbital ordering. Energy scans at constant wavevector have been compared to theoretical predictions and show that at all temperatures there are two separate contributions to the observed scattering, direct Goodenough orbital ordering and strong cooperative Jahn-Teller distortions of the Mn 3+ ions. Fachvortrag TT 14.9 Di 17:20 H18 The interplay of orbital and lattice degrees of freedom in titanates — •M. Grüninger, R. Rückamp, A. Gößling, M. Cwik, H. Roth, J. Baier, M. Kriener, T. Lorenz, M. Braden, and A. Freimuth — II. Physikalisches Institut, Universität zu Köln, Germany Recently, several interesting phenomena have been proposed in which orbitals play a key role, e.g. orbital order, dispersing orbital waves or orbital liquids. However, the driving force in most theoretical treatments is based on electronic interactions, the possible role of the lattice is often neglected. One interesting phenomenon which still has to be confirmed experimentally is the existence of orbital liquids. The pseudo-“cubic” d 1 antiferromagnet LaTiO3 seemed a promising candidate. We discuss the structure, the thermal expansion and the optical conductivity of LaTiO3 and of orbitally ordered YTiO3. A consistent description of the data of both compounds is obtained within a Jahn-Teller scenario. Orbital excitations are observed in the optical conductivity spectra of both LaTiO3 and YTiO3 at about 0.25eV, which is difficult to reconcile with an orbital liquid ground state of LaTiO3. On contrary, the data suggest that the coupling to the lattice is of dominant importance not only for eg systems, but also for t2g electrons. This point of view is corroborated by the optical conductivity data of TiOCl. There, the splitting of the t2g levels is larger than 0.5eV. TT 14.10 Di 17:40 H18 Spin-orbital physics in Raman and optical spectra of Mott insulators — •Giniyat Khaliullin — a:Max-Planck-Institut FKF, Heisenbergstr.1, 70569 Stuttgart We review our recent work which focuses on Raman [1] and optical [2] spectroscopy in Mott insulators. First, we discuss different Raman scattering channels involving orbital excitations in titanates. Next, we consider the spectral weights of optical transitions in titanates and cubic vanadates. We show that the temperature and polarization dependences of the Raman and optical spectra are directly determined by the underlying spin and orbital correlations, and discuss the role played by orbital quantum fluctuations. [1] G. Khaliullin, (unpublished). [2] G. Khaliullin, P. Horsch, and A.M. Ole´s, (unpublished). TT 14.11 Di 17:55 H18 Direct observation of charge order in La1.8Sr0.2NiO4 — •C. Schüßler-Langeheine 1 , J. Schlappa 1 , Z. Hu 1 , M. W. Haverkort 1 , M. Benomar 1 , O. Friedt 1 , E. Schierle 2 , H. Ott 2 , E. Weschke 2 , G. Kaindl 2 , G. A. Sawatsky 3 , A. Tanaka 4 , M. Braden 1 , and L. H. Tjeng 1 — 1 II. Physikalisches Institut, Universität zu Köln — 2 Institut für Experimentalphysik, Freie Universität Berlin — 3 Department of Physics and Astronomy, University of British Columbia, Vancouver, Canada — 4 ADSM, Hiroshima University, Japan We report on the direct observation of charge order in Sr-doped La2NiO4 using resonant soft x-ray scattering at the Ni L2,3 and La M4,5 resonances. Unlike conventional scattering techniques, which are essentially probing lattice modulations, resonant soft x-ray scattering is very sensitive to the oxidation state and hence particularly suited to study charge-order phenomena. The charge-order superstructure peak from La1.8Sr0.2NiO4 shows a resonant enhancement predominantly at Ni L2,3 edges, in contrast to the x-ray absorption signal, which is dominated by the La absorption. The details of this energy dependence agree well with charge order in the Ni system, providing a direct experimental observation of this ordered phase. Furthermore, the superstructure peak observed with resonant soft x-ray scattering is much narrower in momentum space than known from conventional scattering techniques, because the comparably short penetration depth of soft x-rays together with the availability of well focused x-ray beams makes this technique sensitive to slight local inhomogeneities of the doping level, which cannot be probed by other techniques. TT 14.12 Di 18:10 H18 Extended moment formation and magnetic ordering in the trigonal chain compound Ca3Co2O6 — •Volker Eyert 1 , Christian Laschinger 1 , Thilo Kopp 1 , and Raymond Frésard 2 — 1 Institut für Physik, Universität Augsburg, Germany — 2 Laboratoire Crismat, UMR CNRS-ENSICAEN (ISMRA) 6508, Caen, France The results of electronic structure calculations for the one-dimensional magnetic chain compound Ca3Co2O6 are presented. The calculations are based on density functional theory and the local density approximation and used the augmented spherical wave (ASW) method. Our results allow for deeper understanding of recent experimental findings. In particular, alternation of Co 3d low- and high-spin states along the characteristic chains is related to differences in the oxygen coordination at the inequivalent cobalt sites. Strong hybridization of the d states with the O 2p states lays ground for polarization of the latter and the formation of extended localized magnetic moments centered at the high-spin sites. In contrast, strong metal-metal overlap along the chains gives rise to intrachain ferromagnetic exchange coupling of the extended moments via the d 3z 2 −r 2 orbitals of the low-spin cobalt atoms. TT 14.13 Di 18:25 H18 Excitation spectrum of the cobaltite NaxCoO2 yH2O as function of Na content and hydration — •P. Lemmens 1,2 , K.-Y. Choi 2 , V. Gnezdilov 3 , N.N. Kovaleva 1 , H. Sakurai 4 , K. Takada 4 , T. Sasaki 4 , E. Takayama-Muromachi 4 , F.C. Chou 5 , C.T. Lin 1 , and B. Keimer 1 — 1 MPI for Solid State Research, D-70569 Stuttgart — 2 2. Phys. Inst., RWTH Aachen, D-52056 Aachen — 3 B.I. Verkin Inst. for Low Temp. Phys., NASU, 61164 Kharkov — 4 Superconducting Mat. Center and Advanced Mat. Lab., NIMS, Tsukuba, Ibaraki 305-0044 — 5 Center for Material Science and Engineering, MIT, Cambridge, MA 02139 We report on a Raman scattering study on the superconducting cobaltite NaxCoO2 yH2O as function of Na content and hydration
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Page 427 and 428: Ausschuss Industrie und Wirtschaft
Page 429 and 430: Arbeitskreis Biologische Physik Tag
Page 431 and 432: Arbeitskreis Biologische Physik Tag
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Arbeitskreis Biologische Physik Mon
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Arbeitskreis Biologische Physik Die
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Arbeitskreis Biologische Physik Don
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Arbeitskreis Biologische Physik Fre
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Arbeitskreis Physik sozio-ökonomis
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Symposium Fat-Tail Distributions -
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Symposium Life Sciences on the Nano
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Symposium Non-Fermi Liquids in Quan
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Symposium Functional Nanoparticles
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Symposium Organic and Hybrid System
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Symposium Physics of Foams Mittwoch
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Symposium Physics of Foams Mittwoch
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Symposium Quantum Shot Noise in Nan
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Symposium X-RAY Magneto-Optics Tage
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Symposium X-RAY Magneto-Optics Dien
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Lehrertage Regensburg Hauptvorträg
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A. D., Mirlin .................HL 1
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Breidenbach, Boris ........ AKB 50.
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Elli, Alexandra .............SYLS 3
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Greer, Lindsay ......... M 9.1, M 1
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Horn-von Hoegen, M. O 13.2, O 14.40
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Korn, Tobias ...............MA 13.6
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Martin, Tobias ............. MA 13.
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Partyka, Ewa ................ M 18.
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Rugeramigabo, Eddy Patrick O 14.38,
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Sihler, J. .................... DS
Page 539 and 540:
Volz, K. .................... HL 44
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