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Oberflächenphysik Montag<br />

O 12 Magnetismus in reduzierten Dimensionen<br />

Zeit: Montag 15:45–17:00 Raum: H45<br />

O 12.1 Mo 15:45 H45<br />

Magnetische Röntgenstreuung an lateral strukturierten<br />

Co/CoO Filmen — •Arndt Remhof, Johannes Grabis,<br />

Alexei Nefedov und Hartmut Zabel — Experimentalphysik/Festkörperphysik,<br />

Ruhr-Universität Bochum<br />

Nano- und Mikrostrukturierung von dünnen magnetischen Systemen<br />

ermöglicht das Ummagnetisierungsverhalten, d. h. die Hystereseschleife,<br />

gezielt zu verändern. Wir haben ein quadratisches Muster aus Co/CoO<br />

Inseln mittels Elektronenstrahl-Lithographie hergestellt. Die Inseln haben<br />

einen Durchmesser von 1µm und eine Periode von 3µm. Die magnetische<br />

Hysterese wurde mit Bragg-MOKE und mit resonanter magnetischer<br />

Röntgenstreuung (XRMS) an der Co L2,3 bei verschiedener Ordnung der<br />

Interferenz bestimmt. Bragg-MOKE liefert eine Fourieranalyse des Magnetisierungsprofils<br />

während des Ummagnetisierungs-prozesses. Analog<br />

dazu liefern auch Hysteresen, die mit XRMS an verschiedenen Ordnungen<br />

von Bragg-Reflexen gemessen werden, eine Fourieranalyse der Ummagnetisierung.<br />

Im Vergleich zu Bragg-MOKE zeichnet sich XRMS durch<br />

Elementspezifität und durch höhere Eindringtiefen aus. Wir präsentieren<br />

erste Ergebnisse, die mit Bragg-MOKE und XRMS an strukturierten<br />

Co/CoO Proben gewonnen wurden, und vergleichen die Ergebnisse.<br />

Gefördert durch SFB 491.<br />

O 12.2 Mo 16:00 H45<br />

Spin effects in Coulomb blockade of Fe/MgO/Fe — •Wulf<br />

Wulfhekel 1 , F. Zavaliche 1,2 , M. Klaua 1 , C.C. Kuo 1,3 , M.T.<br />

Lin 1,3 , and J. Kirschner 1 — 1 MPI für Mikrostrukturphysik, Weinberg<br />

2, 06120 Halle — 2 Departement de physique, Universite de Montreal,<br />

Quebec H3C 3J7, Canada — 3 Department of Physics, National Taiwan<br />

University, Taipei 106, Taiwan<br />

The Coulomb blockade (CB) of nanometer sized Fe islands grown on<br />

single crystalline MgO films on Fe(001) was studied using scanning tunneling<br />

microscopy (STM) at 25 K in ultra high vacuum. After deposition<br />

of 3-4 monolayers (ML) MgO, a sub-ML amount of Fe was deposited<br />

leading to the formation of Fe islands on the MgO films as observed by<br />

STM. Scanning tunneling spectroscopy was then used to locally measure<br />

the tunneling characteristics for tunneling from the tip via the island<br />

into the Fe substrate. The I(V) curves showed the characteristic steps of<br />

CB. The position of the steps in the I(V) characteristics of periodicity<br />

UC are proportional to the Coulomb charging energy e/C, where e is<br />

the electron charge and C the islands capacitance. A plot of UC versus<br />

e/C for the Fe islands, where C was estimated from the island size as<br />

observed with STM, reveals a linear dependence in agreement with CB.<br />

We, however, observe a constant and positive offset in UC by 1 eV, which<br />

cannot be explained by spin independent tunneling. We propose a model<br />

for spin-dependent CB, that relates the offset to the exchange the additional<br />

electron feels in the Fe islands. No systematic offset in UC has<br />

been found for identical experiments with Pd islands indicating that the<br />

observed offset is related to the island material.<br />

O 12.3 Mo 16:15 H45<br />

Valence band electronic structure and chemical reactivity in<br />

MgO/Fe(100) and MgO/Co/Fe(100) oxide-metal interfaces<br />

grown on GaAs(100) — •Liu-Niu Tong 1 , Frank Matthes 1 ,<br />

and C.M. Schneider 2 — 1 Leibniz Institut für Festkörper- und<br />

Werkstoffforschung — 2 Institut für Elektronische Eigenschaften,<br />

Forschungszentrum<br />

O 13 Methodisches (Experiment und Theorie)<br />

The interface electronic structure of MgO/Fe(100) and MgO/Co/<br />

Fe(100) films epitaxially grown on GaAs(100) was studied by employing<br />

spin-polarized photoemission spectroscopy (SPPES) and magnetic circular<br />

dichroism (MCD) techniques. With increasing excitation energy from<br />

30 eV to 60 eV, we observe an enhanced spectral intensity in the SPPES<br />

data of pure Fe for transitions from bulk ∆ 1 and ∆ 5 initial states near<br />

the Fermi energy that is accompanied with an increase in the detected<br />

spin polarization. After covering the Fe(100) surface by 0.5 ML MgO,<br />

the shape of the Fe ∆ 5 minority-spin peak becomes significantly broadened,<br />

while the shape of the Fe ∆ 1 majority-spin peak is only weakly<br />

affected. Additionally, we observed that 1 ML MgO on top of Fe(100)<br />

suppresses almost all contribution from the Fe ∆ 5 minority transition in<br />

the measured spin polarization data. This observed effect is especially<br />

strong for an excitation energy of 40 eV. Furthermore, our MCD data<br />

show that the O 2p peak is shifting towards the Fermi level as a function<br />

of time after preparation, indicating a slow change in the film chemistry.<br />

This chemical reaction can also be seen for MgO/Fe samples that were<br />

immediately covered after preparation with an additional Fe film on top.<br />

O 12.4 Mo 16:30 H45<br />

X-ray magnetic circular dichroism sum rule correction for the<br />

light transition metals — •Eberhard Goering — Max-Planck-<br />

Insitut für Metallforschung, 70569 Stuttgart<br />

Quantum mechanical mixing of the L2 and L3 edge excitations strongly<br />

increases with reduced 2p spin-orbit-splitting. For a large number of<br />

2p→3d absorption spectra the shape has been fitted nearly perfectly by a<br />

model, which takes into account lifetime and jj-mixing effects. X-ray magnetic<br />

circular dichroism (XMCD) sum rule correction factors have been<br />

determined for V and Cr, which are consistent to complementary investigations.<br />

This fitting procedure and the estimated correction factors are<br />

the basis for a future light element XMCD effective spin renormalization<br />

technique.<br />

O 12.5 Mo 16:45 H45<br />

Spin-resolved inverse photoemission with improved energy resolution<br />

— •Michael Budke, Volker Renken, Helmut Liebl,<br />

Georgi Rangelov, and Markus Donath — Physikalisches Institut,<br />

Universität Münster, Wilhelm-Klemm-Str. 10, 48149 Münster<br />

Spin-resolved inverse photoemission (IPE) is a powerful tool that measures<br />

the spin-dependend electronic structure above the Fermi level of<br />

magnetic surfaces and thin films. We have developed a source for spinpolarized<br />

electrons with variable energy resolution from 150 meV to 400<br />

meV (FWHM) at currents between 0.5 µA and 5 µA on the sample. The<br />

photon detector consists of a conventional Geiger tube filled with either<br />

acetone or iodine [1,2]. MgF2 is used as entrance window, followed by a<br />

SrF2- or CaF2-window. The transmission cutoff was shifted by varying<br />

the temperature of the windows. With this arrangement the energy resolution<br />

of the counters is continuously variable between 150 meV and 400<br />

meV (FWHM). Depending on the experimental requirements the total<br />

energy resolution of our IPE system can therefore be varied between 500<br />

meV and nearly 200 meV. The latter value is an improvement of the<br />

energy resolution by a factor of two compared to previous spin-resolved<br />

IPE systems [3]. [1] Dose V., Appl. Phys. 14, 117 (1977) [2] Funnemann<br />

D., Merz H., J. Phys. E: Sci. Instrum. 19, 554 (1986) [3] Dose V., Fauster<br />

T., Schneider R., Appl. Phys. A 40, 203 (1986)<br />

Zeit: Montag 17:00–17:30 Raum: H45<br />

O 13.1 Mo 17:00 H45<br />

Experimente mit kinematischen stehenden Röntgenwellen an<br />

CaF2/Si(111) — •Martin Tolkiehn 1 , Dmitri V. Novikov 1 und<br />

Cunrang Wang 2 — 1 HASYLAB am DESY, Notkestraße 85, D-22603<br />

Hamburg — 2 Institut für Halbleiterbauelemente und Werkstoffe, Universität<br />

Hannover, Appelstraße 11A, D-30167 Hannover<br />

Die Methode der stehenden Röntgenwellen (XSW) ist sehr gut geeignet<br />

zur Bestimmung der Position von Adsorbatatomen an Oberflächen<br />

und Dotieratomen in perfekten Kristallen [1,2]. Sie beruht auf der Ver-<br />

änderung der Phase des stehenden Wellenfelds in der Nähe eines Bragg–<br />

Reflexes, die mit Hilfe der dynamischen Theorie der Röntgenbeugung<br />

berechnet wird. Die Anwendung dieser Theorie auf nicht perfekte Kristalle<br />

ist ohne weiteres nicht möglich. Das stehende Wellenfeld ist jedoch<br />

auch noch bei größeren Abweichungen vom Braggwinkel vorhanden, bei<br />

denen die kinematische Näherung gilt.<br />

Wir zeigen theoretisch und experimentell am Beispiel CaF2/Si(111)<br />

[3], daß sich der Bereich fern vom Bragg–Winkel zur Bestimmung der<br />

Adsorbatposition nutzen läßt und dasselbe Ergebnis liefert wie die kon-

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